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Pharmaceutical Substances Syntheses, Patents, Applications - Part 90 pps

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0.01 % Trade Names: D: Flucinar medphano Jellin Griinenthal Jellisoft Griinenthal Procto-Jellin Griinentha1- comb... with neomycin GB: Metosyn Zeneca USA: Dermacin Pedinol F: Topsync C

Trang 1

Fluocinolone acetonide F 891

H3C-CO-NH-Br HCIO,

b

N-bromoacetamide

1

0 CH,

0

Se02, (H3C)3C-OH

selenium fluoride

i

fluocinolone (IV)

-

- Fiuacinolone acetonide

US 3 014 938 (Syntex; 26.12.1961, appl 23.8.1960; MEX-prior 7.9.1959)

US 3 124 571 (Syntex; 10.3.1964; appl 19.5.1960; MEX-prior 26.1.1960)

Djerassi, C et al.: 3 Am Chem Soc (JACSAT) 82, 3399 (1960)

starting material:

Julian, P.L et al.: J Am Chem Soc (JACSAT) 72, 5145 (1950)

alternative syntheses:

GB 933 867 (American Cyanamid; appl 5.12.1959; USA-prior 8.12.1958)

US 3 197 469 (Pharmaceutical Research Prod.; 27.7.1965; appl 6.8.1958)

Formulation(s): cream 0.025 9%; ointment 0.025 %: topical sol 0.01 %

Trade Name(s):

D: Flucinar (medphano)

Jellin (Griinenthal)

Jellisoft (Griinenthal) Procto-Jellin (Griinentha1)-

comb

Trang 2

892 F Fluocinonide

F: Antibio-Synalar

(Cassennc)-comb

Synalar (Cassenne)

Synalar Neomycin

(Cassenne)-comb

GB: Synalar (Zeneca)

I: Alfabios (Biotekfarma)

Alfafluorone (Biotekfarma)

Boniderma (Boniscontro &

Gazzonc)

Coramide (Ottolenghi)

Cortanest Plus (Piam)-

comb with lidocaine

Dermobeta (Terapeutico

M.R.)

Dermolin (Lafare)

Doricum (Farmila)-comb

with neomycinc

Doricum Semplice (Farmila)

Esacinone (Lisapharma) Fluocit (CT)

Fluomicetina (Zoja)-comb

with kanamycin Fluomix Same (Savoma) Fluovitef (Italfarmaco) Lauromicina Pomata (Lafare)-comb with eritromycin Localyn (Recordati) Mccloderm (Schwa@- comb with meclocycline Meclutin (ABC-Torino)- comb with meclocycline Nefluan (Mo1teni)-comb

Neoderm (Crosara)

Omniderm (Face) Proctolin (Recordati)- comb with lctocaine Sterolone (Francia Farm.) Ultraderm (Ecobi) J: Benamizol (Mohan Yakuhin) Biscosal (Ohta Seiyaku) Cortiphate (Tokyo Tanabe) Flucort (Syntex-Tanabe) Fluvean (Kowa) Fluzon (Taisho Seiyaku) USA: Derma-Smoothe (Hill) Fluonid (Allergan)

FS Shampoo (Hill) Synalar (Medicis) Synemol (Medicis)

Use: glucocorticoid, anti-inflammatory RN: 356-1 2-7 MF: C,,H,,F,O, MW: 494.53 EINECS: 206-597-6

LD,,: >6 glkg (M, p.0.);

14 m g k g (R, p.0.)

CN: (6a,11~,16a)-21-(acetyloxy)-6,9-difluoro-l 1-hydroxy-16,17-[(l-~ethylethylidene)bis(oxy)]pregna-l,4-

diene-3.20-dione

Reference(s1:

GB 916 996 (Olin Mathieson; appl 21.7.1959; USA-prior 6.8.1958)

US 3 124 571 (Syntex; 10.3.1964; appl 19.5.1960; MEX-prior 26.1.1960)

fluocinolone ocetonide

Forrnulation(s): cream 0.5 mglg; ointment 0.5 mglg, sol 0.5 mg/g

Trade Narne(s):

D: Topsym (Grunenthal) Topsyne nkomycine J: Bestasone (Kodama)

comb with neomycin GB: Metosyn (Zeneca) USA: Dermacin (Pedinol)

F: Topsync (Cassenne) I: Flu 21 (Select Pharma) Lidex (Medicis)

Topsyn (Recordati) Lidex E Cream (Medicis)

Fluocinonide

1

Trang 3

Fluocortin butyl F 893

Fluocortin butyl

(Fluocortin butyl ester)

ATC: D07AB04 Use: glucocorticoid RN: 41767-29-7 MF: C2,H3,F05 MW: 446.56 EINECS: 255-543-8

LD,: >5 g/kg (M, p.o.1;

>4 g/kg (R, p.0.);

>I &/kg (dog, p.0.)

