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Pharmaceutical Substances Syntheses, Patents, Applications - Part 147 pps

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Trade Names: D: Conceplan Grunentha1- comb.. Micronovum Janssen- Cilag TriNovum Janssen-Ci1ag- comb.. GB: Micronor Janssen-Cilag Noriday Searle Primolut N Schering Utovlan Searle numero

Trang 1

Norethandrolone N 1461

Use: anabolic RN: 52-78-8 MF: C2,H3,02 MW: 302.46 EINECS: 200-153-5

norethisterone

(9 v.)

1 Norethandrolone

Reference(s):

US 2 721 871 (Searle; 1955; appl 1954)

alternative synthesis:

17s 2 691 028 (Searle; 1954; prior 1952)

Colton, EB et al.: J Am Chem Soc (JACSAT) 79, 1123 (1957)

Formulation(s): tabl 10 mg

Trade Name(s):

F: Nilevar (Laphal) GB: Nilevar (Searle); wfm USA: Nilevar (Coastal); wfm

Norethisterone

(Norethindrone)

ATC: G03ACO1; G03DC02 Use: progestogen

RN: 68-22-4 MF: C,H,O, MW: 298.43 EINECS: 200-681-6

LDso: 6 d k g (M, PO.)

CN: (17a)-17-hydroxy-19-norpregn-4-en-20-yn-3-one

1 Li, NH3

2 Crop CH3COOH

0 2 chromium(W) oxide O

3.1 7-dioxo- 1 %nor- 4-androstene (I)

orthoformic acid

triethyl ester

Trang 2

1462 N Norethisterone acetate

1 K tert-amylate

2 HCI

+ H C E C H -+

I

Reference(s):

US 2 774 122 (Syntex; 1956; MEX-prior 1951)

US 2 774 777 (Syntex; 1956; prior 1952)

Djcrassi, C et al.: J Am Chem Soc (JACSAT) 76,4092 (1954)

alternative syntheses:

US 2 849 462 (P dc Ruggieri; 1958; appl 1957)

Ringold, H.J et al.: J Am Chem Soc (JACSAT) 78,2477 (1956)

Ringold, H.J et a].: Ann N Y Acad Sci (ANYAA9) 71,500 (1958)

Ueberwasser, H et al.: Helv Chim Acta (fICACAV) 34,344 (19631

Ullmanns Encykl Tech Chem., 4 Aufl., Vol 13, 31

Onken, D.; Meublein, D.: Pharmazie (PHARAT) 25, 3 (1970)

total synthesis of 3,17-dioxo- 19-nor-4-androstene:

DE 1 958 600 (Hoffmann-La Roche; appl 21.1 1.1969; USA-prior 22.11.1968)

Formulation(s): tabl 0.35 mg, 0.5 mg (also in comb.)

Trade Name(s):

D: Conceplan (Grunentha1)-

comb

Micronovum (Janssen-

Cilag)

TriNovum (Janssen-Ci1ag)-

comb

numerous generics

F: Norluten (SmithKline

Beecham)

Ortho-Novum 1135

(Janssen-Ci1ag)-comb

Triella (Ci1ag)-comb

GB: Micronor (Janssen-Cilag)

Noriday (Searle) Primolut N (Schering) Utovlan (Searle) numerous combination preparations

I: Trinovum (Janssen-Ci1ag)- comb

J: Norluten D (Shionogi) Primosiston Tab (Nihon Schering)-comb

Sophia-A, C (Teikoku Zoki)-comb

USA: Brevicon (Sear1e)-comb

Micronor (Ortho-McNeil) Modxon (Ortho-McNei1)- comb

Nclova (Warner Chi1cott)- comb

Norinyl (Sear1e)-comb

Ortho-Novum (Ortho- McNci1)-comb

generic and combination preparations

Norethisterone acetate

(Norethindrone acetate)

ATC: G03D Use: progestogen RN: 51-98-9 MF: C22H2,03 MW: 340.46 EINECS: 200-132-0

CN: (17a)- 17-(acetyloxy)-19-norpregn-4-en-20-yn-3-one

Trang 3

Norethisterone enanthate N 1463

norethisterone acetic anhydride

(4 v.)

