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ENCYCLOPEDIA OF ENVIRONMENTAL SCIENCE AND ENGINEERING - RADON pdf

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Following the discovery of very high levels of indoor radon associated with homes in northeastern Pennsylvania in December of 1984, the New Jersey Department of Environmental Protection

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Following the discovery of very high levels of indoor

radon associated with homes in northeastern Pennsylvania

in December of 1984, the New Jersey Department of

Environmental Protection was designated as the lead state

agency to address the potential for radon problems in New

Jersey The Department was charged with characterizing the

problem as it might exist in New Jersey and developing a

coordinated state response to the problem

Due to the potentially serious public health implications

of exposure to high levels of radon, the characterization of

New Jersey’s radon problem proceeded simultaneously with

the development of a program to educate the public

regard-ing radon and respond to residents’ needs for reliable radon

testing and radon remediation services

The current data indicates that New Jersey’s indoor radon

levels are among the highest known and that as many as 1 6

million homes in New Jersey may be at risk for radon

prob-lems Approximately one-third of homes studied thus far

test at or above the 4 picocuries per liter guidance level

rec-ommended by the United States Environmental Protection

Agency as a feasible goal for remediation of high

concentra-tions of indoor radon New Jersey’s response to this problem

is characterized by an integrated multi-agency approach and

the growth of firms providing reliable, regulated radon

test-ing and remediation services in the private sector

BACKGROUND

Radon-222 is the single gaseous isotope among the fourteen

principal decay products composing the 4n + 2 natural decay

series beginning with uranium-238 and terminating in

lead-206 The principal decay products of this series, their half

lives and principal associated emissions are given in Table 1.1

The atmospheric concentration of radon varies with

loca-tion, but is typically on the order of 0.1 picocuries per liter

(0.1 pCi/1) over land masses. 2 The average radon

concentra-tion indoors in the United States in not well known, but has

been estimated 3 to be in the range of 1 to 2 pCi/1

In December of 1984, previously unheard of levels of

radon were found in the home of an engineer, Stanley Watras

who worked at the Limerick Nuclear Generating Station and

lived in the Boyertown, Pennsylvania area. 4 The engineer

had been tripping portal monitor radiation alarms

indicat-ing radioactive material on his clothindicat-ing when leavindicat-ing work

Investigations conducted by the utility and the Pennsylvania

Department of Environmental Resources demonstrated that the radioactive material on the engineer’s clothing consisted

of the short lived decay products of radon-222 (Po-218 through Po-214 in Table 1) which had originated in his home

The concentrations of radon in the home ranged as high as 2,600 pCi/1 Subsequent investigations of the area around the discovery home demonstrated that elevated levels of indoor radon were common to the area and that the probable source

of the radon was the underlying gramitec rock formation known as the Reading Prong. 5

In May of 1985, an article 6 by Phillip Shabecoff appeared

in the New York Times reporting the Watras incident and noting that the Reading Prong ran in a northeasterly direc-tion out of Pennsylvania, through northern New Jersey and into New York The article also identified an increased risk

of lung cancer as a possible outcome of exposure to elevated levels of radon and its decay products Immediately, state agencies in New jersey, particularly the Department of Environmental Protection, were deluged by telephone and written requests for information on radon and assistance in obtaining radon testing services

Numerous studies have demonstrated the link between exposure to radon and its decay products in mining situa-tions and an increased risk of lung cancer. 7 Research efforts directed at establishing a link between residential exposure

to radon and its decay products have been far more limited in scope than the mining studies and the data derived from them are, at best, equivocal. 8 Studies underway now in Sweden, New Jersey, Pennsylvania and New England may have suf-ficient power to elucidate the residential exposure risks

Based primarily on the results of the mining studies he United States Environmental Protection Agency (EPA) has estimated that from 5,000 to 20,000 of the 130,000 lung cancer deaths annually in the United States are attributable

to radon. 9 EPA has further estimated that 1 to 5 persons in

100 exposed in their homes to radon at 4 pCi/1 over a 70 year lifetime, with 75% occupancy, will develop lung cancer. 10 As this risk is assumed to be linear, the risk at 200 pCi/1 under similar conditions of exposure is estimated to be from 44 to

77 in 100 These risks are two or more orders of magnitude greater than other environmental health risk levels which traditionally trigger actions to reduce them

