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Tiêu đề Guidance on the interpretation of carbon dioxide and 2-furfuryl dehyde as markers of paper thermal degradation in insulating mineral oil
Trường học International Electrotechnical Commission
Chuyên ngành Electrical and Electronic Technologies
Thể loại Technical Report
Năm xuất bản 2015
Thành phố Geneva
Định dạng
Số trang 28
Dung lượng 0,95 MB

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IEC TR 62874 Edition 1 0 201 5 05 TECHNICAL REPORT Guidance on the interpretation of carbon dioxide and 2 furfuraldehyde as markers of paper thermal degradation in insulating mineral oil IE C T R 6 2[.]

Trang 1

IEC TR 62874

Editio 1.0 2 15-0

Guidance on t he int erpret at ion of carbon dioxide and 2- fur uraldehyde as

markers of paper t hermal degradat ion in insulat ing mineral oi

Trang 2

THIS PUBLICATION IS COPYRIGHT PROTECTED

Copyr ight © 2 15 IEC, Ge e a, Switzer la d

Al rig ts r es r ve Unle s oth rwis s e ifi d, n p rt of this p blc tio ma b r epr od c d or uti z d in a y form

or b a y me n , ele tr onic or me h nic l in lu in p oto o yin a d microfim, with ut p rmis io in wr itin from

eith r IEC or IEC's memb r Natio al Commite in th c u tr y of th re u ste If y u h v a y q e tio s a o t IEC

c p r i ht or h v a e q ir y a o t o tainin a ditio al ri hts to this p blc tio , ple s c nta t th a dr es b low or

y ur lo al IEC memb r Natio al Commite for ur th r informatio

Th Intern tio al Ele trote h ic l Commis io (IEC) is th le din glo al org niz tio th t pr ep res a d p bls e

Internatio al Sta d r ds for al ele tri al ele tr onic a d relate te h olo ie

Abo t IEC p blc tio s

Th te h ic l c nte t of IEC p blc tio s is k pt u d r c n ta t r eview b th IEC Ple s ma e s re th t y u h v th

late t e itio ,a c rr ig n a or a ame dme t mig t h v b e p bls e

IEC Cat alo ue - webst ore.e ch/ cat alo ue

Th st an -alo e a plc t io for c n ultin th e tire

biblo ra hic l informat io o IEC Intern tio al Sta d rd ,

Te h ic l Sp cific tio s, Te h ic l R ep rts a d oth r

d c me ts A v aia le for P , Ma OS, A ndroid Ta let s a d

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IEC p blc t i ns s arch - www ie ch/ se rch u

