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Epigenetics: the study of embryonic stem cells byrestriction landmark genomic scanning Naka Hattori* and Kunio Shiota Laboratory of Cellular Biochemistry, Animal Resource Sciences ⁄ Vete

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Epigenetics: the study of embryonic stem cells by

restriction landmark genomic scanning

Naka Hattori* and Kunio Shiota

Laboratory of Cellular Biochemistry, Animal Resource Sciences ⁄ Veterinary Medical Sciences, University of Tokyo, Japan

Differentiation of a specific cell type involves the

establishment of a precise epigenetic profile comprised

of genome-wide epigenetic modifications such as DNA

methylation and histone modification Because

epi-genetic modifications in gene areas regulate

transcrip-tional activity, the epigenetic profile of the cell reflects

the transcriptome of the cell, at least partially DNA

methylation is a major component of epigenetic

modi-fication in mammals [1,2] The DNA methylation

pro-file at tissue-specific differentially methylated regions

(originally named tissue-dependent and differentially

methylated regions: T-DMRs) in one cell type is

differ-ent from others and represdiffer-ents a unique property of

the cell [3,4] However, the precise mechanism behind formation of the epigenetic profile, including the DNA methylation profile during development, remains to be elucidated

A wide range of methods has been developed for qualitative and quantitative DNA methylation assays [5] Although methods based on microarray technology are undoubtedly useful and promising for analyzing whole-genome profiles of DNA methylation, as well as histone modifications [4], restriction landmark genomic scanning (RLGS), which is based on 2D electrophore-sis in combination with methylation-sensitive restric-tion enzymes [6], is still a powerful method for DNA

Keywords

DNA methylation; DNA methylation profile;

Dnmt; epigenetics; ES cells; histone

methylase; histone modification; mammalian

development; RLGS; T-DMR

Correspondence

N Hattori, Institute of Life Sciences,

Ajinomoto Co., Inc., 1-1 Suzuki-cho,

Kawasaki-ku, Kawasaki-shi 210-8681, Japan

Fax: +81 44 244 9617

Tel: +81 44 210 5959

E-mail: naka_hattori@ajinomoto.com

*Present address

Institute of Life Sciences, Ajinomoto Co.,

Inc., Japan

(Received 30 November 2007, revised 25

January 2008, accepted 29 January 2008)

doi:10.1111/j.1742-4658.2008.06331.x

During mammalian development, it is essential that the proper epigenetic state is established across the entire genome in each differentiated cell To date, little is known about the mechanism for establishing epigenetic modi-fications of individual genes during the course of cellular differentiation Genome-wide DNA methylation analysis of embryonic stem cells by restriction landmark genomic scanning provides information about cell type- and tissue-specific DNA methylation profiles at tissue-specific methy-lated regions associated with developmental processes It also sheds light

on DNA methylation alterations following fetal exposure to chemical agents In addition, analysis of embryonic stem cells deficient in epigenetic regulators will contribute to revealing the mechanism for establishing DNA methylation profiles and the interplay between DNA methylation and other epigenetic modifications

Abbreviations

Dnmt, DNA methyltransferase; EB, embryoid body; ED, epigenetic distance; EG cell, embryonic germ cell; ES cell, embryonic stem cell; RLGS, restriction landmark genomic scanning; T-DMR, tissue-specific differentially methylated region or tissue-dependent and differentially methylated region; TS cell, trophoblast stem cell; Vi-RLGS, virtual image restriction landmark genomic scanning.