It is important to note that radon itself is not believed

to be the major contributor to the possible development of lung cancer. 11 As radon is an inert gas there is not preference for deposition with the body When radon decays in ambient

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air, however, the decay products formed are metals which

initially associated with aggregates of water molecules in the

air These aggregates in turn adhere to airborne dust

parti-cles When inhaled, the dust particles, if of appropriate size,

will preferentially deposit in the tracheobronchial region of

the lung Radioactive decay of the short lived alpha emitting

progeny of radon will result in intense local irradiation of

the tissue underlying the deposited dust It has been

calcu-lated that the vast majority of the total radiation dose to the

lung tissue is due to the alpha decay of Po-218 and Po-214. 12

It is this localized irradiation which is believed to trigger the

development of lung cancer

In order to have a radon problem in a home, three

conditions are necessary First, the immediate parent of

radon-222, radium-226, must be present in the underlying

soil or rock to yield a radon source term Second, the home

must have penetrations in the basement or the ongrade slab

which provide entry points for the gas Third, the pressure

inside the home must be less than the surroundings so as to

provide a pressure differential to facilitate the entry of radon

into the home The first condition is geologic in origin and

is met in many locations in the United States The second

condition is a typical consequence of standard construction

techniques, particularly in homes where a peripheral channel

in the basement slab and an associated sump pump are used

to control wet basement problems Other points of entry for radon in a home include unsealed openings around piping,

at or below grade, cracks in the walls and floor, and porous concrete The third condition is met by a combination of fac-tors which include the normal stack effect associated with the house, combusting fuels for heating, and the use of appli-ances such as dryers which are vented to the outside These conditions are met in homes in much of the northern portion

of New Jersey, and to a lesser extent, in specific locations in southern New Jersey

THE NEW JERSEY RADON PROGRAM

Shortly after the Watras incident, Pennsylvania Department

of Environmental Resources personnel contacted their coun-terparts in the New Jersey Department of Environmental Protection (DEP) to advise them of the problem In the beginning months of 1985, DEP staff working with the New Jersey Department of Health began to assess New Jersey’s potential for a radon problem and develop a response to it

TABLE 1 The Uranium Decay Series

Nuclide Half Life

Alpha Energy (MeV)

Beta Energy (MeV)

Gamma Energy (MeV)

0.24 (7%) 0.30 (9%) 0.35 (37%)

0.77 (5%) 1.12 (15%) 1.24 (6%) 1.38 (5%) 1.76 (15%) 2.20 (5%)

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A review of available data demonstrated that New Jersey

had significant potential for a random problem and that it was

likely that the problem would not be confined solely to New

Jersey’s section of the Reading Prong The National Uranium

Resource Evaluation data 13 indicated that significantly

ele-vated levels of uranium, and hence radon, could exist both

north and south of the Reading Prong Outside the Reading

Prong elevated levels of uranium were associated with

lime-stone, shales and clays Additionally, a literature survey 14

pre-viously conducted by the New Jersey Geological Survey had

found reports of more than 100 locations of radioactive

min-erals in New Jersey, many well outside the Reading Prong

Early State planning activities focused on the need to

edu-cate the public with regard to radon and develop legislation

providing specific programmatic mandates and associated

funding

In January of 1986, Governor Kean signed a bill providing

$3.2 million to begin New Jersey’s radon program A second

bill, signed into law in August of 1986, provided an additional

$1 million, mandated the development of certification for

testing and remediation firms and also guaranteed the

confi-dentiality of random test results The major components of the

radon program developed using this funding include:

Radon Information Program

By December 1, 1987 the DEP’s toll free information line

had received and responded to more than 52,000 telephone

inquiries As a result of these inquiries more than 20,000

informational packages have been mailed out to New Jersey

residents As the knowledge of radon has grown among New

Jersey residents so has the sophistication and complexity of

the telephone inquires Currently, a great deal of staff time is

spent providing telephone consultation to residents who wish

to discuss the interpretation of their radon test results or who

wish an in depth discussion of the relative effectiveness of

alternative remediation methods The Department of Health

also provides telephone consultation on specific health issues

related to radon The Department of Environmental Protection

and the Department of Health provide speakers for groups

interested in learning about radon By December 1, 1987,

more than 250 presentations have been made to interested

groups Also, a slide presentation on radon was developed for

use with general audiences throughout the state This slide

presentation is currently being expanded and re-packaged in

a video tape format for distribution to local libraries

Statewide Study of Radon

In 1986 the DEP contracted with the environmental

engi-neering firm of Camp, Dresser and McKee, Inc (CDM) to

perform a $1.3 million statewide study of radon The

spe-cific tasks within this study are to:

a Map areas of potential radon problems using all available geographic, geologic, radiometric and demographic data

b Develop a model to predict indoor radon exposure statewide

c Test the model developed in Task b using a sampling program including approximately 6,000 structures statewide

residents of the dangers posed by exposure to radon gas

collected in the study

f Propose and prioritize further research suggested

by the statewide study

g Provide a summary report containing the most salient findings of the study for presentation to the legislature and the public

Epidemiologic Study

The New Jersey Department of Health is conducting a case-control study of female lung cancer victims and case-controls

in New Jersey The primary aim of this study is to deter-mine whether or not the lung cancer risk estimates derived from studies of uranium and other miners are applicable to individuals exposed to radon in their homes The DEP has supported this effort by performing radon tests in more than

800 homes of cases and controls

Confirmatory Monitoring

As the radon program was being planned the spring of

1985, it was recognized that as many as 1.6 million New Jersey homes might be at risk for elevated levels of indoor radon It was clearly outside the resources of state govern-ment to offer free testing to each potentially affected house-hold Preliminary cost analyses of no-charge testing for 1.6 million homes indicated a cost ranging from $40 million

to $200 million A conscious decision was therefore made

to allow, and even assist in, the development of a radon test-ing industry in the private sector It was also recognized however, that the unregulated growth of such a new industry carried with it a significant potential for error and for con-sumer fraud Therefore, to protect New Jersey citizens, it was decided to offer confirmatory testing to those residents who had commercial radon tests performed in their homes and obtained radon concentrations equal to or greater than the 4 pCi/1 guidance level at which the EPA recommends consideration of remedial action

Certification of Radon Testing and Mitigation Firms

The DEP is in the process of promulgating regulations for the mandatory certification of radon testing and mitigation firms In the interim, a voluntary certification program has been implemented This program currently enrolls 58 radon testing firms and 24 radon mitigation firms Respectively, these total represent about one-half the number of firms applying for enrollment in the two programs The firms are required to document specific expertise, refrain from scare-tactic advertising, participate in the EPA Radon Proficiency

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Valley & Ridge

Average = 8.2 pCi/l

N = 634

Reading Prong

Average = 8.1 pCi/l

N = 1443

Pledmont

Average = 4.2 pCi/l

N = 2169

Inner Coastal Plain

Average = 2.5 pCi/l

N = 745

Outer Coastal Plain

Average = 1.8 pCi/l

N = 297

State

Average = 5.4 pCi/l

N = 5288

N = Number of Homes Tested

BERGEN

HUDSON ESSEX

UNION

MERCER

HUNTERDON

MIDDLESEX SOMERSET

MONMOUTH

GLOUCESTER

SALEM

BURLINGTON

CAMDEN

ATLANTIC

CUMBERLAND

CAPE MAY

WARREN

SUSSEX

PASSAIC

MORRIS

OCEAN

FIGURE 1 New Jersey Department of Environmental Protection, preliminary report on statewide radon study.

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Measurement Program 15 and meet other quality assurance

objectives

Follow-Up Testing

As residents tested for radon and remediated their radon

prob-lems, they requested access to reliable, unbiased radon

test-ing which would enable them to determine whether or not the

remediation methods employed were effective In response

to these requests, DEP began a program of testing

remedi-ated homes at no charge to the owner As of December 1,

1987, a total of 774 homeowners had availed themselves of

this service In general, these follow up tests document the

effectiveness of the remedial actions employed When they

do not, DEP staff advise both the homeowner and the

con-tractor and then assist in working out a mutually acceptable

solution

Radon Cluster Identification

In March of 1986, through the Confirmatory Monitoring

program, the DEP became aware of several homes in Clinton,

New Jersey which had unusually high concentrations of

indoor radon The DEP and Department of Health worked

closely with municipal and county officials to identify other homes in the area which also had very high radon levels