Th a v an e s arc e a le t o fin IEC p blc t io s b a

variety of crit eria (efere c n mb r, t ext, t ec nic l

c mmitt e,…) It als gives informatio o projec t s, re la e

a d wit hdrawn p blc tio s

IEC Just P blshed - webst ore.e ch/ just pu lshed

St ay u to d te o al n w IEC p blc tio s Ju t Pu ls e

d t ais al n w p blc t io s rele s d A v aia le o ln a d

als o c a mo t h b emai

Ele t ro edia - www ele t ro edia.org

Th world's le din o ln dic t io ary of elec t ro ic a d

ele t ric l t erms c ntainin more t ha 3 0 0 terms a d

d finitio s in En ls a d Fre c , wit h e uiv ale t t erms in 15

a ditio al la g a e Als k nown a t he Int ern t io al

Elec t rot ec nic l Vo a ulary (IEV ) o ln

IEC Glos ar y - st d.e ch/ glos ary

More t ha 6 0 0 ele t rot ec nic l termin lo y e t rie in

En ls a d Fre c e tra t ed fom t he Terms a d Definitio s

cla s of IEC p blc t io s is u d sin e 2 0 Some e t rie

h v e b e c le t ed fom e rler p blc tio s of IEC TC 3 ,

7 ,8 a d CISPR

IEC Cust omer Servic Cent re - webst ore.ec ch/ csc

If y ou wis to giv e u your fe d a k o t his p blc tio or

n e furt her a sista c , ple s c nta t t he Cu tomer Serv ic

Ce t re:c c@ie c

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IEC TR 62874

Edit io 1.0 2 15-0

Guidance on t he int erpret at ion of carbon diox ide and 2- fur uraldehyde as

markers of paper t hermal degradat ion in insulat ing mineral oi

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FOREWORD 4

INTRODUCTION 6

1 Sco e 7

2 Normative ref eren es 7

3 Sig if i an e 8

3.1 General 8

3 2 Thermal an mec anical degradation of p p r

8 3.2.1 General 8

3.2.2 Imp ct of temp rature 8

3.2.3 Imp ct of h midity an ox gen 9

3.3 Symptoms of p p r agein in in ulatin oi 10 3.3.1 General 10 3.3.2 Volati e by-prod cts 1

3.3.3 Soluble by-prod cts 1

3.3.4 In oluble by-prod cts 1

3.4 Op rational p rameters in uen in p p r thermal agein 1

3.5 Role of oi typ an con ition 12 3.6 F ult con ition that may af fect thermal agein 12 3 7 Maintenan e o eration that may aff ect thermal agein in icators 1

3 3.7.1 General 13 3.7.2 Ef fects of oi recon itionin 13 3.7.3 Ef fects of oi reclamation 13 3.7.4 Ef fects of oi c an e 13 4 Monitorin protocol 14 4.1 General 14 4.2 Parameters 14 4.2.1 Basic monitorin 14 4.2.2 Complementary monitorin 14 4.3 Recommen ed testin f req en ies 14 5 Typical values of p p r agein s mptoms 15 5.1 General 15 5.2 F mi es of eq ipment 15 6 Estimation of p p r thermal degradation an agein rate 16 6.1 General a pro c 16 6.2 Practice 16 7 Action 17 An ex A (informative) Typical values ta les 19 A.1 General warnin 19 A.2 2-FAL typical values 19 A.2.1 General 19 A.2.2 F miy: GSU (generation ste -up u its) 19 A.2.3 F miy: network tran mis ion u its 2

A.2.4 F miy: large distribution u its 2

A.2.5 F miy: in u trial distribution u its 2

A.2.6 F miy: LVDC u its 21

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A.3 Carb n dioxide typical values 21

A.3.1 General 21

A.3.2 F mi y: GSU (generation ste -up u its) 21

A.3.3 F mi y: network tran mis ion u its 21

A.3.4 F mi y: large distribution u its 2

A.3.5 F miy: in u trial distribution u its 2

A.3.6 F miy: LVDC u its 2

Biblogra h 2

Fig re 1 – Sc ematic diagram s owin rate of agein k, de en in on dif ferent agein mec anisms 9

Fig re 2 – Relation hip b twe n mec anical pro erties of in ulatin p p r an p per degre of p lymerization (DP) [5] 10 Fig re 3 – Example of f low-c art f or the estimation of p p r degradation con ition 17 Ta le A.1 – 2-FAL typical values for GSU tran f ormers, fi ed with u in ibited mineral oi (b sed on a p pulation of 1 8 0 u its) 19 Ta le A.2 – 2-FAL typical values for GSU tran formers, f il ed with in ibited mineral oi (b sed on a p pulation of 17 units) 19 Ta le A.3 – 2-FAL typical values for network tran mis ion tran formers, fi ed with u in ibited mineral oi (b sed on a p pulation of 2 8 5 u its) 2

Ta le A.4 – 2-FAL typical values for large distribution tran formers, with o en bre thin con ervator, f il ed with u in ibited mineral oi (b sed on a p pulation of 7 10 u its) 2

Ta le A.5 – 2-FAL typical values for large distribution tran formers, with se led con ervator, fi ed with u in ibited mineral oi (b sed on a p pulation of 2 8 u its) 2

Ta le A.6 – 2-FAL typical values for in u trial distribution tran formers, fi ed with u in ibited mineral oi (b sed on a p pulation of 3 8 5 u its) 2

