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Watson1 1 University of Birmingham, Edgbaston, UK In this study, we show that the G protein-coupled receptor agonist thrombin, the glycoprotein VI agonist convulxin, and the cytokine rec

Trang 1

Regulation of RAS in human platelets

Evidence that activation of RAS is not sufficient to lead to ERK1-2 phosphorylation David Tulasne1, Teresa Bori2and Steve P Watson1

1

University of Birmingham, Edgbaston, UK

In this study, we show that the G protein-coupled receptor

agonist thrombin, the glycoprotein VI agonist convulxin,

and the cytokine receptor Mpl agonist thrombopoietin

(TPO) are able to induce activation of RAS in human

platelets Recruitment of GRB2 by tyrosine-phosphorylated

proteins in response to TPO and convulxin but not by

thrombin occurred with a similar time-course to RAS

acti-vation, consistent with a causal relationship On the other

hand, activation of ERK2 by thrombin and convulxin is

delayed and also inhibited by the protein kinase C inhibitor

Ro-31 8220, whereas RAS activation is unaffected Further

evidence for differential regulation of RAS and ERK is provided by the observations that TPO, which activates RAS but not protein kinase C, does not activate ERK, and that the inhibitor of SRC kinases PP1 inhibits activation of RAS but not ERK2 in response to thrombin Our results demonstrate that activation of RAS is not necessarily cou-pled to ERK in human platelets

Keywords: ERK; glycoprotein VI; platelet; protein kinase C RAS; signalling; thrombin; thrombopoietin

RAS is a ubiquitously expressed GTPase protein, which is

activated following conversion from a GDP to GTP-bound

state GDP–GTP exchange is stimulated by SOS, which is

constitutively associated through its proline rich domain to

the SH3 domains of the adapter GRB2 The Src homology

(SH)2 domain of GRB2 is able to bind phosphorylated

tyrosine residues on tyrosine kinase receptors or

membrane-localized adapters Localization of GRB2–SOS complex to

the plasma membrane, following this recruitment, promotes

RAS activation [1–3]

RAS was discovered as an oncogene, which was in its

activated state by constitutive binding of GTP A number of

proteins, including RAF, GAPp120, MEKK1, and

phos-phatidylinositol-3 kinase (PtdIns3K) are able to interact

with activated RAS (for review see [4]) The interaction of

RAS with the serine threonine kinase RAF is the most

thoroughly characterized of these interactions RAF

regu-lates the kinases MEK, which in turn activates ERK1-2

(MAPK p44, p42) ERK1-2 are able to regulate a number

of transcription factors, cytoplasmic proteins and

down-stream kinases

RAS and all of the components of the RAS–ERK

signalling pathway (RAS, RAF, MEK, ERK) are expressed

in platelets and undergo activation It has been shown that

the G protein-coupled receptor agonists thromboxane A2 and thrombin stimulate GDP–GTP exchange of RAS [5]; the cytokine receptor Mpl agonist thrombopoietin (TPO) is able to induce activation of RAF [6]; and collagen and thrombin induce MEK and ERK activation [7] In the present study, we show that whereas RAS is activated in platelets in response to activation by thrombin, glycoprotein

VI (GPVI) agonists and TPO, this is not necessarily coupled

to activation of ERK

M A T E R I A L S A N D M E T H O D S Antibodies and reagents

Anti-RAS (clone RAS 10, recognizing p21 H-, K- and N-RAS) and anti-phosphotyrosine 4G10 monoclonal Ig were purchased from Upstate Biotechnology (TCS Biologi-cals Ltd, UK) Anti-SHC polyclonal and anti-GRB2 mono-clonal Ig were purchased from Transduction Laboratories (Becton Dickinson Ltd, UK) Anti-GRB2 polyclonal Ig and anti ERK2 polyclonal Ig were purchased from Santa Cruz Biotechnology, Inc Anti-(phospho active ERK phospho-Thr202/Tyr204) polyclonal Ig was purchased from Promega Biosciences, Inc Anti-SYK rabbit polyclonal serum was a generous gift of M Tomlinson (DNAX, Palo Alto, Ca, USA) Gluthatione S-transferase (GST)–RAF–RBD fusion protein was generous gift of Dr F McKenzie (CNRS UMR

