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In any case, these external signals occur inciden-tally and ‘on average’ elicit the same response in all cells; this means that they may have different effects depending on the status of

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Collective behavior in gene regulation: Metabolic clocks and cross-talking

Michele M Bianchi

Department of Cell and Developmental Biology, University of Rome ‘La Sapienza’, Italy

By cosmic rule, as day yields night, so winter

sum-mer, war peace, plenty famine All things change…

the harmonious structure of the world depends

upon opposite tensions

(Heraclitus, 500 bc)

In the modern age, life scientists subscribe to the

ergo-dic cell hypothesis (Fig 1): they use homogenized

tissues or cultured cells, analyze extracts and draw

conclusions about a hypothetical representative cell on

the basis that all cells are ‘on average’ identical over

(short) time and space scales [1] In this representation

(statistical mechanics, where it allowed a microscopic

basis to be given to thermodynamics), the average of a

process parameter for a single cell over time and the

average over the statistical ensemble of individuals at a

given time coincide

In the ergodic hypothesis, genes are generally

divided into housekeeping genes, which are always

expressed, and regulated genes, which are expressed or

repressed under the effect of external signals The external signal might have various origins: an environ-mental condition, a physiological signal from other regions of a multicellular organism, the result of a developmental programme, epigenetic control and so

on In any case, these external signals occur inciden-tally and ‘on average’ elicit the same response in all cells; this means that they may have different effects depending on the status of each cell but, given that the population is very large and a point in time displays the same distribution of states, the average result is the same irrespective of time If we want to study the behavior of a single cell in a time-dependent manner,

by analysing a representative population of individuals,

we must artificially put all the cells into the same state

by synchronization, in order to collapse the ensemble distribution into a single state This collapse is usually unstable and, after a relatively short time, the cell pop-ulation reverts to the statistical distribution of states

Keywords

circadian clock; cross-talk; cycles; ergodic

system; message; metabolism; redox;

synchronization; transcription dynamics;

ultradian clock

Correspondence

M M Bianchi, Department of Cell and

Developmental Biology, p.le Aldo Moro 5,

00185 Rome, Italy

Fax: +39 064 991 2351

Tel: +39 064 991 2215

E-mail: michele.bianchi@uniroma1.it

(Received 10 December 2007, accepted 30

January 2008)

doi:10.1111/j.1742-4658.2008.06397.x

Biological functions governed by the circadian clock are the evident result

of the entrainment operated by the earth’s day and night cycle on living organisms However, the circadian clock is not unique, and cells and organisms possess many other cyclic activities These activities are difficult

to observe if carried out by single cells and the cells are not coordinated but, if they can be detected, cell-to-cell cross-talk and synchronization among cells must exist Some of these cycles are metabolic and cell syn-chronization is due to small molecules acting as metabolic messengers We propose a short survey of cellular cycles, paying special attention to meta-bolic cycles and cellular cross-talking, particularly when the synchroniza-tion of metabolism or, more generally, cellular funcsynchroniza-tions are concerned Questions arising from the observation of phenomena based on cell com-munication and from basic cellular cycles are also proposed

Abbreviations

ROS, reactive oxygen species; YGO, yeast glycolytic oscillation; YMC, yeast metabolic cycle.

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Clocks Looking closer at the cell or organism and taking time into account, in addition to space, chronobiologists have shown that life actually has an intimate dual existence between opposite states: day and night, wake and sleep, oxidation and reduction The organism moves cyclically from one physiological state to the other during its life Besides the intuition of Heraclitus, it has been known for a long time that animals and plants have light-dependent physiological activities entrained to the earth’s day–night cycle Over the past few decades, the molecular bases of these cyclic activities, governed by the circadian clock, have been elucidated [2] In mam-mals, they are based on the autoregulation of transcrip-tion factors and the translatranscrip-tion feedback loops of specific clock genes [3] Circadian clocks are also present