Ta le A.7 – 2-FAL typical values for LVDC tran formers, f il ed with u in ibited mineral oi (b sed on a p pulation of 3 0 u its) 21

Ta le A.8 – CO 2 typical values for GSU an ex itation tran f ormers, fi ed with u in ibited mineral oi (b sed on a p pulation of 1 0 8 u its) 21

Ta le A.9 – CO 2 typical values for network tran mis ion tran f ormers, fi ed with u in ibited mineral oi (b sed on a p pulation of 4 5 u its) 21

Ta le A.10 – CO 2 typical values for large distribution tran formers, f iled with u in ibited mineral oi (b sed on a p pulation of 7 2 1 u its) 2

Ta le A.1 – CO 2 typical values for in u trial distribution tran formers, fi ed with u in ibited mineral oi (b sed on a p pulation of 4 5 6 u its) 2

Ta le A.12 – CO 2 typical values for LVDC tran f ormers, fi ed with u in ibited mineral oi (b sed on a p pulation of 2 3 u its) 2

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INTERNATIONAL ELECTROTECHNICAL COMMISSION

1 Th Intern tio al Ele trote h ic l Commis io (IEC) is a worldwid org niz tio for sta d rdiz tio c mprisin

al n tio al ele trote h ic l c mmite s (IEC Natio al Commite s) Th o je t of IEC is to promote

intern tio al c -o eratio o al q e tio s c n ernin sta d rdiz tio in th ele tric l a d ele tro ic f i ld To

this e d a d in a ditio to oth r a tivitie , IEC p bls e Intern tio al Sta d rd , Te h ic l Sp cific tio s,

Te h ic l Re orts, Pu lcly Av ia le Sp cif i atio s (P S) a d Guid s (h re f ter refer e to a “IEC

Pu lc tio (s)”) Th ir pre aratio is e tru te to te h ic l c mmite s; a y IEC Natio al Commite intere te

in th s bje t d alt with ma p rticip te in this pre aratory work Intern tio al g v rnme tal a d n n

-g v rnme tal org niz tio s laisin with th IEC als p rticip te in this pre aratio IEC c la orate clo ely

with th Intern tio al Org niz tio f or Sta d rdiz tio (ISO) in a c rd n e with c n itio s d termin d b

a re me t b twe n th two org niz tio s

2) Th f ormal d cisio s or a re me ts of IEC o te h ic l maters e pre s, a n arly a p s ible, a intern tio al

c n e s s of o inio o th rele a t s bje ts sin e e c te h ic l c mmite h s re re e tatio fom al

intere te IEC Natio al Commite s

3) IEC Pu lc tio s h v th form of re omme d tio s f or intern tio al u e a d are a c pte b IEC Natio al

Commite s in th t s n e Whie al re s n ble ef forts are ma e to e s re th t th te h ic l c nte t of IEC

Pu lc tio s is a c rate, IEC c n ot b h ld re p n ible for th wa in whic th y are u e or f or a y

misinterpretatio b a y e d u er

4) In ord r to promote intern tio al u if ormity, IEC Natio al Commite s u d rta e to a ply IEC Pu lc tio s

tra s are tly to th ma imum e te t p s ible in th ir n tio al a d re io al p blc tio s An div rg n e

b twe n a y IEC Pu lc tio a d th c re p n in n tio al or re io al p blc tio s al b cle rly in ic te in

th later

5) IEC its lf d e n t pro id a y ate tatio of c nf ormity In e e d nt c rtific tio b die pro id c nf ormity

a s s me t s rvic s a d, in s me are s, a c s to IEC mark of c nf ormity IEC is n t re p n ible f or a y

s rvic s c rie o t b in e e d nt c rtific tio b die

6) Al u ers s o lde s re th t th y h v th late t e itio of this p blc tio

7) No la i ty s al ata h to IEC or its dire tors, emplo e s, s rv nts or a e ts in lu in in ivid al e p rts a d

memb rs of its te h ic l c mmite s a d IEC Natio al Commite s f or a y p rs n l injury, pro erty d ma e or

oth r d ma e of a y n ture wh ts e er, wh th r dire t or in ire t, or for c sts (in lu in le al f ee ) a d

e p n e arisin o t of th p blc tio , u e of, or rela c u o , this IEC Pu lc tio or a y oth r IEC

