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Tiêu đề Cholecystokinin rapidly stimulates CrkII function in vivo in rat pancreatic acini formation of CrkII–protein complexes
Tác giả Alberto G. Andreolotti, Maria J. Bragado, Jose A. Tapia, Robert T. Jensen, Luis J. Garcia-Marin
Trường học Universidad de Extremadura
Chuyên ngành Biochemistry
Thể loại Scientific report
Năm xuất bản 2003
Thành phố Caceres
Định dạng
Số trang 8
Dung lượng 248,81 KB

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In unstimulated acini, the majority of CrkII was present in the lower band which shows higher electrophoretic mobility... In acini stimulated with 10 nMCCK-8 themajority of CrkII is shif

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Cholecystokinin rapidly stimulates CrkII function in vivo in rat

pancreatic acini

Formation of CrkII–protein complexes

Alberto G Andreolotti1, Maria J Bragado2, Jose A Tapia3, Robert T Jensen3and Luis J Garcia-Marin1

1 Departamento de Fisiologia, Universidad de Extremadura, Caceres, Spain; 2 Departamento de Bioquimica, Biologia Molecular y Genetica, Universidad de Extremadura, Caceres, Spain;3Digestive Diseases Branch, National Institute of Diabetes and Digestive and Kidney Diseases of the National Institutes of Health, Bethesda, MD, USA

Crk belongs to a family of adapter proteins whose structure

allows interaction with tyrosine-phosphorylated proteins

and is therefore an important modulator of downstream

signals, representing a convergence of the actions of

numerous stimuli Recently, it was demonstrated that

chole-cystokinin (CCK) induced tyrosine phosphorylation of

proteins related to fiber stress formation in rat pancreatic

acini Here, we investigated whether CCKreceptor

activa-tion signals through CrkII and forms complexes with

tyro-sine-phosphorylated proteins in rat pancreatic acini We

demonstrated that CCKpromoted the transient formation

of CrkII–paxillin and CrkII–p130Cascomplexes with

maxi-mal effect at 1 min Additionally, CCKdecreased the

elec-trophoretic mobility of CrkII This decrease was time- and concentration-dependent and inversely related with its function Carbachol and bombesin also decreased CrkII electrophoretic mobility, whereas epidermal growth factor, vasoactive intestinal peptide, secretin or pituitary adenylate cyclase-activating polypeptide had no effect CCK-induced CrkII electrophoretic shift was dependent on the Src family

of tyrosine kinases and occurred in the intact animal, sug-gesting a physiological role of CrkII mediating CCKactions

in the exocrine pancreas in vivo

Keywords: Crk; protein complex; CCK; transduction path-ways; pancreatic acini

Cholecystokinin (CCK) is a peptide acting as a hormone/

neurotransmitter that controls several physiological effects

in the gastrointestinal tract [1,2] and in the central nervous

system (CNS) [3,4] Additionally, CCKhas potent growth

effects both in normal tissues, such as pancreas [3], and in

neoplasic tissues, such as stomach and pancreas

adenocar-cinomas [3,5] It has been clearly established that its

physiological effects on the gallbladder, pancreas and

CNS are mediated in part by the CCKAreceptor, a member

of the G-protein-coupled receptor (GPCR) superfamily

[1,2] Intracellular pathways of CCKA receptor activation

have been investigated extensively in pancreatic acini [1,2]

In these cells, we reported recently that CCKstimulates

tyrosine phosphorylation of several proteins related with

fiber stress formation such as the focal adhesion kinase

p125FAK, paxillin [6], p130Cas[7] and PYK2 [8], dissecting

alternative transduction cascades involved in several cellular functions, such as cystoskeleton reorganization [9]

