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Deletions of the dystrobrevin protein were performed and the ability of the mutated forms to bind to dystrophin was tested both in vitroand in a two-hybrid assay, as well as their abilit

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Dystrobrevin requires a dystrophin-binding domain to function

Karine Grisoni, Kathrin Gieseler and Laurent Se´galat

CGMC, CNRS-UMR, Universite´ Lyon, Villeurbanne, France

Dystrobrevin is one of the intracellular components of the

transmembrane dystrophin–glycoprotein complex (DGC)

The functional role of this complex in normal and

patho-logical situations has not yet been clearly established

Dystrobrevin disappears from the muscle membrane in

Duchenne muscular dystrophy (DMD), which results from

dystrophin mutations, as well as in limb girdle muscular

dystrophies (LGMD), which results from mutations

affect-ing other members of the DGC complex These findaffect-ings

therefore suggest that dystrobrevin may play a pivotal role in

the progression of these clinically related diseases In this

study, we used the Caenorhabditis elegans model to address

the question of the relationship between dystrobrevin

binding to dystrophin and dystrobrevin function Deletions

of the dystrobrevin protein were performed and the ability

of the mutated forms to bind to dystrophin was tested both

in vitroand in a two-hybrid assay, as well as their ability to rescue dystrobrevin (dyb-1) mutations in C elegans The deletions affecting the second helix of the Dyb-1 coiled-coil domain abolished the binding of dystrobrevin to dystrophin both in vitro and in the two-hybrid assay These deletions also abolished the rescuing activity of a functional transgene

in vivo These results are consistent with a model according to which dystrobrevin must bind to dystrophin to be able to function properly

Keywords: dystrophin; dystrobrevin; nematode; Caeno-rhabditis elegans

Duchenne muscular dystrophy (DMD) is an inherited

muscular disease in which the patients’ muscles gradually

degenerate So far, no treatment exists for DMD The

disease is caused by mutations affecting the dystrophin gene,

which encodes a 3685-amino-acid protein (reviewed in [1])

Dystrophin is a submembrane protein associated with a

transmembrane dystrophin–glycoprotein complex (DGC)

comprising dystroglycans, sarcoglycans, sarcospan,

syntro-phins and dystrobrevins [1–3] DGC proteins have attracted

an increasing amount of attention over the last few years,

because they might help to explain the physiopathology of

the disease, and may also provide therapeutic clues

Dystrobrevins form a family of proteins that are unique

in that they are both dystrophin-associated proteins, and

homologous to the C-terminal region of dystrophin

Alpha-dystrobrevin was originally identified as a molecule that

copurifies with nicotinic acetylcholine receptors in sucrose

gradients [4,5] It was later recognized as one of the proteins,

which associates with dystrophin to form the dystrophin–

glycoprotein complex (DGC) [4,6,7] A second

dystro-brevin, b-dystrodystro-brevin, is mainly expressed in nerve tissues

[8,9] Mice carrying a knockout mutation of the a-dystrobrevin gene (adbn mice) suffer from a cardiac and skeletal muscle myopathy reminiscent of dystrophin (mdx) mutations [10]

a-Dystrobrevin binds to dystrophin via a coiled-coiled motif present in both proteins, and to the PDZ domain containing syntrophins [11,12] Indirect evidence suggests that dystrobrevin may also bind to other members of the DGC [13] Although no enzymatic activity has yet been assigned to dystrobrevins, there are several indications that they may play a role in signalling mechanisms First, dystrobrevins are tyrosine-phosphorylated proteins [5,14] Secondly, in the absence of a-dystrobrevin, the signalling molecule, neuronal nitric oxide synthase (nNOS) disappears from the muscular membrane [10]

In addition, two lines of evidence suggest that dystro-brevin may play a key role in the muscle degeneration observed in DMD and sarcoglycanopathies; first, dystro-brevin immunostaining decreases greatly in DMD and in several sarcoglycanopathies [15] Secondly, although the DGC components (with the exception of NOS) are not affected by the absence of dystrobrevin in adbn mice, muscle degeneration occurs