in micro-organisms, such as cyanobacteria and fungi [4,5], and involve similar transcription⁄ translation feedback oscillators [6] By definition, clocks are self-sustained and temperature compensated [7] Clocks are also cell-autonomous, i.e they work even in isolated cells, independent of the presence of other cells [8] Although the clocks of different organisms share many characteristics, it is becoming clear that the underlying molecular mechanisms might involve differ-ent and functionally unrelated actors, cyclic cellular activity being the only common behavior of function-ally convergent evolutionary pathways [9] In theory, cellular clocks are self-sustained and hence can work

in the absence of external input signals Such signals (light, temperature, metabolites, other environmental inputs) do exist but their modes of action are not always known The outward effect of the clock is the output signal, which modulates the activity⁄ transcrip-tion of target gene(s) and⁄ or affects the functioning of target cells and is fundamental for cellular cross-talk and synchronization Multicellular organisms are com-posed of tissues and organs with highly specialized physiological functions and which work in a coordi-nated manner With respect to this organization, cells

of mammalian peripheral tissues also possess internal clocks, but they are hierarchically synchronized by the pacemaker activity of the suprachiasmatic nucleus [10] However, the autonomous timekeeping of peripheral tissues remains an open question [11]

The circadian clock is intimately connected with metabolism, in particular with the redox balance in the cell [the NAD(P)H⁄ NAD(P) ratio] and heme metabo-lism [12,13] and with cyclic transcriptome profiling [14,15] Cyclically expressed genes allow the chronolog-ical separation of antagonistic metabolic pathways and confine them to the appropriate time of day [16]

t1 t2 t3 t4

a b c d

Ergodic system: cells with

clocks not entrained

Ergodic system: cells

without a clock

t1 t2 t3 t4

a b c d Space

Space

Space

Non-ergodic system: cells

with entrained clocks

t1 t2 t3 t4

a b c d

Fig 1 Application of the ergodic hypothesis to a cell population.

Expression of a representative gene in individual cells a, b, c and

d (space dimension) at different but close time points t1, t2, t3

and t4 (time dimension) The colour of the cell indicates the

gene-expression level: black, high expression; white, low

expres-sion; grey, average ⁄ physiological expression, for example, as

reported for the metabolic status in current transcription analysis.

(Upper) The ergodic hypothesis: all cells are similar in time and

space and the ‘average’ cell is truly representative of the cell

population (Middle) Cells have clocks affecting gene expression

but these clocks are not synchronized The ergodic cell is

aver-agely representative of the population in time and space, but not

of single cells Only analysis on individuals can detect the actual

oscillatory situation (Lower) The nonergodic model with

synchro-nized cellular clocks Gene expression does not vary in space,

but changes cyclically over time Expression waves are

detect-able in the population.

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In addition to the circadian cycle, other cycles are

known Infradian cycles, like the female oestrus cycle

or temperature cycles during hibernation [17], have

periods longer than 24 h Ultradian cycles, like the

neuron electric firing, the heart beat, the basic rest–

activity cycle during sleep and the yeast metabolic

cycle (YMC) have periods shorter than 24 h [18,19] In

yeast, an ultradian glycolytic cycle (yeast glycolytic

oscillation; YGO) has been known for 50 years [20]

All these cycles are composed of recurrent transitions

of the cell from one state to another, often with

oppos-ing characteristics Some can be defined as clocks

because they are cell-autonomous, self-sustained and

temperature compensated, and for some, like the

YMC, important transcriptional effects have been

demonstrated at the genomic level [21]

Cross-talking

If one were able to look at the level of the individual

cell, in addition to constitutive and regulated gene

expression, gene transcription should also vary in a

way related to the clock activity When cell

popula-tions are considered, the situation is more complex In

the ergodic cell hypothesis, expression cycles are barely

observable because each cell goes its own way, thus

averaging out any population-level oscillation

How-ever, if cells could talk to each other, synchronization

of cycles may happen The molecular oscillators of

cells in tissues and organs might be entrained by an

external pacemaker (zeitgeber in the chronobiology

literature), such as occurs in mammals, where

periph-eral clocks are synchronized by signals from the

suprachiasmatic nucleus [10] The logic underlying

temporal segregation of metabolic activities in the

single cell is then transferred to the entire tissue and to

the organism level The biological significance of the

synchronization of cellular clocks is thus correlated

with the organ’s function and is obtained by a

hier-archical cascade of signals Many different

signal-ing pathways might finally be involved in the

entrainment of the individual oscillator of peripheral

cells to the main circadian rhythm of the

suprachias-matic nucleus [22]