CN: (6a,11 P, 16a)-6-fluoro- 1 1 -hydroxy-16-methyl-3,20-dioxopregna-l,4-dien-21 -oic acid butyl ester

fluocortin

RN: 33124-50-4 MF: C22H27FOs MW: 390.45 EINECS: 251-383-8

F

fluocortolone

(9 v.)

MnOZ CW2CIZ

manganese

dioxide

Fluocortin butyl

DOS 2 150 268 (Schering AG; appl 4.10.1971)

DOS 2 204 361 (Schering AG; appl 27.1.1972)

DOS 2 260 303 (Schering AG; appl 6.12.1972)

GB 1 387 91 1 (Schering AG; valid from 19.3.1975; D-prior 4.10.1971,27.1.1972)

Laurent, H et al.: Arzneim.-Forsch (ARZNAD) 27 (II), 2187 (1977) (also other methods)

DOS 2 441 284 (Schering AG; appl 27.8.1974)

BE 823 682 (Schering AG; appl 20.12.1974; D-prior 21.12.1973, 27.8.1974, 16.9.1974)

Formulation(s): cream 7.5 mglg; ointment 7.5 mglg; powder 100 mgl4 g

Trade Narnefs):

D: Bi Vaspit (Asche)-comb Lenen (Alk-Scherax; Vaspit (Asche)

H02AB03; S01CA04 Use: glucocorticoid RN: 152-97-6 MF: CZ2H2,FO4 MW: 376.47 EINECS: 205-811-5

CN: (6a,11~,16a)-6-fl~oro-11,21-dihydroxy-l6-methylpregna-l,4-diene-3,20-dione

Trang 4

894 F Fluocortolone

1 BrZ

2 Nal

3 KOwCH3

b I N-bromo-

succinimide

16a rnethylpregnenolone 21 -0cetoxy-3p-hydraxy-16-a-

3@-ocetote methyl-20-axo-5-pregnene fluoride

(cf flumetasone synthesis)

OH microbiological dehydrogenation

Fluocortolone

Referetrce(s):

DE 1 135 899 (Schering AG; appl 20.5.1960)

BE 614 196 (Schering AG; appl 21.2.1962; D-prior 22.2.1961)

Domenico, A et al.: Arzneh-Forsch (ARZNAD) 15,46 (1965)

Dl3 1 169 444 (Schering AG; appl 22.2.1961)

synthesis of starting cotnpound:

Petrov, V.; Williamson, D.M.: J Chem Soc (JCSOA9) 1959, 3595

alternative synthesis:

Kieslich, K ct a].: Justus Liebigs Ann Chem (JLACBF) 726, 168 (1969)

DOS 1 909 152 (Schering AG; appl 19.2.1969)

review:

Akhrem, A.A et al.: Russ Chem Rev (Engl Trans].) (RCRVAB) 34,926 (1965)

Formulation(s): cream 2.5 mglg; lotion 2.5 mglg; ointment 2.5 mglg; tabl 5 mg, 20 mg, 50 mg

Trade Name(s):

D: Ultralan (Schering) Ultralanum (Schering) Ultralanum oint

CB: Ullradil (Schering); wfm

Trang 5

Fluocortolone caproate F 895 Ultraproct (Schering)- I: Ultralan (Schering)-comb Ultraproct (Schering)-

-F ~ u o c o ~ ~ o ~ o ~ ~ caproate ATC: C05AA08; D07AC05; H02AR03

Use: glucocorticoid RN: 303-40-2 MF: C2,H,,FOs MW: 474.61 EINECS: 206-140-0

CN: ( 6 a , l l P, 16a)-6-fluoro-1 l-hydroxy-l6-methyl-21-[(1-oxohexyl)oxy]pregna-1,4-diene-3,20-dione

fluocortolone c a p r o i c a n h y d r i d e Fluocortolone c o p r o a t e

Referencefs):

FR 1 561 884 (Schering AG; appl 10.5.1968; D-prior 13.5.1967)

Forrnulation(s): cream; lotion; ointment 2.5 mglg in comb with fluocortolone

Trade Narnefs):

D: Ultralan Creme (Schering)-

comb

Ultralan Salbe (Schering)-

Ultraproct (Schering)-

comb

F: Myco-Ultralan (Schering)-

comb

Ultralan (Schering)-comb Ultralanum (Schering Ultraproct (Schering)- Chemicals)-comb.; wfm