A central role in signal transduction pathways down-stream of different stimuli is played by the adapter protein, Crk A new oncogene identified from a chicken tumor that activated a cellular adapter-type SH2-SH3-containing G-protein led to the name of crk (chicken tumor virus regulator of kinase) [10] The product of the proto-oncogene

in human and mouse, c-Crk, is expressed as two distinct proteins c-CrkI contains one SH2 and one SH3 domain, while c-CrkII has an additional SH3 [11] The SH2 domain of Crk binds to phosphotyrosine-containing proteins such as p130Cas, paxillin or Cbl [10,12] The first SH3 domain (N-terminal) of CrkII binds to guanine nucleotide exchange factors such as C3G, which in turn activate transduction cascades involving small GTP-binding proteins [10,12] Recent investigations reported that CrkII complex formation

is induced by oncogenes such as Bcr-Abl [13], integrins [14], growth factors [15,16] and ligands of G-protein-coupled receptors (such as bombesin [17] or angiotensin II [18]) and thus CrkII represents a convergence of the signal transduc-tion cascades of different stimuli Summarizing these data, the Crk family seems to be involved in different signaling systems including the formation of focal adhesion complexes and actin cytoskeleton regulation, receptor tyrosine kinases signaling pathways and pathogenesis of different leukemias related with the Bcr/Abl tyrosine kinases [10,12]

A peculiar feature of CrkII is that, unlike some other adapter proteins, CrkII itself is tyrosine phosphorylated by tyrosine kinases such as the cytoplasmic c-Abl and the epidermal growth factor (EGF) receptor [19–21] It is

Correspondence to L J Garcia-Marin, Departamento de Fisiologia,

Facultad de Veterinaria, Universidad de Extremadura,

Avda de la Universidad, s/n, 10071 Caceres, Spain.

Fax: + 34 927 257 110, Tel.: + 34 927 257 154,

E-mail: ljgarcia@unex.es

Abbreviations: BAPTA-AM,

1,2-bis(2-aminophenoxy)ethane-N,N,N¢,N¢-tetraacetic acid tetrakis (acetoxymethyl ester); CCK,

cholecystokinin; CNS, central nervous system; crk, chicken tumor

virus regulator of kinase; EGF, epidermal growth factor; GPCR,

G-protein-coupled receptor; PKC, protein kinase C; TPA,

12-O-tetradecanoylphorbol 13-acetate.

(Received 29 August 2003, accepted 6 October 2003)

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binding site for its SH2 domain that inhibits the

inter-molecular interactions mediated by both SH2 and SH3

domains of CrkII [19,20] Thus, changes in CrkII

phos-phorylation state would explain the regulation of CrkII–

protein complex formation Stimuli that induce CrkII

tyrosine phosphorylation include growth factors other than

EGF, such as nerve growth factor and insulin-like growth

factor, sphingosine 1-phosphate [15,16,22,23], the

engage-ment of T-cell receptor or B-cell antigen receptor [24,25]

Although it has been demonstrated that activation of

GPCRs stimulates the formation of CrkII–protein

com-plexes [7,17,18], nothing is known about the effect of a

GPCR activation, such as CCKA, on CrkII signaling and

its subsequent effect on the formation of CrkII–protein

complexes in rat pancreatic acini Thus, in the present work,

we investigated whether in vivo activation of the CCKA

receptor regulates CrkII function to form protein complexes

in rat pancreatic acini, one of its main physiological cell

targets [1,2] We also studied the electrophoretic mobility

shift of CrkII observed after CCKtreatment and its possible

contribution to the regulation of CrkII function Moreover,

we have investigated whether CCKintracellular actions in

the pancreas of the intact animal involved a CrkII signal

Materials and methods

Materials

Male Wistar rats (150–200 g) were obtained from the

Animal Section (Veterinary Resources Branch, NIH,

Bethesda, MD, USA) or from the Veterinary Faculty

(UEX, Spain); purified collagenase (CLSPA) from

Worth-ington Biochemicals (Freehold, NJ, USA);

COOH-ter-minal octapeptide of cholecystokinin (CCK-8) from

Peninsula Laboratories (Belmont, CA, USA); EGF,

thapsigargin, A23187, tyrphostin B44, PP2, PP3 from

Calbiochem;

1,2-bis(2-aminophenoxy)ethane-N,N,N¢,N¢-tetraacetic acid tetrakis (acetoxymethyl ester)

(BAPTA-AM), bombesin, pituitary adenylate cyclase-activating

polypeptide, secretin, vasoactive intestinal peptide,

12-O-tetradecanoylphorbol 13-acetate (TPA) from Bachem AG

(Switzerland); anti-Crk mAb, anti-p130CasmAb,

anti-paxillin mAb, anti-phosphotyrosine mAb (PY20) from

Transduction Laboratories (Lexington, KY, USA) and

vitamin/aminoacid mixture from Sigma

In vivo injection of CCK and preparation of pancreatic

homogenates

Experiments performed using animals were in line with the

Ethical Principles and Guidelines for Scientific Experiments

on Animalsof the Swiss Academy of Medical Sciences Male

Wistar rats weighing 150–200 g and fed a standard diet were

injected with either saline or 15 lgÆkg)1of

CCK(intraperi-toneal) between 09:00 and 11:00 h Rats were killed after

10 min and the pancreas was removed and homogenized

(Polytron homogenizer) in seven volumes of lysis buffer:

50 mMTris/HCl, pH 7.5, 150 mMNaCl, 1% Triton X-100,

1% deoxycholate, 1 mM EGTA, 0.4 mM EDTA,

2.5 lgÆmL)1 aprotinin, 2.5 lgÆmL)1 leupeptin, 1 mM

phenylmethanesulfonyl fluoride, and 0.2 mMNaVO The

the supernatant containing microsomes and soluble proteins was used to analyze the CrkII phosphorylation state Rat pancreatic acini preparation

Dispersed rat pancreatic acini were isolated according to modifications [6] of the procedure published previously [26] Unless otherwise stated, the standard incubation solution contained 25.5 mM Hepes, (pH 7.4), 98 mM NaCl, 6 mM

KCl, 2.5 mM NaH2PO4, 5 mM sodium pyruvate, 5 mM

sodium fumarate, 5 mM sodium glutamate, 11.5 mM glu-cose, 0.5 mM CaCl2, 1 mM MgCl2, 2 mM glutamine, 1% (w/v) albumin, 1% (w/v) trypsin inhibitor 1% (v/v) vitamin mixture and 1% (w/v) amino acid mixture with 100% (v/v)

O2as the gas phase

Immunoprecipitation Pancreatic acini isolated from one rat were preincubated with standard incubation solution for 3 h at 37C Acini were then incubated with agonists at concentrations and times indicated, washed with phosphate buffered saline (NaCl/Pi) with 0.2 mMNa3VO4and sonicated (5 s at 4C)

in lysis buffer Lysates were centrifuged at 10 000 g for

15 min Protein concentration in the supernatant was standardized to 500 lgÆmL)1 and 1 mL was incubated overnight at 4C with anti-phosphotyrosine (PY20) mAb (4 lg) or anti-Crk Ig (6 lg), bridging antibody (4 lg) and

25 lL of protein A-agarose Immunoprecipitates were washed three times with NaCl/Pi and analysed by SDS/ PAGE and Western blotting

Western blotting Proteins in total cellular lysates, immunoprecipitates or pancreatic homogenates were resolved by SDS/PAGE and transferred to nitrocellulose membranes Western blotting was performed as described previously [7,8] using the following primary antibody concentrations: 1 lgÆmL)1 anti-phosphotyrosine (PY20), 0.25 lgÆmL)1 anti-Crk, 0.25 lgÆmL)1anti-p130Casor 0.025 lgÆmL)1anti-paxillin Statistical analyses

All data provided are reported as mean ± SEM Data were analysed using Student’s t-test and only values with

P< 0.05 were accepted as statistically significant

Results

CCK induced CrkII association with p130Casand paxillin

to form protein complexes in rat pancreatic acini

To identify the presence of Crk on rat pancreatic acini, proteins from whole acinar lysates immunoprecipitated with anti-Crk antibody were separated using SDS/PAGE and analysed by Western blotting In acinar lysates (Fig 1A) anti-Crk specific Ig revealed the presence of two bands at the suitable molecular mass of CrkII (40/42 kDa) [23] In unstimulated acini, the majority of CrkII was present in the lower band which shows higher electrophoretic mobility

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(Fig 1A, lane 1) In acini stimulated with 10 nMCCK-8 the

majority of CrkII is shifted to the upper band, showing lower

electrophoretic mobility (lanes 4, 5) These results were

confirmed by immunoprecipitation of acinar proteins with

anti-CrkII Ig followed by Western blotting with the same

antibody (Fig 1B) Two bands with different electrophoretic

mobility were also visualized in these conditions The same

membranes containing anti-CrkII immunoprecipitated

pro-teins were subsequently probed with anti-paxillin Ig (Fig 1C)

to analyze the regulation by CCKof the interaction between

the adapter protein, CrkII and paxillin Data shown in

Fig 1C demonstrated that 10 nMCCK-8 treatment caused a

maximal effect on CrkII–paxillin complex formation at

1 min which decreased rapidly with almost no effect after

5 min of CCK-8 addition (Fig 1C) We have confirmed that

CCKregulates the protein complex formation of CrkII with

other proteins such as p130Cas in rat pancreatic acini

Coimmunoprecipitation studies perfomed in the same

sam-ples as above are shown in Fig 1D and show that treatment

with CCK-8 stimulated the formation of the CrkII–p130Cas

complex with a maximum effect at 1 min that decreased

rapidly (Fig 1D), confirming previous results [7]