In comparison with a developed organism, cells

cul-tured in plates, flasks or bioreactors might be

consid-ered a physiologically homogeneous and isotropic

system in which, according to the ergodic hypothesis,

the cells live without any coordination among them,

each has its own clock working What happens to the

cyclic activities in the case of cultured cells devoid of

any higher level of structuring like tissues and organs?

This question is of particular importance when

single-cell micro-organisms are considered but the results are not concordant In cyanobacteria, the circadian clock

is a self-sustained property of individual cells, not influenced by cell duplication (i.e transmitted in phase

to daughter cells) or by other cells (not entrained by close cells with a different phase) [8] In yeast, how-ever, the ultradian YGO responsible for NADH oscil-lations occurs in isolated cells, although only if the molecular messenger is cyclically and externally provided, and in dense cultures [23] When a high cell density is reached or during colony formation cross-talk between cells becomes critically important In these cases, collective behaviors, which require cell-to-cell communication and simultaneous responses, can be easily detected Growth inhibition by contact and quorum sensing in micro-organisms are typical examples of this kind of communication Quorum-sensing molecules are secreted continuously during growth in amounts proportional to the cell density The accumulation of such chemical signals induces col-lective and coordinated actions, like bioluminescence, horizontal DNA transfer, biofilm formation, secondary metabolite production [24] and morphological transi-tion in yeasts [25,26] Quorum-sensing molecules are oligopeptides [27] and acyl-homoserine lactones [28] in bacteria, and alcohols like farnesol or aromatic alco-hols [29] in yeast, and their production is also affected

by environmental conditions

Metabolic messages Cyclic collective behaviors, by contrast to phenomena induced by quorum-sensing molecules, are not epi-sodic and require synchronization, entrained by a signal transmitted via the medium, to be detectable

in cell populations YGO is a regular alternation of high and low NADH fluorescence [20] that can be explained by regular variation in the glycolytic flux in cells with synchronous metabolism The physiological status of the cells is critical to detect or induce detect-able YGO [30] Provided that a high density of sta-tionary phase cells is attained, YGOs can be synchronized or induced by the metabolic messengers glucose or acetaldehyde [31–33] Pulsed glucose feeds also induce YGO and glucose transport seems to be deeply involved in glycolytic oscillations [34] Some researchers have suggested that the appearance⁄ disappearance of YGOs derive from an on⁄ off set of collective cyclic dynamics, rather than the synchroni-zation⁄ desynchronization of pre-existing⁄ persisting cycles [32,34]

Furthermore, continuously cultured yeast cells at high density show a cyclic metabolism, YMC, that

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alternates between high and low redox conditions [35].

YMC has the characteristics of an ultradian clock and

in continuous cultivations individual cellular oscillators

are entrained by the secretion of a signal molecule

from other cells and become synchronized The

imme-diate macroscopic event is a cyclic variation in

dis-solved oxygen, as a result of the simultaneous

transition of a large number of cells between different

phases of respiratory metabolism Many other

intracel-lular and extracelintracel-lular metabolic parameters change

during YMC, e.g carbon catabolite concentrations,

ATP, NAD(P)H and sulfur compounds [36]

Acetalde-hyde and hydrogen sulfide are highly diffusible

mole-cules that entrain individual cellular oscillators and

synchronize the culture [37,38]