The nematode Caenorhabditis elegans has homologues of most of the DGC proteins (L Se´galat, unpublished results) There is one dystrophin- and one dystrobrevin-like gene in the genome of C elegans (dys-1 and dyb-1, respectively) [16,17] C elegans dystrophin and dystrobrevin are able to bind to each other in vitro [18] in the same way as their mammalian counterparts [12], and they also bind to syntrophin [18] dys-1 and dyb-1 mutants display a similar behavioural phenotype consisting of hyperactivity, exagger-ated bending of the head when moving forward, and a tendency to hypercontract [16,17] In addition, progressive muscle degeneration is observed when dys-1 or dyb-1

Correspondence to L Se´galat, CGMC, Universite´ Lyon1, 43 bld du 11

Novembre, 69622 Villeurbanne cedex, France.

Fax: + 33 4 72 44 05 55, Tel.: + 33 4 72 43 29 51,

E-mail: segalat@maccgmc.univ-lyon1.fr

Abbreviations: DGC, dystrophin–glycoprotein complex;

DMD, Duchenne muscular dystrophy; LGMD, limb girdle muscular

dystrophy; nNOS, neuronal nitric oxide synthase; AD, activation

domain; DNA-BD, DNA binding domain; SD, synthetic dropout

medium; SBR, syntrophin binding region.

(Received 16 October 2001, revised 10 January 2002, accepted

11 January 2002)

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its association with dystrophin First, we refined the

dystrophin-binding region on dystrobrevin (Dyb-1) by

performing deletion-mapping experiments in vitro We then

tested the ability of the truncated Dyb-1 proteins to bind to

dystrophin (Dys-1) in a yeast two-hybrid assay, as well as

their ability to rescue dyb-1 mutants

E X P E R I M E N T A L P R O C E D U R E S

Construction of deleted forms of Dyb-1

forin vitro binding experiments

Deletions were carried out on the dyb-1 coding sequence,

using clone AN450 [encoding Dyb-1 amino acids 390–543

fused in frame to the GST coding sequence; plasmid pGEX

3X (Pharmacia)] [18] AN450 DNA (500 ng) was cut with

the restriction enzyme MfeI The cut DNA was then

distributed among several tubes incubated with 0.05 lL of

BAL31exonuclease for various times (typically 0–10 min)

The reactions were stopped by adding EGTA to 4 mMand

heating at 65°C for 10 min DNA was purified on a Wizard

column (Promega) and the action of BAL31 was checked by

loading an aliquot of each tube onto an agarose gel column

The DNA corresponding to the deletions required was

treated by applying T4 DNA polymerase in the presence of

nucleotides to create blunt ends, which were ligated and the

plasmids were transformed in Escherichia coli DH5 Clones

were picked randomly and analysed using sequencing

procedures Any clones carrying a frame shift were rejected

Construct 6¢4 was built using similar procedures, but using

the enzyme HindIII instead of MfeI The amino acids

removed in the deletions were 489–499 (clone 2¢5), 487–513

(clone 5¢1), 489–528 (clone 5¢2B), 471–517 (clone 5¢5B), 478–

543 (clone 2¢1), and 391–450 (clone 6¢4) Clones 2¢1 and 6¢4

have been described previously [18], but clone 2¢1 was

erroneously reported to be deleted in amino acids 478–521

This correction makes no difference to the interpretation of

our previous data

In vitro interactions

Constructs were transformed into the E coli strain BL21

DE3 and the fusion proteins were produced as follows

After cell sonication and centrifugation, the supernatant

was loaded onto glutathione–Sepharose beads

(Pharma-cia) Approximately 20 lg of resin bound proteins were

washed in binding buffer [Hepes 20 mM pH 7.4, KOAc

110 mM, NaOAc 5 mM, Mg(OAc)22.5 mM, NP40 0.05%,

dithiothreitol 1 mM, leupeptin 10 mgÆmL)1, aprotinin

10 mgÆmL)1, pepstatin 10 mgÆmL)1,

phenylmethanesulfo-nyl fluoride (1 mM)] The 35S-labelled Dys-1 C-terminal

end was synthesized using a coupled in vitro transcription

and translation kit (Promega) with cDNA yk12c11 [16]