134, Nice, France) Human recombinant TPO was from Genentech, Inc Other reagents were from previously described sources [8,9]

Platelet preparation Blood samples were collected from healthy volunteer donors into 1/10 vol 3.8% trisodium citrate (w/v) and then 1/10 vol

of acid/citrate/dextrose (ACD; 120 mM sodium citrate/

110 m glucose/80 m citric acid) was added Platelet-rich

Correspondence to D Tulasne, Department of Pharmacology,

University of Oxford, Mansfield Road, Oxford OX1 3QT, UK.

Fax: +44 1865 271853, Tel.: + 44 1865 271590,

E-mail: david.tulasne@pharmacology.oxford.ac.uk

Abbreviations: GST, gluthatione S-transferase; GPVI, glycoprotein

VI; PtdIns3K, phosphatidylinositol 3-kinase; PVDF, poly(vinylidene

difluoride); PKC, protein kinase C; PP1,

(4-amino-4-(4-methylphe-nyl)-7-(t-butyl)pyrazola[3,4-d]pyrimidine); SH2, Src homology 2;

SH3, Src homology 3; TPO, thrombopoietin.

(Received 19 October 2001, revised 1 November 2001, accepted

21 January 2002)

Trang 2

plasma was obtained by centrifugation at 200 g for 20 min.

Platelets were isolated from platelet-rich plasma by

centrif-ugation at 1000 g for 10 min, in the presence of prostacyclin

(0.1 lgÆmL)1) The pellet was resuspended in 25 mL of a

modified Tyrode’s/Hepes buffer (134 mM NaCl, 0.34 mM

Na2HPO4, 2.9 mMKCl, 12 mMNaHCO3, 20 mMHepes,

5 mMglucose, 1 mMMgCl2pH 7.3) and 3 mL ACD in the

presence of prostacyclin (0.1 lgÆmL)1) Platelets were

recen-trifuged at 1000 g for 10 min and resuspended at 5· 108

plateletsÆmL)1in Tyrode’s/Hepes buffer Platelet

stimula-tions were performed at 37°C in a PAP4 aggregometer with

continuous stirring at 1200 r.p.m (BioData Corporation)

Immunoprecipitation

Platelets (4· 108 cellsÆmL)1) treated for 10 min with

2 UÆmL)1apyrase, 10 lMindomethacin and 1 mMEGTA

were lysed with an equal volume of ice-cold Nonidet P-40

buffer [20 mMTris, 300 mMNaCl, 2 mMEDTA, 2% (v/v)

NP40, 1 mM phenylmethanesulfonyl fluoride, 2 mM

Na3VO4, 10 lgÆmL)1 leupeptin, 10 lgÆmL)1 aprotinin,

1 lgÆmL)1 pepstatin A, pH 7.3) Lysed cells and debris

were removed by centrifugation Cell lysates were precleared

for 1 h at 4°C with protein A–Sepharose Platelet lysates

were incubated overnight at 4°C with 3 lL anti-GRB2 or

anti-SHC polyclonal Ig under constant rotation Protein A–

Sepharose was added and samples were rotated for a further

60 min The pellet of protein A–sepharose was washed once

in lysis buffer and three times in NaCl/Tris/Tween (10 mM

Tris, 160 mMNaCl, 0.1% Tween 20 (pH 7.3)]