Pu lc tio s

8) Ate tio is drawn to th Normativ refere c s cite in this p blc tio Us of th refere c d p blc tio s is

in is e s ble for th c r e t a plc tio of this p blc tio

9) Ate tio is drawn to th p s ibi ty th t s me of th eleme ts of this IEC Pu lc tio ma b th s bje t of

p te t rig ts IEC s al n t b h ld re p n ible f or id ntif yin a y or al s c p te t rig ts

The main tas of IEC tec nical commit e s is to pre are International Stan ard However, a

tec nical commit e may pro ose the publ cation of a Tec nical Re ort when it has col ected

data of a diff erent kin f rom that whic is normaly publs ed as an International Stan ard, f or

example "state of the art"

IEC TR 6 8 4, whic is a Tec nical Re ort, has b en pre ared by IEC tec nical commit e

10: Fluid f or electrotec nical a pl cation

The text of this stan ard is b sed on the f ol owin doc ments:

En uiry draft Re ort o v tin

Ful information on the votin for the a proval of this Tec nical Re ort can b f ou d in the

re ort on votin in icated in the a ove ta le

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This publ cation has b en draf ted in ac ordan e with the ISO/IEC Directives, Part 2.

The commit e has decided that the contents of this publ cation wi remain u c an ed u ti

the sta i ty date in icated on the IEC we site u der "ht p:/webstore.iec.c " in the data

related to the sp cif i publ cation At this date, the publ cation wi b

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The cel ulosic sol d in ulation of tran f ormers an other electrical a p ratu is s bject to

thermal degradation d rin their o erational lfetime This res lts in a progres ive los of

p p r’s mec anical pro erties, s c as ten i e stren th, whic are related to the d ration of

the tec nical l fe of the eq ipment [3,4]

1

Durin its thermal degradation proces (also cal ed “agein ” in this Tec nical Re ort ,

cel ulose forms several by-prod cts, some of whic may b detected by me n of in ulating

oi s c emical analy is [1,2] The con entration an rate of in re se of those by-prod cts can

b u ed as a to l to estimate the progres of p p r thermal degradation in tran f ormers an

other electrical a p rata in service

For this re son, IEC tec nical commit e 10 has pre ared this Tec nical Re ort for the

monitorin of in ulatin oi p rameters related to celulose agein an the interpretation of

res lts, as a g idan e to the thermal degradation evaluation of in ulatin p p r

This Tec nical Re ort is b sed on the evaluation of cel ulose agein by-produ ts content in

in ulatin oi , an their rate of f ormation d rin the l fe of the oi-immersed electrical

eq ipment Statistical referen e values re orted in An ex A of this Tec nical Re ort are

b sed on data col ected by TC10 The final re ort of CIGRE WG D1.01.TF13 [7] was taken as

a source of inf ormation con ernin mec anisms an p rameters influen in the formation of

furanic comp u d

NOT Meth d f or th e timatio of a tu l d gre of p lymeriz tio (DP) v lu s of p p r, whic are wid ly

a aia le in lterature, were n t a ple within this Te h ic l Re ort This is d e to th f act th t a n mb r of

diff ere t mo els h v b e d v lo e a d re orte , a d th y of te le d to dif fere t re ults More v r, th

a plc bi ty of th s mo els h s n t b e s f ficie tly pro e b c mp ris n with f i ld e p rie c to b in lu e

into a IEC sta d rd

He lth a d s fety

This Tec nical Re ort do s not purp rt to ad res al the safety pro lems as ociated with its

u e It is the resp n ibi ty of the u er of the Tec nical Re ort to esta ls a pro riate he lth

an safety practices an determine the a pl ca i ty of reg latory l mitation prior to u e

