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Pharmaceutical Substances Syntheses, Patents, Applications - Part 50 doc

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formulation with penicillins and cephalosporins: DOS 2 559 41 1 Beecham; appl.. with amoxicillin Trade Names: D: Augmentan SmithKline Beecham; 1982-comb.. with amoxicillin Betabactyl S

Trang 1

Hepasteril B compositum, Reducdyn (Nordmark)- F: Thioncycline (Merrel1)-

wfrn

Use: liver therapeutic RN: 372-75-8 MF: C6H,,N303 MW: 175.19 EINECS: 206-759-6

CN: fl-(aminocarbony1)-L-ornithine

malate (1:l)

RN: 70796-17-7 MF: C6H,,N303 C,H,O, MW: 291.26

@ by fermentation

o from Socchorornyces genus

L-arginine hydrochloride

b from orniihine

Citrulline

c from Arthrobaciel

Referencefs):

1 Fox, S.W.: J Biol Chem (JBCHA3) 123,687 (1938)

2a JP 52 143 288 (Kyowa; appl 20.5.1976)

2b JP 50 148 588 (Miura; appl 23.5.1974)

2c JP 53 075 387 ( ~ y o w a ; appl 13.12.1976)

alternative syntheses:

JP 122 48/67 (Ajinomoto; appl 1 1.9.1965)

JP 117 58/68 (Kyowa; appl 15.1 1.1965)

Fox, S.W et al.: J Org Chem (JOCEAH) 6, 410 (1 941)

crystallization:

JP 7 100 174 (Ajinomoto; appl 20.1 1.1968)

isolation from Citrullus vulgaris Schrad.:

Wada, M.: Biochem Z (BIZEA2) 224,420 (1930)

use as liver therapeutic:

FR-M 4 182 (Inst de Recherche Sci.; appl 9.3.1965)

FR-M 5 594 (Dimaphar; appl 1.7.1966)

FR-M 5 703 (Lab Carriere Carron; appl 30.8.1965)

FR-M 6 305 (Dimaphar; appl 15.12.1966)

use as digestant:

FR-M 5 695 (Lab Carriere Carron; appl 29.8.1966)

citrulline fumarate:

FR-M 6 306 (Dimaphar; appl 15.12.1966)

Trang 2

492 C Cladribine

citrulline maleate:

FR-M 6 443 (Dimaphar; appl 21 A.1967)

Formulation(s): amp 60 mg/15 ml; drg 25 mg, 100 mg

Trade Name(s):

D: Polilevo (Taurus Pharma)- Perifago (Pharmacia & Citruplexina (Synthe1abo)-

F: Azonutril (Pharmacia & Stimol (Biocodex; as Ipoazotal (SIT)-comb

Epurarn (Pharmafarm)- I: Biotassina (UCM)-comb

comb

Cladribine

(NSC- 105014-F; RWJ-2625 1 ; 2-CdA)

RN: 4291-63-8 MF: C,,H,,CIN,O, MW: 285.69

CN: 2-chloro-2'-deoxyadenosine

ATC: LOlBB04 Use: antineoplastic

CH, 2.6-dichloro- 2-deoxy-3.5-di-O-p-

p u r i n e toluayl-a-D-erythro-

pentofuronosyl chloride

1 NH3, CH,OH 100 O C

2 chrornatogrophy

Clodribine

I

purine (I)

Trang 3

guanosine

1 pyridine OMF k

1 pentyl nitrite, K2C03,

CH2C12 (C,H,),CCI

2 NH,OH, THF

OH OH

Z-chloro- odenosine

pyridine

111 1.3-dichloro- 1 l.3,3-tetro-

DMAP, ocetonitrile

+ c ' r O ~ -+

0-phenyi chloro- thioformote

1 Bu3SnH AIBN, benzene, A

2 Bu,N+F- THF

Clodribine

1 tributyltin hydride

2 tetrobutvlommonium fluoride E l

2-chloro-2'-0-phenoxy-

thiocorbonyl-3'.5'-0-

(tetroisopropyldisiioxonylene)-

Trang 4

494 C Clavulanic acid

Refc?rence(s):

a Kazimierczuk, Z et al.: J Am Chem Soc (JACSAT) 106,6379-6382 (1984)

EP 173 059 (Univ Brigham Young; appl 17.7.1985; USA-prior 6.8.1984, 15.1.1987)

Christensen, L.F el al.: J Med Chem (JMCMAR) 15,735 (1972)

b US 5 208 327 (Ortho Pharm Corp.; appl 16.4.1992; USA-prior 18.12.1991)

compositions for treatment of rheumatoid arthritis:

US 5 310 732 (Scripps Res Inst.; appl 19.2.1992; USA-prior 3.2.1986)

Formulatiort(s): inj sol 10 mg/lO ml

Trade Name( s):

D: Leustatin (Janssen-Cilag) GB: Leustat (Janssen-Cilag)

F: Leustatine (Janssen-Cilag) USA: Leustatin (Ortho Biotech)

Use: P-lactamase inhibitor RN: 58001 -44-8 MF: C,H,NO, MW: 199 I6 EINECS: 261-069-2

LDS,,: 4 g/kg (M, i.v.); 4526 mg/kg (M, p.0.);

7936 rnglkg (R, p.0.)

CN: [2R-(2a,3Z,5a)]-3-(2-hydroxyethylidene)-7-oxo-4-oxa-l-azabicyclo[3.2.0]heptane-2-carboxylic acid

monosodium salt

RN: 57943-81-4 MF: C,H,NNa05 MW: 221.14 EINECS: 261-032-0

LD,,,: 4 glkg (M, i.p.); 4500 rnglkg (M, LC.)

From cultures of Streptornyces clavuligerns

Reference(s);

US 4 529 720 (Beecham; 16.7.1985; GB-prior 2.4.1974)

US 4 367 175 (Glaxo; 4.1.1983; GR-prior 7.2.1975)

GB 1 508 977 (Beecham; appl 11.4.1975; GB-prior 2O.4.l974,2l.6.l974.9.lO.l974, 1 I 12.1974) DOS 2 517 316 (Beecham; appl 18.4.1975; GB-prior 20.4.1974, 21.6.1974,9.10.1974, 11.12.1974)

DE 2 560 074 (Beecham; appl 18.4.1975; GB-prior 20.4.1974, 21.6.1974.9.10.1974, 1 1.12.1974)

pure salts ( e g Nu-, Li- and other salts);

US 4 490 294 (Beecham; 25.12.1984; GB-prior 7.2.1975, 17.3.1975)

US 4 490 295 (Beecham; 25.12.1984; GB-prior 7.2.1975, 17.3.1975)

GB 1 543 563 (Glaxo; appl 7.2.1975, 17.3.1975; Compl Spect 6.2.1976)

tert-bu~lamine salt:

EP 26 044 (Beecham; appl 15.8.1980; GB-prior 24.8.1979)

US 4 454 069 (Beecham; 12.6.1984; GR-prior 24.8.1979)

various salts:

US 4 367 175 (Glaxo; 4.1.1983; GB-prior 7.2.1975, 17.3.1975)

esters:

Trang 5

formularion with amoxicillin:

US 4 301 149 (Beecham; 17.1 1.1981; GB-prior 11 lO.I977)

EP 49 061 (Beecham; appl 6.9.198 1 ; GB-prior 27.9.1980)

EP 52 962 (Beecham; appl 2.1 1.1981; GB-prior 20.1 1.1980)

GB 2 084 016 (Beecham; GB-prior 27.9.1980)

formulation with penicillins and cephalosporins:

DOS 2 559 41 1 (Beecham; appl 18.4.1975; GB-prior 20.4.1974,21.6.1974,9.10.1974, 11.12.1974)

Fonnulution(s): drops 12.5 mglml; f c tabl 125 mg; tabl 125 mg; vial 0.1 g, 0.2 g, 0.275 g, 0.6 g, 1.2 g, 2.2 g

(as potassium salt)-comb with amoxicillin

Trade Name(s):

D: Augmentan (SmithKline

Beecham; 1982)-comb

with amoxicillin

Betabactyl (SmithKline

Beecham)-comb, with

t~carcillin

F: Augmentin (Sm~thKline

Beecham; 1984)

I

Ciblor (Inava)

Claventin (SmithKline

Beecham)

GB: Augmentin (SmithKline

Beecham; 1984)-comb

with amoxicillin

Timentin (SmithKline Beecham)-comb

I: Augmentin (SmithKLine

B Farm.)-comb

Clavucar (Smith Kline &

French)-comb with ticarcilline Clavulin (Carlo Erba)- comb

Neoduplamox (Smith Kline

& French)-comb:

Timentin (SmithKline Beecham)-comb with ticarcilline

all combination preparations with amoxicillin J: Augmentin (Beecham- Meiji)-comb with amoxicillin USA: Augmentin (SmithKline Beecham: 1984)-comb with amoxicillin Timentin (SmithKline Beecham)