Norethisterone ocetote

19-norpregno-3,5-dien-20-yne- 3.1 78-diol diacetate (I)

Reference (s):

US 2 964 437 (Schering AG; 13.12.1960; appl 11.6.1957; D-prior 16.6.1956)

Djerassi, C et al.: J Am Chem Soc (JACSAT) 81,436 (1959)

DE 1 017 166 (Schering AG; appl 16.6.1956)

alternative synthesis:

DD 136 502 (VEB Jenapharm; appl 1 1.5.1978)

Formulation(s): f c tabl 1 mg; tabl 1 mg, 5 mg, 10 mg

Trade Name(s):

D: Gestakadin (Kade)

Neorlest 21 (Parke Davis)-

comb

Norethisteron (Jenapharm)

Primolut-Nor (Schering)

Primosiston (Schering)-

comb

Prosiston (Schering)-comb GB:

Sinovula (Axhe)-comb

Sovel (Novartis Pharma)-

comb

Trisequens (Novo Nordisk;

RhBne-Poulenc Rarer)-

comb

F: Kliogest (Specia)-comb

Milli-Anovlar (Schering)- comb

Milligynon (Schering) Miniphase (Schering)- comb

Primolut-Nor (Schering)- comb

Elleste Deret (Sear1e)- comb

Estra combi (Novartis)- comb

Evorel combi (Janssen- Ci1ag)-comb

Klimofem (Novo Nordisk)- comb

Loestrin (Parke Davis)- comb

S.H 420 (Schering Chemicals) Trisequens (Novo Nordisk)-comb

I: Primolut-Nor (Schering) J: Anovlar (Nihon Schering)- comb

Norluten A (Shionogi) USA: Aygestin (ESI Lederle) Estrostep (Parke Davis)- comb

Use: progestogen RN: 3836-23-5 MF: C,,H,,O, MW: 410.60 EINECS: 223-326-7

CN: (17a)-17-[(l -oxoheptyl)oxy]-19-norpregn-4-en-20-yn-3-one

Trang 4

1464 N Noretynodrel

C H

H , C ~ S O , H

or pyridine

,

0

0

norelhisterone enanthic anhydride

( q v.)

Norethisterone enontnate I

Reference(s):

DE 1 017 166 (Schering AG; appl 16.6.1956)

alt~rnative synthesis:

FR 1 349 991 (Parke Davis; appl 29.1 1.1962; GB-prior 1.12.1961)

use as progestogen depot preparation:

DOS 2 548 413 (Schering AG; appl 27.10.1975)

Formulation(s): amp 200 rng/ml

Trade Name($):

D: Noristerat (Schering) F: Noristerat (Schering) GB: Noristerat (Schering)

Noretynodrel

(Norethy nodrel)

ATC: G03D Use: progestogen RN: 68-23-5 MF: C2,H260, MW: 298.43 EINECS: 200-682-1

CN: (17a)-17-hydroxy-19-norpregn-5(10)-en-20-yn-3-one

-+

3-methoxy-17-am- 2.5(10)-estradiene (I)

CH Ill

KOC(CH,)ZC2H5 diethyl ether, toluene

Noretynadrel

L

Trang 5

Norfenefrine N 1465

Reference(s):

US 2 691 028 (Searle; 1954; prior 1953, 1952)

US 2 725 389 (Searle; 1955; prior 1953)

starting material:

US 2 655 51 8 (Searle; 1953; appl 1952)

alterna~ive synthesis:

FR 1 421 476 (Roussel-Uclaf; appl 2.1 1.1964)

Formulation(s): tabl 2.5 mg, 5 mg, 9.85 mg in comb with metranol

Trade Name(s):

D: Kontrazeptivum 63 I: Ebionel (Panther-Osfa USA: Enovid (Sear1e)-comb.;

Zyklustabletten IB 2 (Ce- Elan (Valeas)-comb.; wfm Enovid E (Sear1e)-comb.;

Use: sympathomimetic, circulatory analeptic, adrenergic RN: 536-21-0 MF: CHHl,N02 MW: 153.18 EINECS: 208-626-8

LD,,: 4.9 mglkg (M, i.v.); 263 mgkg (M, p.0.);

17.4 mgkg (R, i.v.); 390 mglkg (R, p.0.)

CN: a-(aminomethy1)-3-hydroxybenzenemethanol

hydrochIoride

RN: 4779-94-6 MF: C8HllN02.HC1 MW: 189.64 EINECS: 225-323-6

LD,,: 113 mglkg (M, i.v.); 3300 mglkg (M, p.0.);

17.4 mglkg (R, i.v.); 390 m g k g (R, p.0.)

