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Pharmaceutical Substances Syntheses, Patents, Applications - Part 151 pptx

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magnesium salt zinc salt choline orotate L-lysine orotate ocetyl chloride I Orotic ocid I 1.. glyoxylic acid ominoaceto- sodium cyon0te hydantoic acid... Behrend: Justus Liebigs

Trang 1

Ornipressin 0 1501

CN: 8-L-ornithinevasopressin

Z OH H

Tos

Z

Tos

Z

R

0

NP:

Ornipressin

FR 1 396 607 (Sandoz; appl 3.4.1964; CH-prior 5.4.1963)

Huguenin, R.L.; Boissonnas, R.A.: Helv Chim Acta (HCACAV) 46, 1669 (1963)

Bodanszky, M et al.: J Am Chem Soc (JACSAT) 86,4452 (1964)

Trang 2

1502 0 Orotic acid

Formulation(s): amp 2.5 iu10.5 ml, 2.5 iu/5 ml

Trade Name(s):

Pharma)

Orotic acid

(Acide orotique)

Use: metabolic therapeutic, electrolyte carrier

LD,,,: 770mg/kg(M, i.v.);2g/kg (M.p.0.)

potassium salt

LD,,,: 10.9 g/kg (R, p.0.)

magnesium salt

zinc salt

choline orotate

L-lysine orotate

ocetyl chloride

I Orotic ocid I

1 OHC-COOH NoOH

0 2 HCI

H 1 glyoxylic acid ominoaceto- sodium cyon0te hydantoic acid

Trang 3

Orotic acid 0 1503

H

Orotic acid

rnaleic acid rnonoureide 5-brornodihydro-

orotic ocid

11 , CH3COOH H

trichloroocetyl 0 0

Reference(s):

a DAS 1 770 117 (Diamalt; appl 2.4.1968)

DAS 2 025 247 (Lonza; appl 23.5.1970; CH-prior 28.5.1969)

b DAS 2 502 951 (Diamalt; appl 24.1.1975)

US 4 113 950 (Diamalt; 12.9.1978; D-prior 24.1.1975)

c CH 595 351 (Lonza; appl 7.5.1975)

d US 4 064 126 (Lonza; 20.1 2.1977; CH-prior 1 1.8.1975)

DOS 2 540 275 (Lonza; appl 24.2.1977; CH-prior 11.8.1975)

alternative syntheses:

j b m oxalacetic acid ester a n d urea:

Miiller: J Prakt Chem (JPCEAO) 56, 488 (1897)

Behrend: Justus Liebigs Ann Chem (JLACBF) 378, 165 (1910)

US 2 937 175 (RhBne-Poulenc; 17.5.1960; F-prior 18.1.1956)

DE 1 034 640 (RhBne-Poulenc; appl 1956)

from aspartic acid:

Nye, F et al.: J Am Chem Soc (JACSAT) 69, 1382 (1947)

from glyoxylic acid and hydantoin:

US 4062 847 (Diamalt; 13.12.1977; D-prior 24.1.1975)

fermentatively:

US 3 086 917 (Kyowa Hakko; 23.4.1963; J-prior 15.6.1960)

lithium orotate:

DOS 2 410 181 (Nadrol-Chemie; appl 4.3.1974)

Formulation(s): cps 250 mg (as hydrochloride); cps 60 mg in comb with a-tocopherol acetate; tabl 20 mg

(as zinc salt), 40 mg (as zinc salt), 500 mg (as choline orotate)

Trade Narne(s):

D : Vigodana N (Loges)-comb numerous combination Orolyl (Porcher-Lavril);

Trang 4

1504 0 Orphenadrine

Vita-thirteen (Sumitomo) generic

Use: antiparkinsonian, muscle relaxant

LD,,,: 33 mgkg(M,i.v.); 125mg/kg(M,p.o.)

hydrochloride

LD,,,: 20 m g k g (M, i.v.); 100 mglkg (M, p.0.);

27.5 mglkg (R, i.v.); 255 m g k g (R, p.0.)

citrate (1:l)

2-methylbenzhydryl Z-dimethylamino-

chloride ethanol

Orphenadrine

Reference(s):

US 2 567 351 (Parke Davis; 1951; prior 1946)

US 2 991 225 (~rocades-~theema;; 4.7.1961; NL-prior 1952)

Bijlsma, U.G et al.: Arzneim.-Forsch (ARZNAD) 5 , 7 2 (1955)