The preparations were incubated for 2 h at 4°C GST

controls were performed using 1–2 times the amount of

fusion protein After five washes with binding buffer, the

labelled proteins were eluted by boiling the preparation for

3 min in gel loading buffer Gels were dried, exposed

Constructs for the yeast two-hybrid assay The C-terminal end of Dys-1 (amino acids 2857–3674) was fused to the DNA binding domain (DNA-BD) of the Gal4 protein For this purpose, a 2,4 kb dys-1 cDNA fragment (yk12c11) was cloned into the polylinker of pAS2-1 (Clontech) with respect to the reading frame

Dyb-1 fragments and deletions were PCR amplified using clones AN 450, 2¢5, 5¢1, 5¢2B, 5¢5B and 6¢4 in pGEX 3X as templates (see below) and cloned into pACT2 (Clontech) in frame with the activation domain (AD) of the Gal4 protein and the HA epitope The resulting constructs were called AD-AN450, AD-2¢5, AD-5¢1, AD-5¢2B, AD-5¢5B, and AD-6¢4, respectively All DNA constructs were checked by performing DNA sequencing

Yeast two-hybrid analysis Construct DNA-BD-Dys-1 was transformed into the yeast strain CG 1945 using the LiAc transformation procedure (Clontech, Yeast protocols Handbook, PT 3024-1) Trans-formants were selected on synthetic dropout (SD) media (Clontech) minus tryptophan

A DNA-BD-Dys-1 expressing yeast strain was selected and transformed with plasmids AD-AN450, AD-2¢5, AD-5¢1, AD-5¢2B, AD-5¢5B, or AD-6¢4 Transformants were selected on SD media minus tryptophan and leucin Interactions between the DNA-BD-Dys-1 protein and the various forms of the AD-Dyb-1 fusion proteins were analysed on the basis of transactivation of the HIS3 reporter gene after 3 days of growth on SD medium devoid

of tryptophan, leucin and histidin A strain carrying both the DNA-BD-Dys-1 protein and the empty pACT2 plasmid was used as a negative control

Western blots with yeast protein extracts For Western blot analysis, yeast protein extracts were prepared from strains carrying both DNA-BD-Dys-1 plasmids and AD-Dyb-1 plasmids (AN450, AD-2¢5, AD-5¢1, AD-5¢2B, AD-5¢5B, or AD-6¢4) Overnight cul-tures (5-mL) were prepared in SD media minus trypto-phan and leucin The next day, 1 mL of overnight culture was transferred into 10 mL of YPD medium The diluted culture was incubated for several hours at 30°C until D600 ¼ 0.3 for 1 mL Cells (3 D600 units) were spun down and frozen at)70 °C for at least one hour The yeast pellet was resuspended in 60 lL of sample buffer [21] After boiling the mixture for 5 min, and centrifuging for 30 s at 13 000 g, 10 lL of supernatant was loaded onto each lane of a 0.1% SDS/10% polyacrylamide gel Proteins were transferred onto a BA83 nitrocellulose membrane (Schleicher & Schuell) in transfer buffer (Tris 25 mM, glycine 190 mM, SDS 0.01%, ethanol 20%) for 1 h at 100 V AD-Dyb-1 fusion proteins were detected using a rabbit polyclonal anti-(Dyb-1) Ig [19] at a dilution 1 : 500 Peroxidase-coupled anti-(rabbit IgG) Ig (Biorad) was used at a dilution of 1 : 3000 Blots

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were revealed using the ECL+ kit (Amersham) as

recommended by the supplier

Functional assay inC elegans

First, a dyb-1 functional construct was obtained by

modi-fying a previously built dyb-1:gfp construct [19] The

dyb-1:gfp construct, which has been previously described,

was shortened on the 5¢ end to leave 2.9 kb of upstream

sequence, and various restriction enzyme sites were removed

and added by performing synonymous point mutations to

yield the construct dyb-1:gfp VII, which has single AgeI and

MluI sites at codons 390 and 543 This construct encodes a

functional Dyb-1 gene as it can rescue dyb-1 mutations (data

not shown)

Secondly, Dyb-1 construct AN450 and the deletion

derivatives described above were transferred from pGEX

into dyb-1:gfp VII using PCR-amplifying procedures with

primers carrying AgeI and MluI sites, and cloned into the

single AgeI and MluI sites of dyb-1:gfp VII (Fig 5)