GST precipitation

Platelets (4· 108 cellsÆmL)1) treated for 10 min with

2 UÆmL)1apyrase, 10 lMindomethacin and 1 mMEGTA

were lysed with an equal volume of ice-cold Nonidet P-40

buffer containing additional 1% N-octyl glucoside and

5 mM MgCl2 Lysed cells and debris were removed by

centrifugation Cell lysates were precleared for 1 h at 4°C

with glutathione–agarose Platelet lysates were incubated

3 h at 4°C with 5 lg GST–RAF–RBD immobilized on

agarose The pellet was washed once in lysis buffer and three

times in NaCl/Tris/Tween

Immunoblotting

For ERK phosphorylation, platelets were lysed in 10·

de-naturating buffer (10% SDS, 100 mMNaCl, 50 mMTris,

pH 7.3) Lysed cells and debris were removed by

centrifu-gation Laemmli buffer was added, and the lysate was boiled

for 2 min Proteins were separated by SDS/PAGE and

transferred to poly(vinylidene difluoride) (PVDF)

mem-brane Blots were developed by using the enhanced

chemi-luminescence detection (ECL) system

Cytoplasmic and cytoskeleton localization

Platelets were prepared and stimulated as described above

and then lysed with an equal volume of ice-cold Triton

X-100 lysis buffer (100 mM Tris, 10 mM EDTA, 2 mM

phenylmethylsulphonyl fluoride, 10 lgÆmL)1 leupeptin,

pH 7.3) Cell lysates were centrifugated at 4°C for 2.5 h

at 100 000 g Pellets containing cytoskeleton proteins were

solubilized in SDS sample buffer (40% glycerol, 8% SDS, 20% b-mercaptoethanol, 0.008% Bromophenol blue,

250 mMTris/HCl pH 6.8) Proteins from supernatant and Triton X-100 insoluble-pellet were resolved on SDS/PAGE and transferred to PVDF membrane Blots were developed using the ECL system

Platelet labelling with [32P]orthophosphate Platelets suspended in Tyrode’s/Hepes without phosphate were incubated with [32P]orthophosphate (0.5 mCiÆmL)1) for 1 h at 37°C Platelets were washed once in Tyrode’s/ Hepes and resuspended at 5· 108 plateletsÆmL)1 in Tyrode’s/Hepes plus indomethacin and left 15 min before the experiment as described above Reactions were stopped using Laemmli buffer Proteins were resolved on SDS/ PAGE and visualized by autoradiography

R E S U L T S Platelet aggregation induces RAS localization

to cytoskeleton Subcellular localization of RAS was determined after stimulation of platelets by thrombin, convulxin and TPO

In nonstimulated platelets, RAS was detected in cytoplas-mic and cytoskeletal fractions, corresponding, respectively,

to detergent soluble and insoluble fractions (Fig 1) Aggregation in response to thrombin induced translocation

of RAS from the cytoplasmic fraction to the cytoskeleton fraction (Fig 1A) In the presence of EGTA or RGDS peptide, both of which inhibit GPIIb-IIIa-dependent aggre-gation, relocalization of RAS was not observed (Fig 1B and C) A similar set of results was obtained in response to aggregation induced by the GPVI agonist, convulxin (data not shown) TPO does not induce aggregation or trans-location of RAS to the cytoskeletal fraction (Fig 1D)

Fig 1 Aggregation in response to thrombin and convulxin induces relocalization of RAS from the cytoplasmic to the cytoskeleton fraction (A, B, C and D) Washed human platelets (4 · 10 8

ÆmL)1) were pre-treated or not for 10 min with 10 m M EGTA or 1 m M of RGDS peptide Platelets were then stimulated with 1 UÆmL)1thrombin or

150 ngÆmL)1TPO Platelets were lysed by the addition of Triton X-100 lysis buffer at 30, 60, 120 or 240 s Triton X-100 soluble and insoluble fractions were isolated Proteins of both fractions were resolved by 12.5% SDS/PAGE and analysed by Western blotting using an anti-RAS Ig.