The mineral oi s whic are the s bject of this Tec nical Re ort s ould b han led with d e

regard to p rsonal saf ety an h giene Direct contact with eyes may cau e sl g t ir itation In

the case of eye contact, ir igation with co iou q antities of cle n ru nin water s ould b

car ied out an medical ad ice sou ht

Some of the tests sp cified in this Tec nical Re ort in olve the u e of proces es that could

le d to a hazardou situation At ention is drawn to the relevant stan ard f or guidan e

En ironme t

This Tec nical Re ort in olves mineral oi s, c emicals an u ed sample containers The

disp sal of these items s ould b car ied out in ac ordan e with c r ent national legislation

with regard to the imp ct on the en ironment Every precaution s ould b taken to prevent the

rele se into the en ironment of mineral oi

_ _ _ _ _ _

1

Fig re in s u re bra k ts refer to th Biblo ra h

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GUIDA NCE ON THE INTERPRETA TION OF CARBON DIOXIDE

IEC TR 6 8 4, whic is a Tec nical Re ort provides g idan e f or the estimation of con umed

thermal l f e of tran formers' cel ulosic in ulators, throu h the analy is of some comp u d

dis olved in the in ulatin mineral oi A comp rison b twe n analytical res lts of 2-f urf ural

(2-FAL) an carb n oxides an their cor esp n ent typical values estimated f or diff erent

f ami es of eq ipment gives information on the estimated thermal degradation of p p rs

The agein rate of in ulatin p p rs can b evaluated, in s ort time ran es (e.g 1 ye r), by

reg larly monitorin 2-FAL an carb n oxides content in the oi an by comp rin them to

typical rates of in re se

A statistical a pro c for the estimation of p p r thermal degradation, an the evaluation of

agein rate is given

Typical values for con entration an rates of in re se of the p rameters related to p p r

agein were extra olated f rom a statistical data ase col ected, an are re orted in An ex A

They may b u ed as a rou h g ide, but they s ould not b con idered as thres old values

This Tec nical Re ort is only a pl ca le to tran formers an re ctors f il ed with in ulatin

mineral oi s an in ulated with Kraft p p r The a proac es an proced res sp cified s ould

b taken as a practical g idan e to in estigate the thermal degradation of cel ulosic

in ulation, an not as an algorithm to calc late the actual degre of p lymerization (DP) of

p p rs

The p p r thermal l fe evaluation protocol des rib d in this Tec nical Re ort a pl es to

mineral oi impreg ated tran formers an re ctors, in ulated with Kraf t p p r An eq ipment

f il ed with in ulatin lquid other than mineral oi (i.e esters, si cones) or in ulated with sold

materials other than Kraft p p r (i.e TUP – thermal y upgraded Kraf t p p r, s nthetic

p lymers) is outside of the s o e of this Tec nical Re ort

This Tec nical Re ort is a pl ca le to eq ipment that has b en s bmit ed to a reg lar

monitorin practice d rin the service, an for whic maintenan e an f ault history is k own

The f ol owin doc ments, in whole or in p rt, are normatively ref eren ed in this doc ment an

are in isp n a le f or its a pl cation For dated ref eren es, only the edition cited a ples For

u dated referen es, the latest edition of the referen ed doc ment (in lu in an

amen ments) a pl es

None

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3 Signif icanc

This Tec nical Re ort des rib s a statistical a pro c to p p r thermal l f e evaluation This

me n that al typical values are o tained f om p pulation of tran formers b lon in to the

same fami y for tec nical c aracteristic an a pl cation (se An ex A)

The a pro c u ed to col ect statistical data, des rib d in 6.1, can b a pl ed by uti ties or

owners havin a large p pulation of u its, to calc late in ivid al ref eren e values related to a

sp cific fami y of tran f ormers or re ctors This is very imp rtant b cau e dif ferent p pulation

of tran f ormers (i.e o eratin in dif ferent clmates or u der diff erent o erational con ition )

may have dif ferent typical values

NOT For a e te siv s rv y o fura ic c mp u d a mark rs f or dia n sis of p p r in ulatio d gra atio ,

s e CIGRE Bro h re 4 4/2 12[7]