Positives clones were checked by determining their

seq-uence dyb-1:gfp VII and constructs carrying either AN450

or the deletions were injected at a concentration of

1 ngÆlL)1 along with the transformation marker KP13

[22] using standard procedures [23] into worms carrying the

putative null allele dyb-1(cx36) [17] Transgenic strains were

grown at 23°C

R E S U L T S

Mapping of the dystrophin-binding site on Dyb-1 The results of a previous study suggested that the Dys-1-binding region on Dyb-1 was located in the second helix of the predicted coiled-coil domain [18] We refined this analysis by creating additional deletions by random muta-genesis and testing their affinity for Dys-1 Clones 2¢5, 5¢1, 5¢2B, and 5¢5B were obtained by inducing exonuclease digestion of the reference clone AN450, which encodes the amino acids 390–543 of Dyb-1 fused to the GST protein [18] These four clones contain various breakpoints within the second helix of the predicted coiled-coil domain (H2) (Fig 1) The deleted amino acids were 489–499 (clone 2¢5), 487–513 (clone 5¢1), 489–528 (clone 5¢2B) and 471–517 (clone 5¢5B) Clone 2¢1, lacking amino acids 478–543, was used as a negative control [18] Clone 6¢4, lacking amino acids 391–450, was used as a second positive control [18] The constructs were used to produce Dyb-1–GST chimeric proteins in E coli, which were affinity purified on gluthati-one–Sepharose beads and subjected to in vitro binding with

35S-labelled Dys-1 Clones 2¢5 and 5¢2B bound to Dys-1 at levels that were not significantly different from those of the positive controls AN450 (Fig 2) and 6¢4 (gel not shown) In contrast, the binding activity of clones 5¢1 and 5¢5B was weaker (Fig 2) The difference between clones 2¢5, 5¢1 and

Fig 1 Deletions used in this study The ‘WT’ line represents the

amino-acid sequence of the wild-type Dyb-1 protein in the predicted

coiled-coil domain region The predicted helices forming the domain are

shown by hatched boxes Numbers above the wild-type sequence

indicate the amino-acid coordinates of the helices Deletions are shown

below the wild-type sequence Numbers indicate the coordinates of the

breakpoints Deletions were generated by exonuclease digestion Note

that the 6¢4 deletion extends on the left side further than shown on the

drawing For in vitro binding experiments, the corresponding DNAs

were cloned into the pGEX vector to produce Dyb-1–GST fusion

proteins [18] The right column gives the binding affinity of the various

constructs to35S-labelled Dys-1 in arbitrary units (mean ± SD) One

unit is defined as the autoradiogram intensity obtained with the

neg-ative control GST Asterisks indicate values significantly different from

wild-type Constructs 5¢1, 5¢5B and 2¢1 have significantly reduced

affinity to Dys-1.

Fig 2 In vitro binding of Dyb-1 (dystrobrevin) to Dys-1 (dystrophin) Representative example of in vitro binding experiments The same gel is shown in Coomassie staining (top) and autoradiography (bottom) The gel was loaded with various GST–Dyb-1 fusion proteins (and GST alone) after incubation with equal amounts of in vitro translated

35

S-labelled DYS-1 The signal intensity of the autoradiogram was quantitated with a radiographic analyser (Biorad) MW, Molecular mass markers T, aliquot of the in vitro translation product.

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5¢2B is of interest because these clones have left breakpoints