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methylation analysis Although RLGS requires a larger

genomic sample than is necessary for microarray-based

methods, it has advantages for analyzing genome-wide

methylation states: (a) it is a highly reproducible

quan-titative method; (b) genomic DNA is not amplified,

thus limiting or avoiding detection bias; (c) it detects

unmethylated landmarks in the genome and keeps out

repeated sequences that are usually highly methylated;

and (d) it targets predominantly CpG islands by using

restriction enzymes that have recognition sites with

high CG contents, such as NotI Moreover, virtual

image RLGS (Vi-RLGS), a recently developed

soft-ware simulating RLGS in silico using genomic

sequences, overcomes the difficulty in identifying

sequences of RLGS fragments [7]

One of the most important advances in

develop-mental biology and cell biology is the establishment

of embryonic stem (ES) cells, which maintain the

ability to form all types of cells in the body, and can

differentiate into a variety of cell types in vitro [8]

The use of ES cells in epigenetic studies enables us to

analyze how epigenetic profiles change during

devel-opmental processes and the effects on epigenetic

regulators of fetal exposure to chemical agents In

addition, gene targeting of epigenetic regulators in ES

cells allows us to investigate the role of each

epi-genetic regulator in establishing the epiepi-genetic profile,

and study the interplay between epigenetic

tions such as DNA methylation and histone

modifica-tion In this minireview, we describe studies using

RLGS to analyze DNA methylation profiles in ES

cells

Investigation of DNA methylation

profiles during mammalian

development using ES cells

In the mammalian genome, DNA methylation occurs

in T-DMRs according to cell- or tissue-type to

regulate the expression of neighboring genes [3] By

comparing 10 different cell types and tissues, we

previously revealed that 247 T-DMRs existed among

1500 genomic loci, and that DNA methylation

pro-files comprise the methylation status of the T-DMRs

[9] The DNA methylation profile of 247 T-DMRs

was identified as a unique code for the cell or tissue

[3,4] Considering that there are more than 15 000

CpG islands in the mouse haploid genome, of which

RLGS can only sample a subset, and that there are

 200 cell types in mammals, the number of

identi-fied T-DMRs is likely to expand in future studies,

exposing even more complex DNA methylation

profiles

Differences in DNA methylation profiles between

ES and other stem cells Comparing ES cells with other stem cells established from developing embryos revealed the uniqueness of the epigenetic profile in ES cells In contrast to ES cells, which maintain the ability to differentiate into all cell types of the embryo proper [10], trophoblast stem (TS) cells originate from the trophectoderm of blast-ocysts and can differentiate only into placental cells

in vivo and in vitro [11] Differentiation of cells from the early blastomere stage to the blastocyst stage is accompanied by a change in the epigenetic profile that directs the differentiation pathway to either the embryo proper or the placenta Thus, a significant dif-ference between ES and TS cells is likely to be observed by comparing their epigenetic profiles Analy-sis by RLGS revealed that DNA methylation profiles

at T-DMRs are totally different between ES and TS cells [9] Compared with TS cells, 20 genomic loci were methylated and 57 loci were demethylated in ES cells, supporting the idea that a bifurcation of the epigenetic profile exists before development of the blastocyst Embryonic germ (EG) cells are known to have simi-lar characteristics to ES cells with respect to differenti-ation and proliferation capabilities, despite their different origins [12,13] It was demonstrated that glo-bal gene-expression profiles of ES and EG cells were indistinguishable [14] However, analysis of DNA-methylation profiles by RLGS revealed a significant difference between ES and EG cells [9] Among 1500 genomic loci in the RLGS profile, 49 (3%) were found

to be methylated differentially in ES and EG cells, indicating that ES and EG cells can be distinguished from each other by the DNA methylation profiles If

we defined ‘epigenetic distance’ (ED) as the number of differentially methylated loci per 1500 genomic loci of two given cell- or tissue types, the ED between ES and

EG cells (49) is less than that between ES and TS cells (77), confirming the previous notion that EG cells are more similar to ES cells than to TS cells (Fig 1)

Change of DNA methylation profiles during the developmental process

To examine how the DNA methylation profile changes

as the embryo develops, we utilized model differentia-tion systems and analyzed the DNA methyladifferentia-tion pro-files of ES cells, embryoid bodies (EBs), teratomas derived from the same ES cells, fetuses at E10.5 and adult organs [15] Teratomas are disorganized agglom-erates with tissue or organ components derived from all three germ layers Teratomas, as well as fetuses, have