CCK-8 induced an electrophoretic mobility shift of CrkII

in a time- and concentration-dependent manner

We next investigated the differences in the electrophoretic

mobility of CrkII observed in Fig 1 CCK-induced CrkII

electrophoretic shift was time-dependent (Fig 2A) with an increase in the upper band detected within 1 min after addition of CCK-8 and a maximum reached within 5 min

Fig 1 Identification of CrkII in rat pancreatic acini (A, B) and

CCK-dependent induction of CrkII function to form CrkII-protein complexes

in vivo (C, D) Rat pancreatic acini were incubated with 10 n M CCK-8

for the indicated times and then lysed Lysates were

immunoprecipi-tated with anti-Crk mAb Resulting immunocomplexes (B) or 10 lg

protein acinar lysates (A) were analysed by SDS/PAGE and Western

blotting with anti-Crk mAb or anti-paxillin mAb (C) or anti-p130Cas

mAb (D) CrkII positions are indicated on the left Results shown are

representative of three independent experiments.

Fig 2 Time-course and concentration-dependence of CCK-8 stimula-tion of CrkII electrophoretic mobility shift Rat pancreatic acini were treated with CCK-8 at concentrations and times indicated and then lysed Cell lysates were analysed by Western blotting using anti-Crk mAb Quantification of bands was performed by scanning densito-metry and is represented in the graphs Results shown are represen-tative of four independent experiments, each one performed in duplicate (A) The upper panel shows a representative experiment with CCK-8 at the indicated times Values shown in the graph are means ± SEM, expressed as the percentage of CrkII upper band with respect to total CrkII (upper and lower band) (B) The upper panel shows a representative experiment where acini were incubated for 2.5 min with indicated CCK-8 concentrations Values are means ± SEM expressed

as the percentage of maximal increase caused by 10 n M CCK-8 above control unstimulated values.

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(65% of total CrkII was shifted to the upper band) The

degree of electrophoretic mobility shift decreased at 40 min

but remained elevated (50% of total CrkII was shifted) The

lower CrkII electrophoretic mobility state induced by

CCK-8 was dose-dependent (Fig 2B) with a half-maximal effect

at 0.1 nM A weak increase was detected after 5 min

incubation with 0.01 nMCCK-8 and the maximum effect

was observed at 100 nMCCK-8

CCK induces the electrophoretic mobility shift of CrkII

in the intact animal

To study whether CCKhas a similar effect in the

electrophoretic mobility of CrkII in vivo, we injected rats

with 15 lgÆkg)1of CCK The injection of CCK reduced the

electrophoretic mobility of CrkII in pancreatic homogenates

(41.8 ± 1.5% of total CrkII was shifted to the upper band)

as shown in Fig 3 This electrophoretic shift effect observed

in the intact rat is comparable to the effect obtained in rat

20 min

Effect of different agonists on the electrophoretic mobility of CrkII in pancreatic acini

Different agonists belonging to the GPCR family [1] were tested to study whether the shift in CrkII electrophoretic mobility also occurred with other stimuli Bombesin and carbachol induced a marked decreased in CrkII electro-phoretic mobility shift (Fig 4, lanes 3, 4), comparable to the effect obtained with CCK-8 (lane 1) The CCK-8 analog, CCK-JMV-180 (1 lM), an agonist at the high-affinity state

of the CCKreceptor and antagonist at the low-affinity state [1], had no effect on CrkII electrophoretic mobility (lane 5)