Formulation(s): amp 60 mgl2 ml; s r tabl 100 mg; tabl 100 mg (as citrate)

Trade Name(s):

Freyssinge)-comb.; wfm

Oseltamivir

(GS 4104)

Use: antiviral, anti-influenza, neuramidase inhibitor

CN: (3R,4R,5S)-4-(Acetylamin0)-5-amino-3-(1 -ethylpropoxy)-1 -cyclohexene- 1-carboxylic acid ethyl ester

phosphate

RN: 2042.55-1 1-8 MF: C,,H2,N2O4 H304P MW: 410.40

hydrochloride

citrate

Trang 5

Oseltamivir 0 1505

HO COOH

QOH

+ H3C-0 0 - C H 3 Tos-OH, ocetone

OH H 3 C C H 3 p-toluenesulfonic

ocid

(-)-quinic acid 2.2-dirnethoxy-

propone

3.4-0-isopropylidene- 1,5-quinic loctone (I)

SO2CI2 -20°C

pyridine CH2CI2

sulfuryl chloride

ethyl 3.4-0-isopropylidene- 3-pentonone (111) ethyl 3.4-0-(1 -ethylpropylidene)-

5-0-(methonesuIfonyl)-

shikimate (11)

5-0-(methonesulfonyl)- shikimate (N)

1 ~ ~ 3 ~ - ~ - ~ - B F ~ ~ - ~n3c/ 'cn3 ~ 3

CH, 0

2 KHC03 aq C2H50H

1v

1 trimethylsilyl triflote

ethyl (3R,4R,5S)-4.5- epoxy-3-(1 -ethylpropoxy)-

1 -cyclohexene- 1 -corboxylote (V)

1 sodium ozide I

2 triphenylphosphine

1 NoN3, NH,CI D M F

2 0 0

H 3 c J - o K c H 3 ,

2 ocetic anhydride

0 C 0 , 3

1 Hz Roney-Ni C2HSOH

Aoc:H3 2 8% H3PO+ ,

N 3

Trang 6

1506 0 Otilonium bromide

H ~ C - O H

_*

H 3 C - 0 ~ 0 - C H 3

OH 2.2-dimethoxy-

isopropylidene- shikirnote (VII)

R

H3C-S-CI , TEA

11

0

V l l b 11 -b V -+

sulfonic ocid

Reference(s):

a RohlofP, J.C et al.: J Org Chem (JOCEAH) 63, 4545-4550 (1998)

WO 9 626 933 (Gilead Sciences; appl 26.2.1996; USA-prior 27.2.1995)

US 5 886 213 (Gilead Sciences; 23.3.1999; USA-prior 22.8.1997)

US 5 859 284 (Gilead Sciences; 12.1.1999; USA-prior 23.8.1996)

b Federspiel, M et al.: Org Process Res Dev (OPRDFK) 3 (4) 266-274 (1999)

Tmde Nurne(s):

CH: Tami flu (Roche; 1999)

LD,,,: 46.5 mglkg (M, i.v.); > I 500 mglkg (M, p.0.);

14.1 mg/kg (R, iv.); >I650 mglkg (R, p.0.)

diaxone, pyridine

- 1

N H 2

4-(2-octyloxybenzoyl-

ornino)benzoic acid (I)

4-(2-octyloxybenzoylornino)- benzoyl chloride

Trang 7

Oxaceprol 0 1507

methyl bromide

Otilonium bromide

Reference(s):

DOS 1 643 458 (Menarini; appl 15.9.1967; I-prior 17.9.1966)

US 3 536 723 (Menarini; 27.10.1970; I-prior 27.9.1966)

Ghelardoni, M et a].: J Med Chem (JMCMAR) 16, 1063 (1973)

Formulation(s): amp 150 mg; drg 4 0 mg; suppos 20 mg; tabl 40 mg

Trade Narne(s):

Oxaceprol ATC: D 1 I A X O ~ ; MO I ~ ~ 2 4

(Aceprolinum; N-Acetyl-4-hydroxy-L-proline) Use: connective tissue therapcutic,

antirheumatic

CN: trans- 1-acetyl-4-hydroxy-L-proline

trans-L-hydroxy- ocetic anhydride

proline

H

CH,COOH

D coo,

HO 0 0 -

Oxaceprol

u

?-

HO

Reference(s):

GB 1 246 141 (P and B Coirre; appl 30.8.1968; F-prior 14.9.1967, 16.5.1968)

DAS 1 795 327 (S.A.R.L Franco-Chimie; appl 13.9.1968; F-prior 14.9.1967, 16.5.1968)