Trang 3

Thombin, convulxin and TPO induce activation of RAS

RAS activation was measured through the ability of its

activated form (RAS–GTP) to bind to a GST fusion protein

consisting of the RAS-binding domain of RAF and

subsequent detection by Western blotting To prevent

trans-location of RAS to the insoluble fraction and secondary

responses, aggregation mediated by the integrin GPIIb-IIIa

was inhibited by EGTA and the activation mediated by

thromboxane A2and ADP were blocked by indomethacin

and apyrase, respectively Thrombin, convulxin and TPO

stimulated a concentration-dependent increase in RAS

activation (Fig 2A, C and E) Thrombin (1 UÆmL)1)

induced maximal RAS activation at 30 s which was

sustained for 240 s Convulxin (10 lgÆmL)1) induced

max-imal RAS activation at 10 s which was also sustained for

240 s TPO (150 ngÆmL)1) stimulated a gradual increase in

RAS activation which was detectable between 60 and 120 s

and maximal at 240 s (Fig 2B, D and F) These results

indicate that thrombin, convulxin and TPO induce RAS

activation, but with different time-courses

Convulxin and TPO induce GRB2 recruitment

to phosphorylated adapters

GDP–GTP exchange in RAS is regulated by the exchange

factor SOS, which is constitutively associated with the

adapter GRB2 A constitutive association between GRB2 and SOS was observed in platelets (data not shown) Tyrosine phosphorylated proteins associated with GRB2 were detected by coimmunoprecipitation and Western blotting using an anti-phosphotyrosine Ig As described previously, in convulxin-stimulated platelets, GRB2 binds

to 36, 50, 70 and 150 kDa phosphorylated-proteins ([10] and Fig 3A) In TPO-stimulated platelets only one

Thr.

WB: RAS

25 16 kDa

0 30 60 120

E

F

25 16 kDa

240 s.

10

Cvx

0 10 30 60 120 s.

TPO

0 10 30 60 120 240 s.

Thr U/ml

0 0.01 0.1 1

Cvx µ g/ml

0 0.1 1 10

TPO ng/ml

0 25 50 100 150

Pull-down: RAF-RBD; WB: RAS

Pull-down: RAF-RBD; WB: RAS

WB: RAS

25 16 kDa

25 16 kDa

Fig 2 Thrombin, convulxin and TPO induce RAS activation in a

concentration-dependent manner with different time-course (A, C and

E) Washed human platelets (4 · 10 8 ÆmL)1), prepared in buffer

con-taining EGTA, indometacine and apyrase, were stimulated with

increasing concentrations of thrombin for 120 s, convulxin for 120 s

and TPO for 240 s (B, D and F) Washed human platelets were

sti-mulated as indicated time with 1 UÆmL)1 thrombin, 10 lgÆmL)1

convulxin or 150 ngÆmL)1 TPO Platelets were then lysed by the

addition of RAS lysis buffer Cell extracts were precipitated using GST

fusion protein containing the RAS-binding domain of RAF

Precipi-tated proteins were resolved by 12.5% SDS/PAGE and analysed by

Western blotting using an anti-RAS Ig (top) Proteins of whole cell

lysate were resolved by 12.5% SDS/PAGE and analysed by Western

blotting using anti-RAS Ig (bottom) Results presented are

represen-tative of three experiments.

Thr.

A

IP:GRB2, WB:P-Y

Cvx _

62

IP:GRB2, WB:GRB2

25 kDa

25 kDa

25 kDa

25 kDa

62 kDa

62

25 kDa 32

Cvx _

IP:SHC, WB:P-Y

IP:SHC, WB:GRB2

IP:GRB2, WB:SYK

IP:GRB2, WB:LAT

IP:GRB2, WB:GRB2

IP:SHC, WB:P-Y

IP:SHC, WB:GRB2

TPO

0 10 30 60 120 240 s.

175 83 62 47 32 kDa

175 83 62 47 32 kDa

Cvx

0 10 30 60 120s.