In addition to NAD(P)H, reduced glutathione seems

to play an important role in recycling damaged proteins

by the reactive oxygen species (ROS) produced by

defective electron transport to molecular oxygen

Pro-tection against ROS damage during chromosomal

DNA replication might also be connected to the YMC

[39] In fact, three distinct phases can be distinguished

within the YMC: an oxidative phase, when oxygen is

reduced in the cell by mitochondrial respiration and

ROS are produced; a reductive phase, when DNA is

synthesized; and a second reductive phase, when

meta-bolic reactions producing NAD(P)H occur (glycolysis,

fatty acid oxidation) Division of the YMC into distinct

metabolic phases, in addition to the physical

compart-mentalization ensured by the presence of specialized

organelles (mitochondria, peroxisomes, endoplasmic

reticulum), prevents dangerous, futile or antagonistic

reactions from taking place simultaneously [40]

A cell will pass through a certain number of

meta-bolic rounds before it duplicates, therefore, the YMC

has been proposed as a unit for measuring cell ageing

in pace with or in addition to the number of

replica-tive cell cycles [41] What happens in the cell between

duplication events? How deeply are cellular activities

involved or entrained with metabolic changes?

Tran-scriptome analysis has revealed that gene expression

follows the metabolic rhythm [21,40] Almost all genes

are cyclically transcribed and can be clustered in three

groups: 650 are expressed in the oxidative phase, and

2429 and 2250 are expressed in the first and second

reductive phase, respectively Fewer than 200 are

expressed in each phase and can be considered ‘phase

independent’ Genes involved in specific cellular

func-tions are preferentially expressed in one phase We can

thus deduce by functional clustering, that amino acid

synthesis, ribosome assembly, sulfur metabolism and

RNA metabolism occur in the oxidative phase; cell

division and mitochondrial biogenesis occur in the first

reductive phase and glycolysis and fatty acid oxidation occur in the second reductive phase As a conse-quence, the metabolic composition of the cell varies cyclically [42]

Different metabolism, different clock? Animals, plants and light-sensitive bacteria have devel-oped and adapted their physiology to the presence of day–night cycles on earth, which is their natural envi-ronment and the circadian clock is their natural rhythm of life However, it has been reported that the circadian clock, although often predominant, is not the only oscillator working in organisms or cells, and that other cycles might emerge when the circadian clock is impaired The YMC has been characterized in yeast cells cultured in a continuous manner, under very low nutrient feed and at very high density Whether these can be considered ‘natural’ conditions for yeast is dubious and poses many questions First, yeast is one

of the oldest domestic organisms, selected over millen-nia of food manufacturing but, in recent decades, also selected in research laboratories where it is extensively studied as model organism Hence, its natural environ-mental conditions must be searched for in the pre-domestication era Like the majority of living organisms, its environment was probably characterized

by alternations between plenty and famine, the abun-dance and scarcity of sugars, high and low growth rates, fermentation and respiration In this scenario, the YMC might be a cycle within a cycle and not be the unique yeast metabolic cycle

Reiterated redox cycles are not exclusive to continu-ous cultivation because they occur also in batch culti-vations [43] (our unpublished results) at the end of cell growth (stationary phase), although with different per-iod length and regularity Metabolic cycles are also present in yeast species other than Saccharomyces cere-visiae The majority of yeasts are not physiologically inclined to fermentative metabolism, as is S cerevisiae, and prefer to respire or ferment and respire The exis-tence of a fermentative mutant of the yeast Kluyver-omyces lactis with an extremely long stationary phase characterized by an active oxidative metabolism in batch cultivation [44] (M M Bianchi, unpublished), might allow us to study redox cycles in other related yeast species

Our preliminary data indicate that cycles, i.e sus-tained oscillations of pH in the medium, are also pres-ent during the exponpres-ential growth phase, suggesting the possibility of a metabolic cycle involving the entire population, even at low cell density, and linked to fermentative metabolism (Fig 2) We have also