DOS 2 139 476 (P and B Coirre; appl 6.8.1971)

For~nulation(s): f c tabl 200 mg

Trade Narne(s):

Trang 8

1508 0 Oxacillin

Use: antibiotic

LD,,,: 1490 m g k g (M, i.v.); 6500 mgkg (M, p.0.)

azabicyclo[3.2.0]heptane-2-carboxylic acid

monosodium salt monohydrate

RN: 7240-38-2 MF: C,yHIRN3Na0,S H 2 0 MW: 441.44

benzoldehyde benzoldoxime benzhydroxirnic

acid chloride (I)

aceloacetic m i d ethyl 5-methyl-3-phenyl- 5-methyl-3-phenylisoxo-

ethyl ester isoxorale-4-corbaxylate zale-4-carbaxylic acid (Il)

11

thionyl

chloride

5-methyl-3-phenyl-

isoxazole-4-carbonyl

chloride

Oxacillin

Refermce(s):

US 2 996 501 (Beecham; 15.8.1961; GB-prior 31.3.1960)

GB 905 778 (Beecham; appl 3 1.3.1960; valid from 14.3.1961)

GB 958 478 (Beecham; appl 28.2.1963: USA-prior 13.3.1962)

Formularion(s): cps 250 mg, 500 mg; vial 0.5 g, 1 g (as sodium salt)

Trade Name( s):

Use: antidepressant

Trang 9

Oxaflumazine 0 1509

hydrochloride

LD,,: 80 mglkg (M, i.v.); 365 mglkg (M, p.0.)

CI+O*%

bromine

2-chloroethyl

vinyl ether

1 -brorno-2-(2-chloro-

ethoxy)-2-(3-trifluoro-

rnethylpheny1)ethone (I)

phenylrnognesiurn (2-ch1oroethoxy)- bromide 1.2-dibrornoethone

toluene, A

isopropylarnine ( Oxoflozane

DOS 1 910 477 (CERM; appl 1.3.1969; F-prior 4.3.1968, 29.5.1968 18.6.1968,27.8.1968, 15.1 1.1968,

19.2.1969)

US3637680(CERM; 25.1.1972;F-prior.4.3.1968,29.5.1968, 18.6.1968,27.8.1968, 15.11.1968, 19.2.1969) Busch, N et a].: Eur J Med Chem.-Chim Ther (EJMCAS) 11, 201 (1976)

Formulation(s): drops 2 %

Trade Narnefs):

Use: psychosedative

hydrogen succinate (1:l)

RN: 41761-40-4 MF: C26H32F,N,02S C4H604 MW: 625.71

10-(3-pipera2inopropyl)- 2-(2-chloroethy1)-

2-trifluorornethyl- 1,3-dioxone

phenothiozine (from acrolein, 1.3-

(cf fluphenozine propanediol ond HCI)

synthesis)

Trang 10

1510 0 Oxaliplatin

Reference(s):

DAS 1 620 281 (Roussel-Uclaf; appl 28.6.1965; F-prior 29.6.1964,28.9.1964)

Ratouis, R.; Boissier, J.R.: Bull Soc Chim Fr (BSCFAS) 1966, 2963

alternative synthesis:

DOS 1 9 11 719 (S.I.F.A.; appl 7.3.1969; F-prior 8.3.1968)

Trade Narne(s):

wfm

Oxaliplatin

( I -0HP; NSC-266046; RP-54780)

LD,,,: 19.8 mg/kg (M, i.p.);

14.3-15.6 mglkg (R, i.p.)

1 (R),P(R)-di-

aminocyclohexone

Oxaliplatin

Reference(s):

Kidani, Y et al.: J Clin Hematol Oncol (JCHODP) 7, 197 (1977)

JP 53 03 1 648 (Kidani; appl 25.3.1978; J-prior 6.9.1976)

JP 09 132 583 (Tanaku Kihinzobo Kogyo; appl 20.5.1997; J-prior 10.11.1995)

as stable aqueous formulation:

WO 9 604 904 (Dehiopharm SA; appl 22.2.1996; CH-prior 8.8.1994)

in combination with cisplatin:

WO 9 412 193 (Debiopharm SA; appl 9.6.1994; CH-prior 24.1 1.1992)

Formulation(s): vial 50 mg, 100 mg

Trade Narne(s):

Use: anti-inflammatory, analgesic

LD,,,: 92 mglkg (M, p.0.);

78 mglkg (R, p.0.)

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