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• Sodium carbonate activator solution For a class of 30 students you will need approximately 8 liters ofsodium carbon -ate activator solution.. Fill the plastic bucket with 8 liters of s

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FLINN SCIENTIFIC INC.

P.O BOX 219 • BATAVIA, ILLINOIS 60510 • 800/452-1261

o

Penney Sconzo

Westminster School

Atlanta, Georgia

The art of dyeing pro ably originated in

IndiaorChina no later than2 50 0BC.Most

natural dyes camefrom parts ofplants such

as the bark, berries, flowers, le ves, and

roots Because these dyes did not have a

strong atraction for thefibersbein dyed, a

process known asm o rd anti nq was used to

improve colorfastness Toreactwih acidic

dyes, fibers were treated with basic or

metallic mordants which might include

solutions of aluminum, copper, iron, or

chromium salts Compounds formed by the

dye and the mordant, called la kes ,

pre-vented the colors from washing out and

madethecolor longer lasting Such natural

dyes became less and less important as

syn-thetic dyes that produced brig ter colors

were developed Today,Iogwood black is the

only natural dye widely used

In 1856 ,William Henry Perkin began the

synthetic organic chemical industry by

accidentally discovering the purple d e,

mauveine, when hetried toproduce quinine

fromaniline.Thesyntheticdyes were known

as coal tar dyes because the six-membered

ring structures ofcarbon atomswere alld

e-rivedfrom coal tar Co goRedwas the first

dyediscovered with so gre t an affinity for

cellulose that a mordant was not requied

About 100years after Perkin's firstdiscov

-ery, fiber eactive dyes capable of formin

covalent linkages with the fiber were d

is-covered Afiber-reactive dye iswashfast

During dyeing, d e molecules must diffuse

from the aqueous solutio and into the

fibers Fibers such as cotton absorb water

readily and are said to be hydrophilic, while

fibers such as polyester absorb water with

difficulty and are described as hydrophobic

Dyeability is influenced if a fiber can some

-how carry an ionic charge and better inte

r-act with oppositely charged colored ions.To

o

d e cellulose, a reactive dyemust combine

with the h droxylgroups in the fiber Tie dyeing is one of the oldest metho s of

printing desig s on fabrics.Typically,parts

of the fabric are bunched together in a

desig and knotted or tied together with

sting Tied sections are protected fom absorbin the d e and patterns are created

Related Che mi cal Concepts: Dyes, chrornophores, affinity (hydro ho

-bic/h drophilic) covalent bonding vs

adsorbtio , electrolyte concentration, equ

i-librium, kinetics, reactio rates (temp

era-ture effects,concentraton effects),pH Materials Needed and Preparation

Instructions

• T-shirts, 100 %cotton, PFD (prepared for

d eing)

If you buyT-shirts that are not prepared

for dyeing, they must be pre-washed in hot water wih 2tablespoons of a mild

detergent likeJoy®, Dawn", Ivory", etc

Donot use adetergent with phosphates

or chlorines Dry shirts on the h t cycle

to remove spinning lubricants or other

surface additives

• Sodium carbonate activator solution

For a class of 30 students you will need

approximately 8 liters ofsodium carbon

-ate activator solution To prepare this

solution, mix 250 grams ofsodium c

ar-b nate anhydrous into 8lite of distilled

water and sti

• Ureasolutio

For a clas ' of30 students youwillneed approximately 8 liters of Urea solutio

To prepare this solutio , mix65 0grams

of urea into 8 liters of water and stir

This solution can be stored if it is not

mixed with the reactive d e Urea increases the solubility of the heavy

shades of reactive dyes

• ReactveDyes

Place a small amount of cold water in a

beaker and add 4 to 6 teaspoons (12-18

grams) of the reactive dye you have

selected Mixuntil lumps are removed

and all dye is moistened Add urea

solu-tion (asdescribed above) to make a total

ofone liter of dye solutio The amount of reactivedye is not specific

asitdepends on howstron y u want the

colors to be.Colors like yellow will need

more dye Remember some of the dye

willwash outwhen theT-shirt is washed

in hot water, so make the color darker than you want as an end product

Each student will require about one cup

of dye solution For a class of 30 stu

-dents, prepare a total of 2 liters <5freac-

tve dyesolution for each color you want

to use

Reactive dyes should be stored at room

temperature

I kept dry, reactivedyes havea shelf life

oftwo ye rs

• Plastic bucket

• Plastic dropcloth

(Con t nu e d on pag e 2 )

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VoL93-4 CHEMISTRY EDITION

TieDyeing-Continued

• Rubber bands! size 33 (3 1I2"L x 1/8"W)

.Jumbo, Beral-type pipets, 15 ml bulb

capacity

• Beakers, 1000 ml

• Oven racks or sturdy plastic coat hangers

interlocked between slats of wood

• Rubber gloves

• Newspaper

Procedure:

1 Fill the plastic bucket with 8 liters of

sodium carbonate activator solution

Soak the T-shirts in the sodium

carbon-ate activator solution for a minimum of

20 minutes The ionization of cellulose

increases with increasing alkalinity of

the solution and above pH 8 there is an

adequate number of ionized hydroxyl

groups in the fiber for most dyeing

pur-poses Soaking the T-shirts for 2 hours

will maximize the number of possible

bonding sites After the T-shirt has

soaked, wring the T-shirt out over the

plastic bucket

The sodium carbonate activator solution

is very basic so be sure to wear rubber

gloves when placing shirts in the

solu-tion and when the shirt is wrung out at

the end of the activation period

2 Shirts are now ready to fold and tie A

spiral pattern is created by laying the

shirt flat on a surface protected by a

clean dropcloth The shirt is held with

the thumb and fingers at the point where

the center of the spiral will be located

Use a twisting motion to coil the shirt

and use your other hand to bring the

loose ends of the shirt into the circle (see

Figure 1) Take four rubber bands and

slide them around the shirt so they

inter-sect at the center where the twist began

(see Figure 2) You now have what

appears to look like a "pie" cut into eight

pieces The bound shirt can be turned

over and dyed on both sides.We selected

this type of folding pattern because it is

the easiest to do and the entire

tie-dye-ing process can be completed in a

50-minute lab period Students also like this

pattern the best

Figure 2 Hint This should be'done in an area sep-arate from the dyeing area to prevent shirts frompickingup dye by mistake

3 Dyeing can be done on oven racks placed over sinks or on racks with newspaper underneath to absorb'excess dye After a shirt is placed on a clean rack, dyes can

be applied using jumbo Beral-type pipets Apply the dye to one side of the shirt by slowly squirting the reactive dye solution onto each section of the shirt A beautiful design can be made by dyeing each section of the shirt a.different color Once you are done dyeing one side

of the shirt, turn the shirt over and repeat the dyeing process Shirts should drain for 15 minutes if possible

Students tend to use a lot of dye and there is a lot of dripping so be prepared

Hint: Fewer beakers of dye and more pipets work best Too many beakers take too long to clean up and reorganize between classes Shirts can pick up some dye by mistake, but students will be applying so much dye that it probably will not matter Clean work areas will minimize problems

4 Place shirts in a plastic Ziplock" bag or small trash bag and close to keep the shirt moist Drying will prevent the

reac-tive dyes from fully reacting Most colors will have completely reacted after 4

hours but less reactive colors such as green and turquoise will take as long as

24 hours Be patient Let the dyes react completely

5 At home, rinse the shirt inwarm water (75-900F) in order to remove the unre-acted dye and the sodium carbonate

acti-vator Change thewater and continue to rinse Repeat until the water remains clear and the shirt does not feel slippery

Set the washing machine on the HOT

water setting and wash as many as 10 shirts at one time in 2 tablespoons of the pre-wash, such as Joy®or Dawn " dish-soap Dryshirts on the hottest dryer set-ting The reactive dye is washfast soit is now safe to washwith other clothes using normal detergents The reactive center on the dyes is a dichloro-triazinyl group so

do not use bleaches on the shirt

6. Now be creative! Try other patterns for folding Dye labcoats,socks, tennis shoes,

etc This makes a great lab to do before the Christmas holidays Students can make personalized gifts that are afford-able Use this activity as a fund raiser for the science club at your school

Safety Precautions:

Students should wear old clothes and shoes Reactive dyes are "wash fast." Once the reactive dye makes contact with clothes

it will not wash out

Do not let the students get sloppy Students should not squirt each other with filled pipets of reactive dye solution

Students should wear appropriate protec-tive clothing, e.g., chemical splash goggles, disposable plastic gloves and chemical-resistant aprons

Hands may become stained from the reac-tive dye.It is not easily washed off and will take about two days for the dye to wear off your hands,

Sodium carbonate activator solution is very basic Be sure to wear rubber or plastic gloves when placing the T-shirts in solution and when the shirt is wrung out at the end

of the activation period

Disposal:

All of the chemical solutions and reactive dyes may be disposed of according to Flinn Suggested Disposal Method #26b Consult your current Flinn Chemical Catalog/ Reference Manual

Literature Cited:

American Association of Textile Chemists

and Colorists (MTCC) Dyeing Primer. A series of short papers on the Fundamentals

of Dyeing P.O Box 12215, Research Triangle Park, NC 27709

Vickerstaff, T "Theoretical Principles of Dyeing with Reactive Dyes." Procion

Dyestuffin Textile Dyeing, 1962, pp 17-40.

Special thanks to Gerald Blackstone, Eastchester High School, Eastchester, NY and Elenore Grow, Horizon High School, Brighton, CO for showing me how to tie-dye Ordering information for Flinn's Tie-Dyeing-Chemistry Fun Kit is listed on page 7 of this Flinn Fax Individual tie-dyeing supplies may be found below

45 grams

45 grams

45 grams

45 grams

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