Use: anti-emetic, specific antagonist of peripheral and central dopamine receptors, reversible MAO-inhibitor RN: 55905-53-8 MF: CzoHz4CIN,02 MW 373.88 EINECS: 259-885-9

LD,,: 260 mg/kg (M, i.m.); 40 mglkg (M, i.p.); 51 mglkg (M, i.v.); 490 mglkg (M, p.0.): 350 mglkg (M, s.c.):

1450 mg/kg (R, i.m.); 155 mglkg (R, i.p.); 39 mglkg (R, i.v.); 2540 mglkg (R, p.0.); 4850 mglkg (R, s.c.) CN: 4-amino-5-chloro-2-methoxy-N-[l-(phenylmethyl)-4-piperidinyl]benzamide

monohydrochloride

RN: 57645-39-3 MF: C2,H2,C1N30, HCI MW: 410.35

LD,,: >I @kg (M, p a )

malate (1:l)

RN: 57645-91-7 MF: C,,Hz4CIN,0z C4H,0S MW: 507.97 EINECS: 260-874-6

LD,: 51 mgtkg (M, i.v.); 490 mglkg (M, p.0.);

39 mgkg (R, i.v.); 2540 mglkg (R, p.0.);

>800 mg/kg (dog, p.0.)

2 CI2, FeCI,

b 1

1 , dimethyl sulfote

HN CH, I' 2 chlorine

0

Trang 6

496 C Clemastine

CI CH3

HN CH3

K

0

methyl 2-methoxy-

4-aceiamido-5-

chlorobenzoate (I)

COOH

2-methoxy-4- amino-5-chloro- benzaic acid (11)

2 111

NH2

Clebopride

1-benzyl-4-amino- piperidine (In)

DE 2 513 136 (Anphar; appl 21.3.1975; GB-prior 21.3.1974)

US 4 138 492 (Anphar; 6.2.1979; appl 17.3.1975; GB-prior 21.3.1974)

Prieto, J et al.: J Pharm Pharmacol (JPPMAB) 29, 147 (1977)

alternative synthesis:

JP 63 295 558 (Asahi; appl 26.5.1987)

JP 63 295 557 (Asahi; appl 26.5.1987)

synthesis of intermediates:

JP 63 295 559 (Asahi; appl 26.5.1987)

transdermal patch:

EP 303 445 (Fordonal; appl 9.8.1988; J-prior 13.8.1987)

Formulation(s): amp 1 mg; sol 0.5 mg; syrup 0.5 mg; tabl 0.25 mg, 0.5 mg (as hydrogen maleate)

Trade Name(s):

I: Cleprid (Recordati; 1987) J: Amicos (Banyu; 1985)

Clemastine

(Meclastine)

ATC: D04AA 14; R06AA04 Use: antiallergic, antihistaminic RN: 15686-51-8 MF: CzIH,,CINO MW: 343.90

CN: [R-(R*,R*)]-2-[2-[1-(4-chlorophenyl)-l-phenylethoxy]ethyl]-l-methylpyrrolidine

hydrogen fumarate (1:l)

RN: 14976-57-9 MF: C2,H2,C1N0 C4H404 MW: 459.97 EINECS: 239-055-2

LD,,: 43 m g k g (M, i.v.); 730 mglkg (M, p.0.);

82 m g k g (R, i.v.); 3550 m g k g (R, p.0.)

Trang 7

d CI

benzophenone chloride

4'-chloro- phenylmognesium

OcetoDhenone bromide

1 NaH, aylene

(+)-2-(2-chloro-

ethyl)-1 -methyl-

pyrrolidine

1 froctionol crystollizotion of rnoleotes

2 resolution with

(-)-dibenzoyl-L-tllrtoric acid

c'l

mixture of

4 isomers (U)

Clemostine

1

Reference(s):

Ebnijther, A.; Weber, H.-P.: Helv Chim Acta (HCACAV) 59, 2462 (1976)

GB 942 152 (Sandoz; appl 14.12.1960; CH-prior 19 I l96O, 3.8.1 960, 27.9.1960)

FR-M 1 313 (Sandoz; appl 13.7.1961)

preparation of 2-(2-chloroethy1)- 1-methylpyrrolidine enantiomers:

Vemier, J.M et al.: I Med Chern (JMCMAR) 42 (10) 1684 (1999)

Formul~ion(s): amp 2 rngl5 ml; gel 300 mglg (as hydrogen furnarate); syrup 0.5 mg/lO ml; tabl 1 mg

Trade Namr(s):

Corto-Tavegil (Novartis

Pharma)-comb

Tavegil (Novartis

Consumer Health)