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DNA methylation profiles that are obtained from a

mixture of heterogeneous tissues or organs, meaning

that the methylation status at each locus in a profile

reflects average levels of DNA methylation of all cell

types analyzed Thus, detectable alterations in the

DNA methylation profiles of teratomas or embryos

indicate common alterations that occurred in the whole

teratoma or embryo concurrent with the differentiation

of ES cells Among the 259 T-DMRs, including the

ori-ginal 247 T-DMRs [9], the fraction of methylated loci,

which was 51.4% in ES cells, was lower in fetuses

(40.2%) and brain of adult mice (48.6%) but higher in

kidney (53.7%) A similar change was observed in the

in vitro differentiation system; methylation levels were

low (39.6%) in EBs and higher (41.3–44.4%) in three

independently developed teratomas derived from ES

cells or EBs The number of methylated loci in the

profiles of teratomas was less than that of the somatic

tissues, probably because the teratomas still contained

a significant number of undifferentiated proliferating

cells, or all cells in teratomas were not fully

differenti-ated yet Because the methylation status of T-DMRs

partially corresponds with the transcriptional status of

the neighboring gene, identifying differentially

methyl-ated genomic loci in ES cells, EBs and teratomas is

expected to provide information about genes that are

responsible for the developmental process

Potential of ES cells in embryotoxicological

studies

Embryonic exposure to chemical agents or medicine

may have deleterious effects on proper embryogenesis,

especially during the early developmental stages Such agents may influence embryos at genetic, transcriptional and protein levels It is also conceivable that epigenetic alterations occur with exposure of embryos to these agents, because epigenetic profiles are established actively in developing embryos Differentiation of ES cells into EBs has been studied as an in vitro model of normal and abnormal mammalian development [16] Because differentiation from ES cells to EBs is accom-panied by changes in DNA methylation profiles at T-DMRs [15], the in vitro differentiation model is useful to assess the epigenetic effect of an agent on the developmental process, and helps avoid the ethical issue

of embryotoxicological surveillance of ‘epimutagens’ [17] In addition, it is necessary to assess the effects of agents on the ES cell itself, for future therapeutic use in regenerative medicine For example, dimethyl sulfoxide,

an amphipathic molecule, is a commonly used cryopre-servative for various cells, including ES cells, and a sol-vent for water-insoluble substances in cytological and cytotoxicological studies [18] It has been reported that exposure to dimethyl sulfoxide induced differentiation

in several types of cells [18], and that dimethyl sulfoxide could improve the frequency of development to the blastocyst stage after nuclear injection in mouse cloning [19] RLGS analysis revealed that dimethyl sulfoxide treatment of ES cells differentiating into EBs, at con-centrations lower than when used as a cryopreservative, resulted in the alteration in the DNA methylation profile [20] Both hypo- and hypermethylation were observed at T-DMRs depending on the genomic loci, with hypermethylation occurring at minor satellite repeats and endogenous C-type retroviruses Among epigenetic regulators, including DNA

methyltransferas-es (Dnmts) and histone modification enzymmethyltransferas-es, Dnmt3a subtypes were upregulated both at the mRNA and pro-tein level in dimethyl sulfoxide-treated cells, suggesting that dimethyl sulfoxide might have a direct impact on DNA methylation via up-regulation of Dnmt3a sub-types, at least, at hypermethylated loci and repetitive sequences

Analysis of the DNA methylation profile for therapeutic use of human ES cells in regenerative medicine

The potential use of human ES cells in the field of regenerative medicine has been discussed previously, and differentiation of human ES cells into various tis-sues has been investigated [8] Several lines of human

ES cells were established, and differences between these

ES cell lines with respect to karyotypic stability [21] and expression profiles [22] have been investigated It

ICM TE

PGC

TS cells 77 ES cells 49 EG cells

Placental cells Embryonic cells

Fig 1 Epigenetic distances between ES cells and other stem cells

derived from developing embryos ES cells derived from the inner

cell mass (ICM) of blastocysts and EG cells derived from the

pri-mordial germ cells (PGCs) in developing genital ridges can develop

into cells of the embryo proper, after they are injected into

blast-ocysts to form chimeras By contrast, TS cells derived from the

trophectoderm (TE) of blastocysts contribute only to placenta.