differing by only two amino acids Although clones 2¢5 and

5¢2B (cutting at position 489) display a wild-type pattern of

binding behaviour, clone 5¢1 (cutting at position 487) does

not Therefore, the third heptad repeat of the second helix of

Dyb-1 (amino acids 484–490) seems to be critical for proper

Dys-1 binding to occur in vitro

Dys-1/Dyb)1 interactions in the yeast two hybrid assay

Next, we tested the ability of the various forms of Dyb-1 to

interact with Dys-1 in a two-hybrid assay The Dyb-1

control and mutant clones were fused to the activation

domain of the Gal4 yeast transcription factor and were

tested against the entire C-terminal end of Dys-1 (amino

acids 2857–3674) fused to the DNA-binding domain of

Gal4 The expression of wild-type and truncated proteins

was checked using the Western blotting procedure This

confirmed that all the fusion proteins were correctly

expressed and that the experiment was not biased by any

differences in the protein expression levels (Fig 3) Among

the six constructs tested, only the wild-type Dyb-1 fragment

and the 6¢4 fragment resulted in the growth of yeasts on

His-plates, which can occur only if Dyb-1 binds to Dys-1

(Fig 4) Similar results were obtained when a shorter Dys-1

fragment (amino acids 3402–3674) encompassing the

syn-trophin-binding domain and the coiled-coil domain

(cor-responding to BB810 in [18]) was used (not shown) These

results indicate that all the deletions affecting the second

helix of Dyb-1, including the shortest deletion (clone 2¢5),

greatly reduce the interactions between Dys-1 and Dyb-1 in

the yeast system

Functional complementation of Dyb-1 deletions

inC elegans

The only functional assay available for dystrobrevin resides

in functional complementation To test whether the

dele-tions of various parts of the coiled-coil domain had an effect

on the in vivo function of Dyb-1, we created transgenes

carrying the same deletions as those tested in vitro and in the yeast system We transferred the deletions into the vector dyb-1:gfp VII, which is a functional transgene consisting of genomic Dyb-1 sequences (Fig 5) Because the deletions are derivatives of clone AN450, a cDNA fragment that encompasses several exons, it was necessary first to check whether removing introns 7 and 8 had any effect on the rescuing activity of dyb-1:gfp VII When the 1.2-kb AgeI– MluI genomic fragment of dyb-1:gfp VII was replaced by the 450-bp AN450 cDNA fragment encoding the same amino acids (Fig 5), rescue of dyb-1(cx36) animals still occurred in two out of three lines transgenic lines (Table 1), which indicates that removing introns 7 and 8 did not impair the rescuing capacity of dyb-1:gfp VII Then we tested the various deletions Three out of the four lines obtained with deletion 6¢4 showed consistent, although only partial, rescue (Table 1) In these lines, the dyb-1 behavioural phenotype (head bending and hyperlocomotion) was intermediate between mutant and wild-type This indicates that, although deleting the syntrophin binding region (SBR) and the first helix reduces the activity of the protein, it remains partly functional Five lines were obtained with deletion 2¢5 (the shortest deletion affecting the second helix); only one out of the five lines tested showed a weak rescuing effect, which was far less conspicuous than that observed with construct 6¢4 (Table 1) Worms carrying the remaining constructs (5¢1, 5¢2B and 5¢5B) did not display any visible rescue All in all, these data indicate that deletions affecting the second helix

of the Dyb-1 coiled-coil domain strongly decrease or abolish the functional properties of Dyb-1

D I S C U S S I O N

The aim of this study was twofold: first, to confirm and refine the localization of Dys-1 binding sites on Dyb-1, and secondly to test whether there may exist a correlation

Fig 3 Western blot of Dyb-1 deletions produced in yeast Western blots

were prepared with protein extracts of yeast carrying DNA-BD-Dys-1

plasmids and empty pACT2 (lane 1), AD-AN450 (lane 2), AD-2¢5

(lane 3), AD-5¢1 (lane 4), AD-5¢2B (lane 5), AD-5¢5B (lane 6) and

AD-6¢4 (lane 7) The blot was probed with mouse monoclonal

antibodies directed against the HA epitope situated between the

C-terminal end of the activation domain of the Gal4 protein and

the various Dyb-1 proteins Molecular mass standards are shown on

the right.

Fig 4 Yeast two-hybrid assay A plate containing SD media minus leucin, tryptophan and histidine was seeded with yeast carrying DNA-BD-Dys-1 and various AD-Dyb-1 plasmids or empty pACT2 (as a negative control), and incubated at 30 °C for 3 days Growth on media devoid of histidine can occur only if Dys-1 and Dyb-1 interact and the HIS3 reporter gene is transactivated Only the wild-type construct AD-AN450 and the AD-6¢4 construct promoted growth in this assay The other constructs, all carrying deletions in the second helix of the Dyb-1 coiled-coil domain (H2), were unable to promote growth in this assay, which indicates that the H2 helix is a critical prerequisite for Dys-1/ Dyb-1 interactions to be possible.