We also evaluated whether CrkII electrophoretic shift was induced by growth factors EGF had no effect on CrkII electrophoretic mobility (Fig 4, lane 6) We further con-firmed the lack of effect of EGF by incubating pancreatic acini with 10 nMEGF for different times (data not shown) EGF did not modify CrkII mobility at any time point studied We also analysed whether occupation of receptors coupled to an enhancement of intracellular cAMP led

to CrkII electrophoretic shift Neither pituitary adenylate cyclase-activating polypeptide, secretin nor vasoactive intes-tinal peptide affected CrkII electrophoretic shift in pancre-atic acini (Fig 4, lanes 7–9) All these agonists have been demonstrated to have biological effects on pancreatic acinar cells at concentrations similar to the one used by us in this work [1,8,27]

Effect of intracellular calcium on CrkII electrophoretic shift induced by CCK in pancreatic acini

CCKreceptor occupation causes activation of phospho-lipase C (PLC), resulting in the generation of inositol phosphates and diacylglycerol releasing intracellular cal-cium and activation of protein kinase C (PKC), respectively [1,2] To investigate the involvement of calcium in CCK-induced CrkII electrophoretic mobility shift, we preincu-bated pancreatic acini with thapsigargin and BAPTA-AM

in a calcium-free medium (with 5 mM EGTA) before addition of CCK-8 Incubation with each compound alone did not affect the electrophoretic mobility of CrkII (Fig 5, lanes 2, 3 and 4) The calcium-free medium, which decreases calcium influx in response to CCK-8 in pancreatic acini [2,8], significantly decreased the CCK-8-induced CrkII mobility shift by 41.5 ± 2.9% (Fig 5, lane 6 compared with 5) Preincubation with thapsigargin, which totally abolished the CCK-8-stimulated increase of intracellular

Fig 3 Exogenous CCK enhances CrkII electrophoretic mobility shift in

the intact animal Rats were injected with 15 lgÆkg)1of CCK-8 and

10 min later pancreas was removed and homogenized Western

blot-ting analysis of total CrkII after SDS/PAGE was performed and the

electrophoretic mobility shift of CrkII assessed The top panel shows a

representative Western blot and the bottom panel shows means ±

SEM of four independent experiments [expressed as percentage of

CrkII upper band with respect to total CrkII (upper and lower band)].

Duplicate samples were analysed for each rat.

Fig 4 Effect of different stimuli on CrkII electrophoretic mobility shift in rat pancreatic acini Acini were treated 5 min with the indicated concentrations of agonists and lysed CrkII was identified by Western blotting as described Results are representative of three experiments performed in duplicate.

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calcium in pancreatic acini [8], significantly reduced the

CCK-induced CrkII electrophoretic mobility shift by

35.5 ± 4.0% (Fig 5, lane 7 compared with 5) Depletion

of intracellular calcium by preincubation with BAPTA-AM

markedly decreased the CCK-induced mobility shift (by

84 ± 11.6%; Fig 5, lane 8 compared with 5) Direct

activation of PKC by 1 lMTPA or simultaneous treatment

with TPA and calcium ionophores did not modify CrkII

electrophoretic mobility (data not shown)

CrkII electrophoretic mobility shift induced by CCK

involves tyrosine phosphorylation

It is well established that CCKstimulates the tyrosine

phosphorylation of several intracellular proteins in rat

pancreatic acini [2,6–8] It is also known that CrkII can be

phosphorylated on tyrosine [19–25] To investigate whether

CrkII electrophoretic mobility shift induced by CCKwas

related with its tyrosine phosphorylation, we pretreated

pancreatic acini with B44, a general inhibitor of protein

tyrosine kinases Previously, we showed that pretreatment

of these cells with 300 lM B44 for 2 h caused almost a

complete inhibition of CCK-stimulated tyrosine

phosphory-lation [7,8] Pretreatment of acini with this tyrosine kinase

inhibitor prevented the CrkII electrophoretic mobility shift

induced by CCK-8 (Fig 6A, lane 4 compared with 2) where

the majority of CrkII protein from whole acinar cell lysates

remained in the lower band in presence of B44 To check

further whether CrkII was tyrosine phosphorylated in

response to CCK, proteins from the same acinar lysates

were immunoprecipitated with an anti-phosphotyrosine Ig

and analysed by Western blotting using a specific anti-Crk

Ig (Fig 6B) Two bands were visible in untreated acini (lane

1) Treatment with CCK-8 caused an increase in the

intensity of the upper, slower migrating band (lane 2),

showing that it contains the more tyrosine phosphorylated

band of Crk Pretreatment with tyrosine kinase inhibitor

alone increased the intensity of the lower migrating band

(lane 3) and markedly reduced the CCK-8-induced

elec-trophoretic mobility shift to the upper, slower migrating

band resulting in an increase of the lower migrating band

(lane 4) Similar results were observed when antibodies were used in the reverse order, (immunoprecipitation with an Crk Ig followed by Western blotting using an anti-phosphotyrosine Ig (Fig 6C)