IP:GRB2, WB:P-Y

IP:GRB2, WB:GRB2

C B

E D

Fig 3 Convulxin and TPO but not thrombin induce the recruitment of GRB2 on phosphorylated adapters (A, B and C) Washed human platelets were stimulated with 1 UÆmL)1 of thrombin for 120 s,

10 lgÆmL)1convulxin for 120 s and 150 ngÆmL)1of TPO for 240 s Platelets were then lysed by addition of Nonidet P-40 lysis buffer (A) Cell extracts were immunoprecipitated using polyclonal GRB2 Ig Precipitated proteins were resolved by 10% SDS/PAGE and analysed

by Western blotting using an anti-phosphotyrosine Ig (top) The filter was stripped and reprobed using a monoclonal anti-GRB2 Ig (bot-tom) (B) Cell extracts were immunoprecipitated using an anti-SHC Ig Precipitated proteins were resolved by 10% SDS/PAGE and analysed

by Western blotting using an anti-phosphotyrosine Ig (top) or a monoclonal anti-GRB2 Ig (bottom) (C) Cell extracts were immuno-precipitated using polyclonal GRB2 Ig Precipitated proteins were resolved by 10% SDS/PAGE and analysed by Western blotting using

an anti-SYK Ig (top) or anti-LAT Ig (middle) The lower part of the filter was stripped and reprobed using a monoclonal anti-GRB2 Ig (bottom) (D) Human platelets were stimulated from 10 to 240 s with

150 ngÆmL)1of TPO and were then lysed Cell extracts were immuno-precipitated using an anti-SHC Ig Precipitated proteins were resolved

by 10% SDS/PAGE and analysed by Western blotting using an anti-phosphotyrosine Ig (top) or a monoclonal anti-GRB2 Ig (bottom) (E) Human platelets were stimulated from 10 to 120 s with 10 lgÆmL)1

of convulxin and were then lysed Cell extracts were immuno-precipitated using polyclonal anti-GRB2 Ig Precipitated proteins were resolved by 10% SDS/PAGE and analysed by Western blotting using

an anti-phosphotyrosine Ig (top) The filter was stripped and reprobed using a monoclonal anti-GRB2 Ig (bottom) Results presented are representative of three experiments.

Trang 4

phosphorylated protein was detected at 50 kDa No change

in the pattern of phosphorylated proteins associated with

GRB2 was observed in platelets stimulated by thrombin

Convulxin and TPO stimulated tyrosine phosphorylation of

the 50 kDa adapter SHC, leading to formation of a

complex with GRB2 (Fig 3B) In convulxin-stimulated

platelets, GRB2 also coimmunoprecipitated with the adapter

protein LAT and the tyrosine kinase SYK, suggesting that

these phosphorylated proteins could also recruit GRB2

after stimulation (Fig 3C) Time-course studies indicated

that SHC phosphorylation and GRB2 association in

response to TPO occurred gradually with a maximal

response at 240 s (Fig 3D) In convulxin

stimulated-platelets, association of phosphorylated proteins with

GRB2 was maximal at 10 s and was sustained for at least

240 s (Fig 3E) The time-course of RAS activation in

response to convulxin and TPO was similar to the

recruitment of GRB2 to phosphorylated adapters

RAS and ERK are regulated differently

The activation of ERK1 and 2, the downstream kinases of

the RAS–ERK signalling pathway, was measured by

Western blotting using an anti-(phospho-specific ERK1-2)

Ig Thrombin and convulxin were able to induce

phos-phorylation of ERK kinase after a delay of 60 s (Fig 4A

and B) Although we have previously shown weak

phos-phorylation of ERK1 in response to thrombin and collagen

[7], only ERK2 phosphorylation was detected using the

antiphospho ERK1-2 In contrast, TPO was unable to

induce ERK1 or 2 activation (Fig 4C)