In one neighborhood in Clinton, 105 homes were found to

be above 4 pCi/1 Forty of the 105 homes were found to be above 200 pCi/1 and five of the forty homes were found to

be above 1000 pCi/1

Through the cooperation of government at all levels, what could have been a disaster for the community became

a solvable problem The DEP, the Department of Health and local officials provided information on radon and access to testing for those judged to be at significant risk The munici-pal government participated fully in all the decision making with regard to the State activities in Clinton and offered access to random testing at reduced cost to all residents

The EPA was invited to extend their radon remediation research program begun in Boyertown, Pennsylvania into New Jersey EPA remediated ten of the highest radon level homes at no cost to the occupants and provided detailed specifications for the remediation of twenty more homes

The successful remedial techniques developed in Clinton have been adapted to hundreds of other homes in northern New Jersey

Due to the experience of finding a clustering of high radon level homes in Clinton, the DEP and Department of Health

TABLE 2 Initial results statewide scientific study of radon, home radon testing results by county

County

Average Radon concentration (pCi/1)

Median radon concentration (pCi/1) Number ofsamples (pCi/1)Range

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TABLE 3 Summary of initial results for radon testing in non-residential buildings

Province buildingType of of buildingsNumber

Average radon concentration (PCI/L) (PCI/L)Range

* Becomes 2.4 if the single 192 pCi/1 value is excluded

** Becomes 2.3 if the single 192 pCi/1 value is excluded

developed a program of responding to reports of high radon

level homes (i.e., homes which are confirmed to have radon

concentrations at or above 200 pCi/1) A report of such a

home triggers the Radon Cluster Identification Protocol under

which the local governing body is advised of the confirmation

of such a home in their community and their cooperation in

sponsoring a public information meeting solicited Following

the public meeting, DEP staff test for radon in homes in the

area around the “discovery” home If this survey yields one or

more additional homes with radon concentrations at or above

200 pCi/1, the survey is repeated in the area around these

homes This process is repeated until all homes in the area

with radon levels at or above 200 pCi/1 have been identified

The specific concern with homes having this level of exposure

to radon is that the lung cancer risk associated with a lifetime

of such exposure at 75% occupancy is estimated by EPA to be

in the range of 44 to 77 in 100 EPA has recommended that

individuals finding such levels in their homes remediate them

within several weeks or temporarily relocate until such

reme-diation can be accomplished. 16

Radon Remediation Research

In addition to supporting EPA’s remediation research in

Clinton, DEP is also cooperating with the EPA on its House

Evaluation Program under which fifteen New Jersey homes,

predominantly in the Piedmont region, are undergoing

in-depth evaluation of their radon problems at no charge to the homeowner This program is expected to yield important information on how specific house characteristics and weather patterns influence the radon levels in homes Additionally, the DEP has contributed $185,000 in funding to a radon reme-diation research program being undertaken cooperatively by EPA, DEP, Lawrence Berkeley Laboratory of the University of California, Oak Ridge Associated Universities and Princeton University The primary aim of this research is to fine tune existing remediation methods so as to make them easier to implement and more cost effective

Radon Database Development

Radon testing firms participating in the voluntary certifica-tion program submit radon testing data they have collected summarized by municipality name and zip code This data is entered into a computerized database by DEP and used as an aid to decision making

Radon in Non-Residential Structures

The DEP issued interim guidance for the testing of non-residential structures such as schools, hospitals, government buildings and businesses in 1986 The Department of Health issued health related guidance for such structures in November

of 1987

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Radon Registry

In order to maintain an open channel of communication

with individuals who have already been exposed to elevated

levels of radon, the Department of Health developed a

Radon Registry for New Jersey residents Participants in the

survey are advised of the most current information regarding

radon and lung cancer via a newsletter Over 200 New Jersey

residents are participating in the registry

Low Interest Loans

In comparison to the equity value of most New Jersey homes,

the cost of remediating a significant radon problem (i.e., initial

test results in excess of 20 pCi/1) is relatively small, currently

averaging about $1,200 There are, however, some New Jersey

resident would find a single expenditure of this amount quite

burdensome In response to this potential problem, the New

Jersey Housing and Mortgage Finance Agency developed a

low interest loan program for affected residents There are no

income requirements associated with the program and the rate

is at or below the best available loan rates, currently 7.875%

For residents with severe radon problems (e.g., radon levels at

or above 200 pCi/1) an expedited loan application processing

procedure is available within three working days

Additional Research

External to the funding provided in the radon legislation, the DEP’s office of Science and Research and the New Jersey Geological Survey are conducting research to deter-mine radon in water levels in selected northern New Jersey aquifers