O K 3 + .I% - 0g3

OH

3'-hydroxyaceto- benzoyl

0%

3'-benzoyloxy-

NH, resp

hexomethylenetetromine

2-bromo-3'-benzoyloxy- ocetophenone

2-omino-3'-hydroxy ocetophenone (Ill)

Trang 6

r

1466 N Norfloxacin

Norfenefrine

u

H2 Roney-Ni

I11 -+

I-C,H,, -0N0,

I

HO

&NH2 OH

Reference (s):

a FR 851 296 (R Sachs; 1938)

FR 866 569 (R Sachs; 1939)

b DE 2 130 7 10 (Godecke; appl 21.6.1971)

Formulation(s): amp 50 mg15 ml; cps 6 mg; drg 15 mg, 45 mg; drops 6 mglml; sol 6 mglml; s r tabl 50 mg;

tabl 45 mg (as hydrochloride)

Trade Nume(s):

ratiopharm (ratiopharm) combination preparations hydrochloride)

I: Euro-Cir (Virgiliano); wfm

Norfloxacin ATC: JOlMA06; SOlAX12

Use: antibiotic (gyrase inhibitor) RN: 70458-96-7 MF: C,,H,,FN30, MW: 319.34 EINECS: 274-614-4

LD,,,: 220 mglkg (M, i.v.); 4 glkg (M, p.0.);

245 mg/kg (R, i.v.); >4 g k g (R, p.0.)

CN: 1-ethyl-6-fluoro-1,4-dihydro-4-oxo-7-(I-piperazinyl)-3-quinolinecarboxylic acid

0

+ H 3 c v o ~ o , c H 3 + :xX&o-cH3

fluorooniline methylenemalonate

1 8 r - c ~ ~ , N ( c ~ H ~ ) ,

2 NoOH

0wCH3 1 ethyl bromide

Trang 7

Norgestimate N 1467

Referencefs):

DE 2 804 097 (Kyorin; appl 3 1.1.1978; J-prior 16.5.1977)

US 4 146 719 (Kyorin; 27.3.1979; J-prior 16.2.1977)

qnthesis of 1-ethyl-6-fluoro-7-chloro-1,4-dihydro-4-oxoquinoline-3-carboxylic acid:

Koga, H et al.: J Med Chem (JMCMAR) 23, 1358 (1980)

Norfloxocin

Fortnulation(s): eye drops 3 mglml; f c tabl 400 rng

chloro-1.4-dihydro-

4-oxoquinoline-3-

carboxylic acid (U)

Trade Nameis):

Chibroxin (Chibret) GB: Utinor (Merck Sharp & USA: Chibroxin (Merck)

& Dohmc-Chibret) I: Fulgram (ABC) Noroxin (Roberts)

Noroxin (MSD)

Use: progestogen, oral contraceptive RN: 35189-28-7 MF: C,,H,,NO, MW: 369.51

CN: (17a)- 17-(acetyloxy)-13-ethyl-l8,19-dinorpregn-4-en-20-yn-3-one oxime

:H3

""2- , - , ,-' " - -

hydroxylomine hydrochloride

levonorgestrel acetate

(cf levonorgestrel)

Reference(s):

GB 1 123 104 (Ortho; appl 2.9.1966; USA-prior 22.10.1965)

DE 1 620 102 (Ortho; appl 9.9.1966; USA-prior 22.10.1965)

medical use for suppression of fertility:

US 4 027 019 (Ortho; 3 1 S.1977; appl 23.1.1976; prior 24.7.1975)

Formulation(s): tabl 0.25 mg in comb with ethinylestradiole

Trade Name(s):

D: Cilest (Janssen-Ci1ag)- F: Cilest (Janssen-Ci1ag)- GB: Cilest (Janssen-Ci1ag)-

Pramino (Janssen-Cilag)- Effiprev (Eflik)-comb 1: Cilest (Cilag)-comb comb

Trang 8

1468 N Norgestrel

USA: Ortho-Cyclen (Ortho- Ortho-Tri-Cyclen (Ortho-

Use: progestogen RN: 6533-00-2 MF: C,,H,,O, MW: 3 12.45 EINECS: 229-433-5

LD,,: 5010 mglkg (M, p.0.);

5010 mglkg (R, p.0.)