Treatment of platelets with the protein kinase C (PKC)

inhibitor Ro 31 8220 abolished phosphorylation of the

major PKC substrate pleckstrin and blocked activation of

ERK in response to thrombin and convulxin (Fig 5 A and

B) This is consistent with previous reports demonstrating

that ERK regulation is mediated downstream of PKC [7] In

contrast, activation of RAS by thrombin and convulxin was

not affected by treatment with Ro 31 8220 (Fig 5C)

suggesting that activation of RAS is not sufficient on its

own to activate ERK in platelets This is consistent with the

observation that TPO was unable to induce pleckstrin

phosphorylation or activation of ERK despite conversion of RAS to its GTP-bound form (Fig 5A and C and Fig 4C)

RAS but not ERK activation induced by thrombin

is dependent on SRC kinases SRC family kinases are necessary for the initial signalling events induced by GPVI, notably for phosphorylation of the GPVI-associated receptor FcR c-chain [11,12] As expected, the SRC kinase family inhibitor PP1 inhibited convulxin-induced ERK and RAS activation (Fig 6A,B) Interestingly, although activation of ERK in response to thrombin was not affected by PP1, activation of RAS was strongly reduced These results suggest that RAS but not ERK activation induced by thrombin is regulated by SRC

Thr.

WB: P-ERK

Ro 318220

_

Ro 318220

_ Reprobe: ERK2

WB: P-ERK

Reprobe: ERK2

Thr.

_

_

_

Cvx Cvx +Ro

TPO

Cvx

Thr _ + _ +

_ + _ +

47 kDa

Ro 318220

_

Thr _ + _ +

25 kDa

Ro 318220

_

Ro 318220

_

WB: RAS

47 kDa

WB: RAS Pull-down: RAF-RBD

WB: RAS Pull-down: RAF-RBD

Pull-down: RAF-RBD

47 kDa

47 kDa

47 kDa

47 kDa

47 kDa

25 kDa

25 kDa

25 kDa

25 kDa

25 kDa

Fig 5 PKC inhibitor Ro-31 8220 inhibited ERK but not RAS acti-vation induced by thrombin, convulxin and TPO (A, B and C) Washed platelets or [32P]orthophosphate-labelled platelets were pretreated for

10 min with 10 l M Ro 31 8220 and stimulated for 2 min with

1 UÆmL)1 thrombin, for 2 min with 10 lgÆmL)1 convulxin or for

5 min with 150 ngÆmL)1TPO (A) Stimulated labelled-platelets were lysed in Laemmli sample buffer and were resolved by 12% SDS/ PAGE Phosphorylated pleckstrin was detected by autoradiography (B) Platelets were lysed by the addition of denaturating lysis buffer Proteins of whole cell lysate were resolved by 10% SDS/PAGE and analysed by Western blotting using an anti-(phospho-specific ERK1-2)

Ig (top) The filter was stripped and reprobed using an anti-ERK2 Ig (bottom) (C) Platelets were lysed by the addition of RAS lysis buffer Cell extracts were precipitated using GST fusion protein containing the RAS-binding domain of RAF Precipitated proteins were resolved

by 12.5% SDS/PAGE and analysed by Western blotting using an anti-RAS Ig (top) Proteins of whole cell lysate were resolved by 12.5% SDS/PAGE and analysed by Western blotting using anti-RAS

Ig (bottom) Results presented are representative of three experi-ments.

Thr.

WB: P-ERK

47 kDa

0 30 60 120 s.

Reprobe: ERK2

47 kDa

2 Cvx

Fig 4 Thrombin and convulxin but not TPO induce ERK activation.

(A, B and C) Washed human platelets were stimulated for the times

indicated with 1 UÆmL)1 thrombin, 10 lgÆmL)1 convulxin or

150 ngÆmL)1TPO Platelets were then lysed by addition of

denatu-rating lysis buffer Proteins of whole cell lysate were resolved by 10%

SDS/PAGE and analysed by Western blotting using an

anti-(phospho-specific ERK1-2) Ig (top) The filter was stripped and reprobed using

an anti-ERK2 Ig (bottom) Results presented are representative of

three experiments.