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dem-onstrated the presence of collective and coordinated

transcriptional cycles in cultured yeast and mammal

cells [1] The cyclically expressed genes were not

func-tionally correlated and yeast cells showing this

behav-ior were from standard batch cultivations The period

of these transcription waves was shorter than the

YMC Our data indicate that the genomic mRNA

pool varies continuously over time, with the

concentra-tion of the majority of mRNA species changing by

two- to fivefold during cycling [1] This suggests that

regulation of gene expression in response to defined

stimuli might not be performed uniquely at the level of

mRNA synthesis, but should also involve coordinated

mechanisms acting at the level of mRNA degradation

or translation (Fig 3) It is not known whether

regula-tory steps downstream of transcription can prevent

cyclic variation of the mRNA pool from being directly

transmitted at the level of protein abundance

Cyclic variation in mRNA should also be taken into

account when planning time-course-based screening of

the global transcription response to external stimuli

The currently preferred hypothesis, that the cell will

synthesize a protein only when transcription of the corresponding gene is induced by a specific input, should inevitably be challenged The mechanistic dogma ‘input fi transcription factor fi gene pro-moter fi mRNA fi protein’ does not seem to be as simple and true as assumed to date, especially in humans, where the genome is pervasively transcribed [45]: it would be of interest to experimentally investi-gate a possible correlation between cyclic and perva-sive transcription

Other questions arising YMC is typical of dense continuous cultures [23], but continuous feeding of yeast per se is unlikely to be a zeitgeber of YMC and the nature of the carbon source does not seem to affect the onset of the cycle, provided that respiration has occurred In continuous yeast cul-tivations, high cell density is inevitably associated with

a low growth rate, low nutrient feed and respiration The effect of each single parameter on YMC is hence hardly determined In the current literature, densities

Fig 2 Growth of yeast cells (cell number · 10 5 ) in a bioreactor (batch culture) is reported, together with changes in pH The course of the three major components of pH during the exponential growth phase (hours 2–14), are reported on the right Factors 2 and 3 show a cyclic behavior.

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as high as 109 cellsÆmL)1 are reported to detect YMC.

This means an average distance of 10 lm between cells

and extremely frequent (and cyclic) contact between

cells Has this phenomenon any relevance for

cell-to-cell communication and the entrainment of the YCM,

besides the chemical signals acetaldehyde and

hydro-gen sulfide? We have mentioned that S cerevisiae is a

domestic organism and that standard methods of

labo-ratory cultivation in flasks or a bioreactor are very far

removed from the natural environmental conditions

for yeast Colony formation on agar plates is probably

closer to wild (nondomestic) growth Interestingly,

yeast growing in a colony undergoes cyclic changes in

metabolism, from acidic to alkaline [46] Furthermore,

alkali-producing colonies can entrain colonies in the

acidic phase and generate synchronous metabolism on

the plate, gaseous ammonia being the zeitgeber

The alternation of conditions with opposing

charac-teristics, as suggested 25 centuries ago, is fundamental

to all phenomena involving oscillations and cycles,

which are diffused in all disciplines of natural (and

not only) sciences In biological studies over recent

decades, it has become more and more clear that

clocks are deeply involved in governing many aspects

of life at different levels: are they tricks to resolve

specific problems or are they intimately linked to the

existence and propagation of living material? One

hypothesis about the evolution of the circadian clock

and YMC is that they allowed the segregation of

potential harmful reactions, UV mutagenesis and

ROS damage, and protect organisms Is this final

statement true or are these side effects of the

basi-cally cyclic nature of life, even at the molecular level?

Is homeostasis an old idea that should be abandoned

and is homeodynamics the new key [47]? Continuous

and cyclic variation in cell composition, transcriptome,

proteome and metabolome, is certainly well suited to the optimization of metabolic reactions, to the amelio-ration of defence and to speeding up responses to envi-ronmental stimuli, but is counterbalanced by the high energetic demand of biosynthetic reactions at the gen-ome size

Acknowledgements This work was supported by MIUR (2006051483); Istituto Pasteur Fondazione Cenci-Bolognetti; Centro

di Eccellenza di Biologia e Medicina Molecolari, and Universita` degli Studi di Roma ‘La Sapienza’

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