Although there is an apparent ED between ES cells and EG cells,

the ED of TS cells to ES cells (77) is greater than that of EG cells

to ES cells (49), confirming the similarity of EG cells to ES cells.

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has been demonstrated that mouse and human ES cells

have unique DNA methylation profiles compared with

other cell types, including EG cells, TS cells and

sev-eral adult stem cell populations [9,23] Also, key

regu-lators of development such as Oct-4 and Nanog are

controlled by epigenetic mechanisms [24,25] To ensure

the safe use of ES cells for regenerative medicine, it

will be necessary to evaluate the nature of

differenti-ated cells as thoroughly as possible Accordingly, it is

also important to evaluate the epigenetic stability of

ES cell lines Using RLGS, Allegrucci and co-workers

investigated the DNA methylation profiles of

indepen-dently isolated human ES cells after culture under

vari-ous conditions [26] They demonstrated that variations

in DNA methylation profile existed between ES cell

lines, which could not be accounted for by genetic

dif-ferences of the source embryos Although the number

of cell passages and culture conditions, such as the

existence of serum or feeder-layer, affected neither

morphology nor expression of cell markers, these

parameters changed the DNA methylation profile of

human ES cells Considerable numbers of loci with

different DNA methylation status were also aberrantly

methylated in human tumor cells [27]

Investigation of epigenetic

mechanisms with ES cells deficient

in epigenetic regulators

Homologous recombination in ES cells enables us to

perform gene targeting at specific chromosomal loci

and to investigate gene function [28] In addition,

knockout mice have been generated to study the

devel-opmental role of the gene by germline transmission of

a targeted allele Genetic manipulations of many

epige-netic regulators, including Dnmts [29–33] and histone

methylases [34,35], have been reported Genome-wide

DNA methylation analysis of ES cells deficient in

epi-genetic regulators will assist in revealing the

mecha-nism for maintaining DNA methylation in T-DMRs,

as well as the interplay between DNA methylation and

other epigenetic modifications

Mechanism for maintaining DNA methylation

at T-DMRs

Based on studies regarding the properties of Dnmts, it is

widely accepted that Dnmt1 is a maintenance DNA

methyltransferase and Dnmt3a⁄ 3b are de novo DNA

methyltransferases in vivo [36] Dnmt3a and Dnmt3b

have no preference for hemimethylated DNA [37], and a

transgene of Dnmt3a, but not of Dnmt1, to Drosophila

exhibited de novo methylation activity [38], indicating

that Dnmt3a⁄ 3b function in de novo DNA methylation, but not in maintenance DNA methylation However, following these studies, it was still unclear how Dnmt1 and Dnmt3a⁄ 3b are involved in DNA methylation

in T-DMRs, thereby establishing DNA methylation profiles of cells, and whether Dnmt3a⁄ 3b have any role

in maintenance DNA methylation in T-DMRs

We demonstrated cooperation of Dnmt1 and either Dnmt3a or Dnmt3b in the maintenance of DNA meth-ylation in gene areas [39] Using RLGS with Dnmt1-, Dnmt3a- and⁄ or Dnmt3b-deficient ES cells, we focused

on the involvement of Dnmts in the methylation of CpG islands and CpG-rich regions near genes Both Dnmt1 single mutation and Dnmt3a⁄ Dnmt3b double mutation in ES cells resulted in the demethylation of many loci Surprisingly, target T-DMRs of Dnmt1 were identical to those of Dnmt3a⁄ Dnmt3b Although a single disruption of Dnmt3a or Dnmt3b resulted in no change in DNA methylation at the same loci, it was shown that maintaining DNA methylation at identified loci requires both classes of Dnmts, Dnmt1 and either Dnmt3a or Dnmt3b Kinetic analysis of ES cells defi-cient in Dnmts indicated that demethylation in repeat sequences was progressive in Dnmt3a⁄ 3b-deficient ES cells, with notable demethylation during later stages of cell culture, whereas demethylation in Dnmt1-deficient