Trang 5

family kinases and suggest that activation of RAS is

dispensable for efficient activation of ERK

D I S C U S S I O N

Activation of RAS was evaluated in platelets through the

ability of the activated RAS–GTP to bind a GST fusion

protein containing the RAS-binding domain of RAF

Different platelet agonists including thrombin, the snake

venom convulxin and TPO were able to activate RAS It has

been shown that H-RAS is expressed in platelets, but

expression of the isoform ki- and N-RAS was not excluded

[5] Activated RAS was detected with an anti-(pan RAS) Ig,

which does not distinguish the various isoforms of RAS In

platelets, SOS, the exchange factor of RAS, was found in complex with the adapter GRB2 In response to convulxin, GRB2 associates with a number of phosphorylated pro-teins Three of these phosphorylated proteins, the adapters LAT and SHC, and the tyrosine kinase SYK were identified These proteins belong to the signalling complex activated by phosphorylation in response to the cross-linking of GPVI, which is associated with the Fc receptor c chain The GPVI-Fc receptor c-chain signalling pathway shares many features with those of ITAM-containing receptors in the immune system [13] Following T-cell receptor activation, recruitment of GRB2 by LAT and SHC was shown to be involved in the activation of the RAS-ERK signalling pathway [14,15] The time-course of RAS activation in response to convulxin was similar to the recruitment of GRB2 to phosphorylated adapters, suggest-ing a possible regulation of RAS by convulxin through this mechanism

In response to TPO, an association between GRB2 and phosphorylated SHC was identified This interaction occurred with a similar time-course to activation of RAS, suggesting a causal relationship In megakaryocytic cell lines, it has been shown that GRB2 recruitment by phosphorylated SHC following c-Mpl receptor activation

by TPO contributes to activation of the RAS–ERK signalling pathway [16]

The SRC kinase family inhibitor PP1 inhibited activa-tion of RAS in response to thrombin Activaactiva-tion of RAS

by G coupled-receptors in other cell types is also mediated through the SRC kinases [17–19] PP1 also inhibited activation of RAS stimulated by convulxin, consistent with the role of these kinases in mediation of the phosphory-lation of the ITAM motif of the Fc receptor c chain [11,12]

As a principal mechanism, the activation of RAS leads to the activation of ERK1-2 by sequential activation of RAS– RAF–MEK and ERK In platelets, phosphorylation of ERK2 in response to thrombin and GPVI agonists is dependent on PKC ([7] and this study) In contrast, we found that a PKC inhibitor did not affect RAS activity in response to thrombin and convulxin This is consistent with the observation that TPO, which is unable to induce activation of PKC, does not stimulate activation of ERK in platelets This result indicates that activation of RAS is not sufficient on its own to lead to ERK activation The differential regulation of RAS and ERK was also shown by the different time-courses of activation between these two proteins in response to thrombin and convulxin

In a number of other cells, PKC is also able to regulate ERK activity In most of these cases, PKC activates RAF, which in turn activates the MEK–ERK cascade, but activation of ERK without involvement of RAF has also been shown [20,21] In platelets, the mechanism of ERK activation by PKC has not been elucidated However, activation of ERK by thrombin, GPVI agonists and phorbol ester is abolished by inhibitors of MEK ([22] and data not shown) suggesting that this activation occurs at the level of, or upstream of, MEK In addition, it has been shown that phorbol ester, which induces efficient activation

of ERK, is not able to induce RAF activation in platelets [6] Taken together these results suggest that regulation of ERK by PKC is not mediated through RAF but more likely through activation of MEK