Tavkgil (Sandoz); wfm

Tavegil (Nnvartis; as

hydrogen furnarate)

Tavegil (Sandoz)

Anhistan (Nippon Zoki) Fulurninol (Tatsumi) Antriptin (Nippon Yakuhin) Fumalestine (Hishiyama)

Kinotomin (Toa Eiyo)

Trang 8

498 C Clemizole

Lacretin (Tokyo Tanabe) Natarilan (Nippon Telgin G (Takata)

Maikohis (Nihon Yakuhin) Piloral (Nippon Kayaku) Xolamin (Sanko)

Masletenc (Shioe) Tavegyl (Sandoz-Sankyo) Travist (Sandoz); wfrn

Use: antihistaminic, antiallergic RN: 442-52-4 MF: C,,H,,CIN, MW: 325.84 EINECS: 207-133-5

CN: l-[(4-chlorophenyl)methyl]-2-(l-pyrrolidinylmethyl)-1H-benzi~dazole

monohydrochloride

RN: 1163-36-6 MF: C19H2,CIN, HCI MW: 362.30 EINECS: 214-605-4

LDso: 75 m g k g (M, i.v.); 837 m g k g (M, p.0.);

7 4 m g k g (R, i.v.); 1950 mgfkg (R, p.0.)

1 -chloro- 4-chloro-

2 - n i t r o - benzylamine

benzene

Reference(s):

US 2 689 853 (Schering AG; 1954; D-prior 1950)

alternative syntheses:

D E 980 644 (Schering AG; appl 1950)

D E 901 649 (Schering AG; appl 1951)

Formulation(s): cream 10 mgl40 g; suppos 5 mg

Trade Name(s):

D: Megacillin (Grunentha1)- F Deliproct (Schering)- Ultraproct (&hering)-

Scheriproct (Scherax)- Ultralan (Schering); wfm I: Ultraproct (Schenng)-

comb.; wfm GB: - Scheriproct (Schering)-

comb.: wfm

Trang 9

Clenbuterol ATC: R03AC14;R03CC13

IJse: bronchodilator

LD5,: 27.6 mgkg (M, i.v.)

CN: 4-amino-3,5-dichloro-a-[[(1,1-dimethylethyl)amino)methyl]benzenemethanol

hydrochloride

RN: 21898-19-1 M E C,2H,8C12N20 HCI MW: 313.66

4'-nitro- 2-brorno-4'-nitro-

acetophenone acetophenone

Hz, Raney-Ni 0 H

0

CI

I Clenbuterol 1

Trang 10

500 C Clidanac

Reference(s):

Keck, J et al.: Arzneim.-Forsch (ARZNAD) 22, 861 (1972)

a DOS 1 793 416 (Thornae; appl 5.9.1967)

BE 704 213 (Thornae; appl 22.9.1967; D-prior 22.9.1966, 15.2.1967, 2.6.1967)

US 3 536 7 12 (Boehringer Ing.; 27.10.1970; D-prior 22.9.1966, 15.2.1967, 2.6.1967)

b DOS 2 157 040 (Thornae; appl 17.1 1.1971)

DE 1 543 928 (Thornae; appl 22.9.1966)

alternative syntheses:

DAS 2 354 959 (Thomae; appl 2.1 1.1973)

Fort?zulation(s): drops 0.059 mg/ml, 15 mg12 ml; syrup 0.005 rnd5 ml; tabl 0.01 mg, 0.02 rng (as

hydrochloride)

Trade Name(s):

D: Contraspasrnin (ASTA I: Broncodil (Leben's) Prontovent (Salus

Spasrno-Mucosolvan Contrasrnina (Falqui) J: Spiropent (Teijin-Kissei) (Boehringer 1ng.)-comb Monores (Valeas)

Use: non-steroidal anti-inflammatory, antipyretic

RN: 34148-01-1 MF: Cl,Hl,CI02 MW: 278.78

LD,,,: 41 mglkg (R, p.0.)

CN: 6-chloro-5-cyclohexyl-2,3-dihydro-1H-indene-l-carboxylic acid

1 Li, ?I

1 AICI, & ~ H ~ c - & ~ H

2 H,SO, 3 HCI CH ,COOH

1.3-dithiane phenylcyclo- J-chloro-

h e x o n e (I) propionyl

chloride

5-cyclohexyl-l- indonane

F'

_*

N-chloro- succinimide 5-cyclohexyl- 1 -indon-

corboxylic acid (11)

Clidonoc

L

TiCI,

CI 0,

1 + Y CH, -+ A

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