3.2 Thermal a d me ha ic l de ra ation of paper

There are main factors: desig an materials, contaminants in the in ulation s stem an

o erational con ition , that wi determine the agein of a tran former [1,2] F r the sold

in ulation – p p r an pres b ard – it me n a combination of mec anical an dielectric

p rorman e, whic are interl n ed an s nergetic F r a tran f ormer, in the context of

thermal agein , it is the mec anical stren th of the p p r that mat ers The agein of p p r

res lts in a decre sed mec anical stren th an is as umed to red ce the a i ty of the

tran former to with tan s ort circ it stres This, however, has not b en statistical y

demon trated, yet

Ten i e stren th, elon ation an foldin stren th al decay with time, an more q ic ly at

hig er temp ratures

The mec anical p r orman e of cel ulosic in ulation is given in terms of ten i e in ex or

degre of p lymerization (DP), whic are stron ly influen ed by agein The DP value is an

average value of c ain len th of the cel ulose molec les given as a n mb r of glu ose rin s

in a cel ulose c ain It is me s red throu h me s rement of the vis osity of a p p r solution,

ac ordin to IEC 6 4 0 [8]

It is more con enient to p rf orm DP than ten i e in ex, b cau e of the lmited amou t of

p p r ac es ible f or tests; theref ore it is widely u ed for the evaluation of the cel ulosic

3.2.2 Impa t of temperature

Temp rature af fects the rate of degradation This fact is reflected in IEC 6 0 6-7 [3] an

IEEE Std C5 91 [4] tran former lo din g ides

IEC 6 0 6-7 [3] s g ests in ac ordan e with Montsin er that the lfe of a tran former can b

Trang 11

p is a con tant (a value of 6 is s g ested in the ran e 8 °C to 14 °C)

θ is the temp rature in degre s Celsiu

This is a simpl f ied version of Ar heniu law u ed in IEEE Std C5 91 [4]

Sin e a precise en -of lne criterion f or a tran former is not re l y avai a le, IEEE an IEC

stan ard u e an a pro c where agein rate is con idered This is the in erse of l f etime –

in Montsin er f orm:

Rate of a eing = c nstant

θ

×p

(2)

The con tant in Eq ation (2) is de en ent on man p rameters, e.g original q alty of

cel ulosic prod cts as wel as environmental p rameters (moisture content and ox gen in the

s stem) A gra hical re resentation of these influen es is s own in Fig re 1

Fig re 1 – Sc ematic dia ram s owing rate of a eing k,

depe ding on dif f ere t a eing me ha isms

3.2.3 Impa t of h midity a d ox ge

Humidity an ox gen in res (oxidation) have an imp rtant imp ct on the agein of Kraft

p p r This me n not only that the mec anical stren th of p p r ra idly decre ses u der

in res of moisture an air, but practical y cau es an in re sin contamination of the

combined l q id-sol d in ulation u der these con ition It is a con eq en e of the

degradation prod cts formed f rom oi an p p r le din to a f urther degradation

Durin the agein of the combined cel ulosic an oi in ulation man by-prod cts are formed –

carb n oxides, water, acid , slu ge an furanic comp u d Man of these degradation

prod cts, e.g furanic comp u d , are soluble in oi an sta le enou h to b u ed as

diag ostic markers Furanic are f ormed by deh dration re ction fol owin h droly is of the

cel ulose an hemicel ulose as wel as by oxidative pyroly is of cel ulose Their analytical

determination is wel k own an rela le (se IEC 61 9 [12])

In a tran f ormer al these proces es – h droly is, oxidation an pyroly is – act

simultane u ly, res ltin in a non-l ne r mec anism (se Fig re 1) Whic proces wi

dominate de en s on the temp rature an the o erational p rameters In fact the a plcation

of one activation energy, althou h of ten practiced, is very dif fic lt b cau e of the complexity

of the degradation proces es

IEC Oxid tio

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3.3 Symptoms of paper a eing in in ulating oi