Ficoid (F1sons)-comb.; Chemicals)-comb.; wfm

Ultradil (Schering Ultraproct (Schering) Chemicals)-comb.; wfm comb

Fluocortolone trimethylacetate

(Fluocortolone 2 1 -pivalate)

ATC: C05AA08; D07AC05; H02AB03 Use: glucocorticoid

RN: 20380-10-3 MF: C2,H3,FO5 MW: 460.59

CN: 6a-fluoro-17,21-dihydroxy-l6a-methyl-pregna-l,4-diene-3,20-dione 21-pivalate

tl~ocortol~ne pivolic anhydride

F

Fluocortolone trimethylacetote

Referencefs):

FR 1561 884 (Schering AG; appl 10.5.1968; D-prior 13.5.1967)

Trang 6

896 F Fluorescein

Formulatio~z(s): cream 20 mg/g; cream 2.5 mglg in comb with fluocortolone; emulsion 2.5 mglg in comb with

fluocortolone/-caproate; suppos 40 mg in comb with lidocain hydrochloride

Trade Name(s):

D: Doloproct (Schering)- Ultraproct (Schering)- Ultraproct (Schering

hydrochloride F: Ultraproct (Schering)- I: Ultralan (Schering)-comb Ultralan Creme (Schering)-

'jmb

Ultraproct (Schering)-

comb

Use: diagnostic RN: 2321-07-5 MF: CZoHj2O5 MW: 332.31 EINECS: 219-03 1-8

LD,,,: 300 mg/kg (M, i.v.)

CN: 3',6'-dihydroxyspiro[isobenzofuran-1(3H),9'-[9H]xanthen]-3-one

disodium salt

RN: 518-47-8 MF: C20H,oNa20S MW: 376.28 EINECS: 208-253-0

' LD,,,: 1 glkg (M, i.v.); 4738 mglkg (M, p.0.);

1 glkg (R, i.v.); 6721 mglkg (R, p.0.);

1 glkg (dog, i.v.)

phthalic resorcinol

anhydride

Fluorescein

Reference (s):

Ullmanns Encykl Tech Chem., 4 Aufl., Vol 23,414

Formulation(s): amp 113.2 mglml (as disodium salt); eye drops 1.7 mg/ml

Trade Name(s):

D: Fluorescein-Losung 1 0 % Thilorbin (Alcon) I: Pancreolauryl Test intravenos 1nj.-Losung GB: Minims Fluorescein (Geymonat; as laurate)

Fluoreszein 0,15 % Thilo Minims lignocaine and Fluores (Showa Yakuhin) Augentropfen (Thilo) fluorescein (Chauvin)- Fluorescein sodium

DlOAAOl; SOlBA07; SOlCBO5 Use: glucocorticoid

RN: 426-13-1 MF: Cz2H2,F0, MW: 376.47 EINECS: 207-041 -5

LD,,,: 443 mglkg (R, i.p.)

CN: ( 6 a , 1 1 P)-9-fluoro- 1 1,17-dihydroxy-6-methylpregna-1,4-diene-3,20-dione

Trang 7

Fluorometholone F 897

Ob ,CH3 pyridine

9-fluoro-6a-methyl- methane- (1)

hydrocortisone sulfonyl

chloride

Zn, CH3COOH

I

rnicrobiologicol dehydration

[Ssptomym offinis (ATCC 6737)]

I1

CH3

Fluorometholone

Referencets):

US 2 867 638 (Upjohn; 6.1.1959; appl 17.5.1967; prior 10.9.1956)

DE 1056 605 (Upjohn; appl 6.5.1959; USA-prior 10.9.1956)

starting material:

Spero, G.B el al.: J Am Chem Soc (JACSAT) 79, 1515 (1957)

Formulation(s): eye drops 1 mglml

Trade Namets):

D: Efflumidex (Pharm-

Efflumycin (Pharm- I:

Allergan)-comb

Ehrtolan (Albert-Rousse1)-

comb

Ejemolin (CIBA Vision)- J:

comb

Fluoropos (Ursapharm)

Isoptotlucon (Alcon) Ursnon (Nihon Yakuhin Flucon collyre (Alcon) K o g ~ o )

Efemoline (CIBA Vision) USA: FML Liquifilm (Allergan);

Fluaton (Allergan) Neo-Oxylone (Upjohn) Flumetol (Farmila)-comb comb.; wfm

Flu-Base (Kowa) Oxylone (Upjohn); wfm Flumetholon (Santen)

Okilon (Sumitorno)

Trang 8

898 F Fluorouracil

Pluorouracil

(Fluracilum)

ATC: LOlBC02 Use: antineoplastic RN: 51-21-8 MF: C4H,FN202 MW: 130.08 EINECS: 200-085-6

LD,,,: 81 m g k g (M, i.v.); 115 mglkg (M, p.0.); !