ASSESSMENT

The various state radon efforts provide a significant body

of data from which an assessment of New Jersey’s radon problem can be drawn

Preliminary radon concentration data from homes tested as part of the statewide study are listed by country in Table 2 The same data is organized by physiographic province in Figure 1 These data are almost exclusively for single family homes

Data on the testing on non-residential structures obtained

as part of the statewide study is summarized in Table 3 All the radon test data presented here were obtained using charcoal canisters 17 exposed for a period of four days under the EPA recommended protocols. 18 All testing was conducted during the period from November 15, 1986 through March 15, 1987 when closed house conditions

RADON CONCENTRATION (PCI/L)

<.5 1–.5–

.9 15.9 31.9 63.9 127.9 2561.9 3.9 7.9

2– 4– 8– 16– 32– 64– 128– >256

7.4

17.2 21.9 21

13.9 13.1

3.5 1.3 0.4 0.2 0.1 0

10 20 30 40

50

FREQUENCY %

TOTAL MEASUREMENTS = 13, 287

FIGURE 2 Commercial firm radon test data distribution, basement measurements.

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RADON CONCENTRATION (PCI/L)

<.5 5– 1–

.9 1.9 3.9 7.9 15.9 31.9 63.9 127.9 256

2– 4– 8– 16– 32– 64– 128– >256

16.33

32.91 23.93

14.65

6.92 3.49 1.00 0.02 0.21 0.02 0.02 0

10 20 30 40

50

FREQUENCY %

TOTAL MEASUREMENTS = 6, 101

FIGURE 3 Commercial firm radon test distribution, ground level measurements.

RADON CONCENTRATION (PCI/L)

<4 4– 8–

7 15 31 63 127 255 511 1023

16– 32– 64– 128– 256– 512– >1024

13.6

26.4 27.3

17.8 9.1 3.7 1.5 0.4 0.1 0.1 0

10 20 30 40

50

FREQUENCY %

TOTAL HOMES = 4, 107

FIGURE 4 Confirmatory monitoring data distribution.

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generally prevail in New Jersey homes In accordance with

the EPA protocols, the canisters were placed in the level of

the home closed to the underlying soil Unless individuals

live at the same level as the tests were made, this testing

method tends to overestimate the average concentrations

actually breathed by residents by a factor of about two

Most participants in the study lived one floor in the home above the testing level An exception to the two fold reduc-tion in radon concentrareduc-tion with a one floor increase in dis-tance from the underlying soil occurs in homes with forced air heat Openings in duct work in the basement make pos-sible the circulation of basement air throughout the home

RADON LEVELS IN WATER

(PCI/L)

0 10 20 30 40

50

FREQUENCY %

TOTAL WELLS = 872

1,000

1,000-5,000

5,000-10,000

10,000-50,000

50,000-100,000

>100,000

0.3 1.6

11.5 9.2

47.6

27.0

2.9

FIGURE 5 Radon in domestic well water obtained in the confirmatory monitoring program.

TABLE 4 Radon cluster identification program data distribution Location ⬍4 pCi/1 4–19pCi/1 20–199 pCi/1 200 pCi/1 N

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BERGEN PASSAIC

MORRIS

UNION ESSEX

MONMOUTH

SALEM GLOUCESTER

CAMDEN BURLINGTON

Tier 1-Test as soon as practical Tier 2- Test within one year Tier 3 - Test if concerned

New Jersey Department of Environmental Protection Testing Recommendation

WARREN

HUNTERDON

MIDDLESEX

MERCER

ATLANTIC

CAPE MAY CUMBERLAND

SUSSEX

SOMERSET

OCEAN

HUDSON

FIGURE 6 New Jersey Department for Environmental Protection, preliminary

recommenda-tions for radon testing.

Under these conditions, radon levels on upper floors have

been observed to equal or, in a few cases, even surpass

basement level radon concentrations

It should be noted that the statewide study was designed

to locate areas of potential radon problems and hence the

area sampling density was varied depending on anticipated results Approximately 20% of the total number of samples were set aside for use later in the sampling period to better define potential problem areas identified in the initial sam-pling Hence, the sampling is somewhat biased in terms of

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