The agein of p p r can b detected by direct in estigation on the p p r or by the

me s rement of by-prod cts dis olved in the oi

Cel ulose degradation mainly af fects the mec anical pro erties ( en i e stren th, elon ation,

burst stren th, double f old stren th, etc.) of p p r (se Fig re 2), but a direct me s re of

those p rameters req ires the sampl n of a large amou t of p p r, whic is normal y

imp s ible d rin the o erational l f etime of a tran former However, the relation hip b twe n

the mec anical in exes an the degre of p lymerization (DP) is wel k own Degradation of

p p r do s not sig ificantly aff ect its resistan e to the compres ion f orces mostly an

contin ou ly a pl ed to tran former win in s throu h clampin

Figure 2 – Relations ip betwe n me ha ic l propertie of

ins latin paper a d paper de re of polymerization (DP) [5]

The DP value is the average n mb r of gly oside rin s in the cel ulose p lymer; in the native

cel ulose DP may b as hig as or more than 10 0 0 u its but after the purification proces

an other tre tments the DP value of the electrical Kraft p p r decre ses to arou d

1 0 0 u its ( ypical value: 1 2 0)

DP is me s red in ac ordan e with IEC 6 4 0 [8] throu h me s rement of the sp cific

vis osity of a very smal amou t of p p r dis olved in c pri-eth lene-diamine (CuED) From

this me s rement the intrin ic vis osity of solution is ded ced an f rom this, u in the

Martin’s formula, the DP value is e si y calc lated

By-prod cts of aged p p r may b clas ified as volati e, soluble an in oluble, an are

de en ent on the sp cif i decomp sition proces : pyroly is, h droly is or oxidation

Relativ d gre of p lymerisatio

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3.3.2 Volati e by-products

Carb n oxides (CO an CO

2) are the ultimate prod cts of cel ulose degradation an are

me s red with dis olved gas analy is (DGA) in ac ordan e with IEC 6 5 7 [9] It mu t b

taken into ac ou t that b th CO an CO

2can b generated fom oi oxidation as wel

Water can re c several p r cent of the p p r weig t Most of the water f ormed is ad orb d

an retained in the sol d in ulation of the tran f ormer an only a l tle p rt is dis olved in oi

Of course another contribution to total water is the in res of moisture f rom atmosphere

The detection of water in oi is p rf ormed in ac ordan e with IEC 6 814 [10]

3.3.3 Soluble by-products

A large n mb r of oi soluble comp u d (acid , alcohols, etc.) are generated f rom p p r

degradation The most commonly u ed comp u d for diag osis is 2-f urf ural (2-FAL) an its

related comp u d :

– 5 hy rox meth l 2- urural (5-HMF)

– 2 f ururylalcohol (2-FOL)

– 2 acetylfuran (2-ACF)

– 5 meth l 2-f urf ural (5-MEF)

The detection of 2-FAL an related comp u d in oi is p r ormed in ac ordan e with

IEC 61 9 [12]

In the same way as with water, a relevant amou t of generated furanic comp u d is retained

in the bulk of the p p r The ratio b twe n the con entration of furanic comp u d in the

p p r an in the oi dif fers for e c sin le comp u d, an is aff ected by temp rature

In reased temp rature forces the eq i brium of f uranic comp u d to a hig er con entration

in the oi Decre sed temp rature forces the eq i brium of f uranic comp u d to a hig er

con entration in the p p r, especial y in the case of dry p p r

Pa er h midity an typ of p p r also in uen e the oi -to-p p r con entration ratio of furanic

comp u d A wet p p r ten s to retain a larger amou t of furanic comp u d , th s red cin

the oi -to-p p r con entration ratio

Furanic comp u d are not hig ly sta le, an may b degraded by oxidation, mostly in ois

with hig ox gen content Decay in the con entration of 2-FAL was o served in tran formers

d rin their o eration, d e to its in erent in ta i ty

Acid comp u d may b f ormed either by celulose an /or oi oxidation, an a hig acidity

of ten ac omp nies other s mptoms of p p r agein

3.3.4 In oluble by-products

Severe p p r agein can final y le d to the f ragmentation of p lymeric celulose, an smal

p p r fibres can b detac ed fom the p p r mas

The celulose f ibres can b detected as p rticles present in in ulatin oi , in ac ordan e with