245 mglkg (R, i.v.); 230 m g k g (R, p.0.);

30 mglkg (dog, p.0.)

CN: 5-fluoro-2,4-pyrimidinediol or 5-fluoro-2,4(1H,3H)-pyrimidinedione

ethylate H 0

ethyl fluoroocetote ethyl formate (1)

S-methylthiouronium

sulfote

5-fluoro- fluorourocil 2-methyl-

thiouracil

F2 or CF30F

b

fluorine

H

trifluoromethyl

urocil

hypofluorite

Refewnce(s):

a US 2 802 005 (C Heidelberger, R Duschinsky; 6.8.1957; prior 26.9.1956)

Duschinsky, R et al.: J Am Chem Soc (JACSAT) 79,4559 (1957)

b US 3 682 917 (I L Knuniants et al.; 8.8.1972; appl 25.3.1970)

US 3 846 429 (S A Giller et al.; 5.1 1.1974; appl 22.9.1971)

US 3 954758 (PCR, Inc.; 4.5.1976; prior 7.8.1967, 1.3.1968,27.5.1970,4.10.1971)

DOS 2 149 504 (Research Inst f Med and Chem.; appl 4.10.1971; USA-prior 5.10.1970)

DOS 2 719 245 (Daikin Kogyo; appl 29.4.1977; J-prior 29.4.1976)

DOS 2 726 258 (Daikin Kogyo; appl 10.6.1977; J-prior 11.6.1976)

synthesisfiom orotic acid by fluorination and following decarboxylation:

DOS 2 826 496 (Asahi Glass; appl 16.6.1978; J-prior 17.6.1977)

Formulation(s): cream 5 %; ointment 50 mglml, 1 g/20 g; plaster 96 ~ g l l l 3 cm2; vial 50 mglml, 250 mg15 ml,

500 mg/lO ml, 1000 mg120 ml

Trade Name(s):

D: Actino-Hermal Pflaster Verrumal (Herma1)-comb GB: Accusite (Matrix)

Efudix Roche (ICN) combination preparations Fluoro-Urac~le (Roche) Fluroblastin (Pharmacia & F: Efudix (Roche) generic

Trang 9

Fluoxetine F 899

Carzonal (Tobishi) Timadin (Torii) USA: Efudex (Roche)

Efudix (Roche) Ulosagen (Kyowa Yakuhin Fluoroplex (Allergan)

inhibitor

f

RN: 54910-89-3 MF: C,,HlnF3NO MW: 309.33

LD,: 464 mgkg (M, p.o.1;

825 mgkg (R, p.0.)

CN: (~)-N-methyl-y-[4-(trifluoromethyl)phenoxy]benzenepropanamine

monohydrochloride

RN: 59333-67-4 MF: C17HlnF3N0 HC1 MW: 345.79

acelophenone paraform- dimethyl- 3-dimethylamino-

aldehyde amine propiophenone (1)

1 B,H,

2 S0Cl2

F 3 c ~ 0 H , NaOH

I 11

CH3 4-trifluoromethyl-

1.BrCN

2 KOH

NNCH3 1 cyanagen bromide

(*)-N,N-dirnethyl-3-phenyl-3-

(4-trifluoromethylphenoxy)-

pmpylamine (11)

NaOH, DMF

Fluoxetine

(*)-I -phenyl-3-(methyl- 1 -chloro-4-(tri-

omino)propan- 1-01 (111) fluoromethyl)-

Trang 10

900 F Fluoxetine

bentyl 4-(tri- fluoromethyl)- phenyl ether

1 o3

2 H2N-CH,

3 NaCNBH3

_*

3 sodium cyano-

Fluoxetine

borohydride

N-methyl-

hydroxyl-

omine

N-methyl- nitrone

2-methyl-5-

phenylisoxo- zolidine (VI)

H Pd-C N

VI 2 111 - ( Fluoxetine (

2 NaH, OMS0

cyanomethyl

phenyl ketone

(?)'-3-phenyl-3- hydroxy-l- proponarnine

0 LIAIH,, THF

+ C I , k O P ' 3

diborone

I - - - +

methyl chloroformoie

Fluoxetine

El

1 CIC02C2H5

2 NaOH

1 ethyl

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