Fig 6 SRC inhibitor PP1 inhibited RAS but not ERK activation

induced by thrombin (A and B) Human platelets were pretreated for

10 min with 10 l M PP1 and stimulated for 2 min with 1 UÆmL)1

thrombin, for 2 min with 10 lgÆmL)1convulxin or for 5 min with

150 ngÆmL)1TPO (A) Platelets were lysed by the addition of

denat-urating lysis buffer Proteins of whole cell lysate were resolved by 10%

SDS/PAGE and analysed by Western blotting using an

anti-(phospho-specific ERK1-2) Ig (top) The filter was stripped and reprobed using

an anti-ERK2 Ig (bottom) (B) Platelets were lysed by the addition of

RAS lysis buffer Cell extracts were precipitated using GST fusion

protein containing the RAS-binding domain of RAF Precipitated

proteins were resolved by 12.5% SDS/PAGE and analysed by Western

blotting using an anti-RAS Ig (top) Proteins of whole cell lysate were

resolved by 12.5% SDS/PAGE and analysed by Western blotting

using anti-RAS Ig (bottom) Results presented are representative of

three experiments.

Trang 6

Nevertheless, RAS could participate in the regulation of

ERK by potentiating the activation mediated by PKC For

instance, it has been shown that TPO is able to potentiate

ERK activation induced by thrombin [6] The authors

proposed that this could be due to the ability of TPO to

activate the early events of the RAS signalling pathway

However, a recent study reported that inhibitors of

PtdIns3K abolished potentiation of ERK by TPO in

response to thrombin, demonstrating that potentiation is

mediated though the PtdIns3K pathway The authors

proposed a model in which activation of PtdIns3K by

TPO potentiates activation of MEK induced by thrombin,

which in turn potentiates activation of ERK [23] Whether

this set of events involves activation of RAS is not clear

TPO is also able to potentiate aggregation and secretion

induced by thrombin Interestingly, although inhibitors of

PtdIns3K abolished this potentiation, the inhibitor of MEK

had no or only a weak effect, suggesting that the MEK–

ERK cascade is not the main downstream event induced by

PtdIns3K to potentiate these functional responses [23]

All of the known components of the RAS–ERK

signalling pathway (RAS, RAF, MEK and ERK) are

expressed in platelets Furthermore, these proteins can be

activated independently, suggesting that each link is

func-tional [5–7] In addition, in megakaryocytic cell lines and in

primary megakaryocytes, the precursor of platelets, the

RAS–ERK signalling pathway is activated by TPO and is

essential for differentiation [16,25] In the last few years, a

number of other proteins able to regulate the RAS–ERK

pathway have been described This includes scaffolding

proteins, which promote interaction between the links of the

pathway For instance, MP1 can bind MEK and ERK1

supporting ERK1 activation [26], and kinase suppressor of

RAS can bind RAF, MEK and ERK favouring activation

of MEK and ERK1-2 through RAS [27] On the other

hand, the RAS–ERK signalling pathway can be

down-regulated by proteins able to bind to its components For

example, the RAF kinase inhibitor protein can bind RAF

and MEK and thereby prevent their interaction [28,29] A

reduction of the expression of the scaffolding proteins or an

over-expression of proteins responsible for down-regulation

could be an explanation for the inefficiency of RAS to

activate ERK in platelets

RAS–RAF interaction and subsequent regulation of ERK

is not the only pathway regulated by RAS For instance, a

mutated form of RAS that is unable to bind RAF is still

able to induce cytoskeletal rearrangements through

activa-tion of the small G protein RAC [30] and is able to regulate

PtdIns3K [31] Relocalization of RAS from the cytoplasmic

to the cytoskeleton fraction could suggest an involvement

of RAS during cytoskeleton rearrangement of platelets

Our study shows that in platelets RAS is not sufficient by

itself to induce activation of its main downstream target

ERK Platelets appear to be a model with which to study

down-regulation of the RAS–ERK signalling pathway and

other functions of RAS Down-regulation of the RAS–

ERK pathway may be a critical step in the process of

end-stage megakaryocyte differentiation

A C K N O W L E D G E M E N T S

This work was supported by the British Heart Foundation (BHF).

S P W is a BHF Senior Research Fellow.

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