IEC 6 9 0 [1 ]

3.4 Operational parameters influe cing paper th rmal a ein

In ad ition to tran former hours of service as a key p rameter in def i in “re l age” of p p r

in ulation in normal workin regimes, other o erational p rameters s c as lo d, typ of

co l n an tran f ormer s b-typ have a major in uen e on p p r thermal agein The nature

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The hig -lo d of a tran former, implyin elevated o eratin temp ratures, promotes the p p r

thermal degradation proces , o served with some typ s of tran formers that are of ten

overlo ded (s u t re ctors, HVDC, generator ste -up (GSU) in thermal p wer plants (TPP),

hig voltage inter tie tran mis ion tran formers)

The typ of co ln , in terms of co l n media (water or air) an typ of flow a pl ed (forced or

natural con ection), aff ects eff i ien y of he t removal, th s influen in the rate of p p r

thermal degradation The most ef ficient co l n can b ac ieved by a plyin water as co lant

in f orced oi flow

For example, it was o served in most cases that the degre of p p r degradation with GSU

tran formers in hy ro p wer plants (HPP) is lower than with thermal p wer plant GSU u its,

havin a simi ar service d ration These fin in s are cor elated to dif ferent types of co l n

(OFWF vers s ONAF an OFAF), hours of service an lo din history of HPP an TPP u its

[6]

Amon dif ferent tran f ormer s b-typ s, air bre thin tran formers are s bjected to more

inten ive p p r degradation than se led ones, d e to hig er ox gen an moisture content

Elevated con entration of ox gen an water ac elerate the p p r degradation proces

Sin e the p p r degradation proces is temp rature driven, every en ironmental an

o erational con ition that may aff ect the temp rature can also modify the degradation rate of

the sol d in ulation An elevated en ironmental temp rature or a hig lo din can th s

in rease the rate of p p r degradation, res ltin in a s d en in re se of 2-FAL, CO

2, CO an

other by-prod cts

3.5 Role of oi type a d condition

Oi typ may af fect the agein rate of p p r In ibited oi s s ow a lower ten en y to form

acidity, an the oxidation proces is slac ened; the ef fect of ox gen in the p p r oxidation

proces is red ced

Tran formers impreg ated with in ibited oi may s ow a lower content of 2-FAL if comp red

with u its in ulated with an u in ibited oi , even if s owin the same degre of p lymerization

(DP) of the p p r

The ef fect of p s ivators ( riazole derivates) in the agein of celuloses is sti not wel

defined By definition, metal p s ivators may in u e a lower rate of the oi degradation

proces by de ctivatin the co p r cataly t in oxidation proces es, theref ore slowin down

the p p r degradation proces , but in uen e of metal p s ivators on 2-FAL con entration in

the oi may not b straig tforward Some la oratory stu ies have s own that p p rs

impreg ated with oi s to whic a p s ivator has b en ad ed, may have a lower ten en y to

f orm f uranic comp u d ; this may le d to o timistic estimation of agein in presen e of

triazol c p s ivators

The agein con ition of the oi may also aff ect the p rtition of furanic comp u d b twe n

sol d and l q id in ulation; acidic oi s may res lt in an in re sed 2-FAL con entration in oi,

d e to its au mented ca a i ty to extract p lar comp u d f rom the p p r

3.6 Fa lt condition th t ma af f ect thermal a eing

In tran f ormers where the degradation mec anism may b either thermal or electrical, the rate

of p p r degradation may in re se ra idly as a con eq en e of sig ificant temp rature rise

Hig energ thermal an electrical f aults in olvin ex es ive c r ents circ latin throu h the

in ulation an large c r ent fol ow-throu h le d to exten ive destru tion an carb nization of

p p r

In presen e of local thermal degradation d e to a fault, the estimation of the p p r’s

con umed thermal l fe may b come very dific lt, sin e the exten ion of the p p r volume

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