ES cells was more rapid and greater during the initial stages of culture [40] This implies a predominant role for Dnmt1 and supportive role for Dnmt3a and Dnmt3b in maintaining DNA methylation at the repeat sequences By contrast, further analysis by bisulfite sequencing of loci studied by RLGS determined that extensive and almost complete demethylation occurred

at genes in Dnmt3a⁄ 3b-deficient ES cells, whereas demethylation was rather moderate in Dnmt1-deficient

ES cells [39] It is probable that in Dnmt1-deficient ES cells, Dnmt3a and Dnmt3b exert de novo DNA methyl-ation activity at these genes, which are demethylated through lack of maintenance activity because Dnmt1 is absent Consequently, Dnmt1-deficient ES cells seem to have partial DNA methylation maintenance activity, which is provided by the re-methylating actions of Dnmt3a⁄ Dnmt3b (Fig 2) Dnmt3a and Dnmt3b appear to function both as maintenance and as de novo methyltransferases in gene areas, and thus are crucial for the establishment of the DNA methylation profile during development

Analyzing the interplay between DNA methylation and histone methylation Chromatin structure, which is affected by DNA meth-ylation and histone modification, is closely associated

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with the transcriptional activity of genes During

mam-malian development, the epigenetic profile is not

estab-lished solely by one particular epigenetic regulator, but

rather by the interplay of epigenetic regulators [41,42]

The relationship between DNA methylation and other

epigenetic modifications can be examined by

genome-wide DNA methylation analysis using ES cells

defi-cient in epigenetic regulators Growing evidence has

indicated that histone lysine methylation can direct

DNA methylation in many organisms [43] G9a is a

euchromatin-localized histone methylase that catalyzes

the methylation of histone H3 at Lys9 and Lys27

(H3–K9 and H3–K27) [44], which are often found in

heterochromatic regions and in transcriptionally

inac-tive loci of the genome [45] RLGS analysis of

G9a-deficient ES cells revealed a direct interaction between

DNA methylation and H3–K9 and H3–K27

methyla-tion at T-DMRs during ES cell differentiamethyla-tion [46] In

G9a-deficient ES cells, the levels of DNA methylation

decreased in some genomic loci, and Vi-RLGS

revealed the location of these loci in euchromatic

regions Chromatin-immunoprecipitation confirmed

the demethylation of H3–K9 and H3–K27 at genomic

loci following G9a knockout, indicating that

demethyl-ation of H3–K9 and H3–K27 triggered the disruption

of maintenance DNA methylation Restoration of G9a

activity by insertion of the transgene into G9a-deficient

ES cells resulted in full recovery of methylation

levels to almost all genomic loci This suggests that

G9a also facilitates de novo DNA methylation of the

target loci Because G9a does not have the

cata-lytic domain of Dnmts, G9a plays a role in DNA

methylation indirectly, possibly via methylation at H3–K9 and⁄ or H3–K27 This study also suggests the potential to discover novel targets of an epigenetic regulator that affects DNA methylation, by analyzing alterations in DNA methylation in cells deficient in the factor

Conclusions Genome-wide DNA methylation analysis of ES cells has the potential to reveal the mechanisms used to establish DNA methylation profiles, and the epigenetic effects of fetal exposure to chemical agents during mammalian development An increased number of ES cell lines deficient in epigenetic regulators will facilitate investigations into the interplay between DNA methyl-ation and other epigenetic modificmethyl-ations through identification of DNA methylation profiles by RLGS

or other genome-wide analysis methods

Acknowledgements

We thank M Higgins for reviewing the original manu-script This work was supported by the Program for Promotion of Basic Research Activities for Innovative Biosciences (PROBRAIN)

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