CN: (17a)-(&)-I 3-ethyl- 17-hydroxy- 18,19-dinorpregn-4-en-20-yn-3-one

CH

(CH,),COK THF

& + HC-CH -

(C)-3-methoxy-18-methyl- acetylene

17-0x0-2.5(10)-estradiene

Reference ( s ) :

GB 1 041 279 (H Smith; appl 19.10.1961)

GB 1 041 280 (H Smith; appl 19.10.1961)

DOS 2 030 056 (Schering AG; appl 13.6.1970)

Buzby, G.C et al.: J Med Chem (JMCMAR) 9 , 7 8 2 (1966)

starting material:

Smith, H et al.: J Chem Soc (JCSOA9) 1964,4472

(+)-3-methoxy-18-methyl- 19-norpregna-2.5(10)- dien-20-yne-178-ol (I)

total synthesis:

NL-appl 6 414 702 (Roussel-Uclaf; appl 17.12.1964; F-prior 17.12.1963)

Smith, H et al.: Experientia (EXPEAM) 19,394 (1963)

Smith, H et al.: J Chem Soc (JCSOA9) 1963,5072

Blickenstaff, R.T.; Ghosh, A.C.; Wolf, G.C.: Total Synthesis of Steroids (Organic Chemistry Vol 30) p 270, Academic Press, New York, London 1974

Formulation(s): drg 0.5 mg in comb with ethinylestradiole

Trade Name(s):

Stediril (Wyeth)-comb Stediril (Wyeth-Leder1e)- Eugynon (Schering)-comb

comb

Trang 9

Norgestrienone N 1469 I: Eugynon (%hering)-comb USA: LoIOvral (Wyeth-Ayerst)- Ovral (Wyeth-Ayerst)-

Ovrette (Wyeth-Ayerst)

Use: progestogen RN: 848-21-5 MF: C2,Hz2O2 MW: 294.39 EINECS: 212-698-6

CN: (17a)-17-hydroxy-l9-norpregna-4,9,11-trien-20-yn-3-one

1 NH,OH NaOCOCH,

& 2 0 0 Al[OCH(CH&l, b

1 hydroxylamine

17p-hydroxy-3-0x0- isopropylate

4.9,1 1 -estratriene

4.9.1 1 -eslrotrien-3.17-diane 3-axime (I)

ethynylmognesium

bromide

178-hydroxy-19-norpregna- 4,9,1 1 -trien-20-yn-3-one oxirne (11)

1 Norgestrienone

I

Reference(s):

US 3 257 278 (Roussel-Uclaf; 21.6.1966; F-prior 5.7.1963,4.10.1963, 15.5.1964, 14.8.1964, 1.6.1965) FR-M 3 060 (Roussel-Uclaf; appl 4.10.1963)

NL 6 401 555 (Roussel-Uclaf; appl 20.2.1964; F-prior 20.2.1963,5.7.1963,4.10.1963)

NominC, G et a].: C R Hebd Seances Acad Sci (COREAF) 260,4545 (1965)

starting material:

BE 631 298 (Roussel-Uclaf; appl 19.4.1963; F-prior 20.4.1 962)

NL 6 414 702 (Roussel-Uclaf; appl 17.12.1964; F-prior 17.12.1963, 14.1.1964, 20.2.1964)

NL6 517 141 (Roussel-Uclaf; appl 30.12.1965; F-prior 31.12.1964,26.2.1965,24.3.1965, 14.6.1965,3.9.1965, 17.9.1965)

Velluz, L et al.: C R Hebd Seances Acad Sci (COREAF) 257,569 (1963)

total synthesis:

Ullmanns Encykl Tech Chem., 4 Aufl., Vol 13, 34

Velluz, L et al.: C R Hebd Seances Acad Sci (COREAF) 257,3086 (1963)

Formulation(s): tabl 0.35 mg

Trang 10

1470 N Normethadone

Trade Nume(s):

Use: antitussive, analgesic RN: 467-85-6 MF: C2,H2,NO MW: 295.43 EINECS: 207-401-1

LD,,: 31 m g k g (M, i.v.)

CN: 6-(dimethylamino)-4,4-diphenyl-3-hexanone

hydrochloride

RN: 847-84-7 MF: C2,,Hz5NO HCI

LD,,: 45 m g k g (M, i.v.)

2-(dimethylomino)ethyl diphenyl-

ethy lmogneslum

bromide

Reference(s):

DE 865 314 (Hoechst; appl 1941)

MW: 33 1.89 EINECS: 212-694-4

NONH2

sodium ornide

nitrile (1)

Normethadone

DE 870 700 (Hoechst; ap& 1942)

Bockmiihl, M.; Ehrhart, G.: Justus Liebigs Ann Chem (JLACBF) 561, 52 (1948)

Formulation(s): drops 10 mg/ml

Trade Name(s):

D: Ticarda (Hoechst); wfm

Normolaxol

RN: 18831-34-0 MF: C,,H,,NO, MW: 327.38

CN: 4,4'-(2-quinolinylmethylene)bis[phenol]

ATC: A06A Use: laxative

hydrochIoride

RN: 19035-45-1 MF: C22H,7N02 HCl MW: 363.84

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