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between the binding of dystrobrevin to dystrophin and

functional activity of dystrobrevin The C elegans model

organism was particularly well suited for the latter part

because transgenic animals can be quickly obtained in this

species As long as the catalytic, enzymatic, or other

functional activity of the dystrobrevin protein will remain

unknown, the only way of making functional

investi-gations will continue to be through complementation of

mutations

A preliminary in vitro study on Dys-1–Dyb-1 interactions

pointed to the second helix (H2) of the predicted coiled-coil

domain of Dyb-1 [18] Here, we refined this analysis by

studying additional deletions that subdivide the H2 domain

Our results confirm the previously published data and show

that H2 is involved in the interaction with Dys-1 in vitro

Within this domain, the first half seems to be particularly

critical as deletions infringing on this side lead to a decrease

in binding Constructs 2¢5, 5¢2B and 5¢1 are of particular

interest; the first two constructs break at amino acid 489 and retain binding to Dys-1, whereas the third one breaks at position 487 and its binding affinity is reduced two-fold Alternatively, this discrepancy might also be attributable to differences in the three dimensional structure of the helix imposed by amino acids on the C-terminal side of the breakpoint The predicted three-dimensional structure of the various constructs has not been investigated so far The two deletions of the H2 region that retained some

in vitrobinding activity (clones 2¢5 and 5¢2B) were unable to promote Dys-1–Dyb-1 interaction in the yeast two-hybrid system, which indicates that the yeast assay is more selective than the in vitro assay A possible explanation may reside in the differences in protein concentrations In the in vitro pull down experiment, the GST–Dys-1 moiety is in great excess

to Dyb-1, whereas Dys-1 and Dyb-1 are thought to be in the same range of concentration in the yeast assay In agree-ment with the yeast results, these two constructs (2¢5 and

Fig 5 Drawing of the constructs used for

in vivo complementation tests Top, map of the

dyb-1:gfp VII construct dyb-1:gfp VII is a

8-kb genomic fragment of the dyb-1 gene

cloned into a pGEM backbone, in which the

gfp coding sequence has been added

termin-ally to the dyb-1 coding sequence Bottom:

map of the constructs used for the in vivo

experiments The various deletions are

deri-vatives of the AN450 construct, a fragment of

dyb-1 cDNA cloned into the GST-containing

vector pGEX Deleted regions are indicated

in dark The deletions were transfered into

dyb-1:gfp VII by PCR using the unique AgeI

and MluI restriction sites of dyb-1:gfp VII As

a result, introns 7 and 8 of dyb-1:gfp VII were

removed in these constructs These construct

were injected in dyb-1(cx36) mutants to assay

their ability to rescue the mutant phenotype.

Table 1 Rescuing activity of Dyb-1 deletions Constructs were injected in dyb-1(cx36) animals along with the transformation marker KP13 [22] dyb-1(cx36) animals display a behavioral phenotype consisting of hyperactivity, exaggerated bending of the head when moving forward, and a tendency to hypercontract when moving backwards + + +, transgenic animals not distinguishable from wild-type animals; + +, transgenic animals resemble wild-type but remain slightly hyperactive and bend their head more than wild-type; +, transgenic animals remain hyperactive and bend their head, but can be distinguished from nontransgenic siblings in blind tests; ±, some transgenic animals show a slightly improved behavior but transgenics cannot be recognized with certainty in blind tests; –, no modification of the phenotype could be observed.

Construct

Number of transgenic lines

Number of rescuing lines

Rescue

in best line(s)

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results Although the 6¢4 deletion was still partly functional,

only very weak activity could be observed with deletion 2¢5

In conclusion, the results presented in this paper show

that the second helix of the coiled-coil domain of Dyb-1 is

necessary for binding to Dys-1 both in vitro and in vivo

These results are consistent with a model in which

dystrobrevin must bind to dystrophin to be able to function

properly

A C K N O W L E D G E M E N T S

We thank L Granger and P Morales for their excellent technical

assistance We wish to thank R Bourette, C Bourgin and V Corset for

helpful discussions, and A Dumont, P Me´rel, and S Que´tat for their

participation in this work during their training courses K G and L S.

were supported by a Rhoˆne-Alpes district grant and L S by an

Association Franc¸aise contre les Myopathies (A F M.) grant.

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