Involvement of Src family of tyrosine kinases

on the CCK-induced CrkII electrophoretic mobility shift

We next examined the effect of a specific Src family tyrosine kinase inhibitor, PP2 and its inactive analog, PP3 [28,29] on CrkII electrophoretic mobility shift Pretreatment of pan-creatic acini with 20 lMPP2 (1 h) did not modify unstim-ulated CrkII electrophoretic migration (Fig 7, lane 4), but significantly reduced the CCK-8-induced CrkII electrophoretic mobility shift by 33.5 ± 4.5 and

Fig 5 Calcium dependence of CCK-8 stimu-lation of CrkII electrophoretic mobility shift in pancreatic acini Acini were pretreated 30 min

at 37 C in a calcium-free medium (with EGTA 5 m M ) either in absence or presence of thapsigargin (10 l M ) or BAPTA/AM (50 l M ) Acini were further incubated for 5 min with

no addition or with CCK-8 (10 n M ) CrkII electrophoretic mobility shift was assayed by Western blotting as described Results shown

in the upper panel are representative of four experiments, each one performed in duplicate Results at the bottom panel are means of CrkII upper band ± SEM expressed as a percentage of CrkII maximal electrophoretic mobility shift (obtained with CCKtreatment

in a medium with normal calcium concentra-tion) **P < 0.01.

Fig 6 Phosphotyrosine dependence of the CCK-8 induction of CrkII electrophoretic mobility shift in pancreatic acini Rat pancreatic acini preincubated for 2 h with the tyrosine kinase inhibitor, B44 (300 l M ), were treated for 5 min with no addition (lanes 1, 3) or with 10 n M

CCK-8 (lanes 2, 4) and then lysed Proteins from whole cell lysates were immunoprecipitated with anti-phosphotyrosine (B) or anti-Crk (C) Igs Cell lysates (A) or immunoprecipitates (IP; B and C) were analysed by Western blotting (WB) using anti-Crk mAb (A and B) or anti-phosphotyrosine mAb (C) CrkII positions are indicated on the left Results shown are representative of three independent experi-ments.

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47.0 ± 6.5% at 5 and 40 min of CCK-8 treatment (Fig 7,

lanes 5 and 6), respectively The inactive analog of the

inhibitor of the Src family tyrosine kinase, PP3 (20 lM),

showed no effect on basal nor CCK-stimulated CrkII

electrophoretic mobility shift (Fig 7, lanes 7–9)

Discussion

In this study, we have demonstrated that CCKrapidly

promotes the formation of CrkII–protein complexes,

CrkII–paxillin and CrkII–p130Cas, in rat pancreatic acini

Recently, it has been demonstrated that CCKactivates

different intracellular pathways in rat pancreatic acinar cells

[2] We have demonstrated previously in these cells that

CCKis a potent activator of the tyrosine phosphorylation

of different proteins such as p130Cas [7] and paxillin [6],

creating potential binding sites for the SH2 domain of

CrkII, necessary for the formation of protein complexes

Our results demonstrated that CrkII is present in rat

pancreatic acini as two bands with different electrophoretic

mobility Moreover, we have shown an inverse correlation

between the electrophoretic mobility and the formation of

CrkII protein complexes Concerning the regulation of CrkII

complex formation, it has been proposed that the SH2

domain of CrkII intramolecularly binds to the CrkII

phosphorylated Tyr221 residue and that this association

inhibits the intermolecular interactions mediated by both the

SH2 and SH3 Crk domains [10,19,30] The electrophoretic

mobility shift of CrkII appears to be due to the

phosphory-lation state of the protein; thus, the upper band corresponds

to the more phosphorylated CrkII and the lower band

corresponds to the less phosphorylated state of the CrkII

protein [23] By using two different approaches, our results

demonstrated that CCKinduced both the apparition of a

slower electrophoretic migrating band of CrkII and an

increase in its tyrosine phosphorylation content Under our conditions we can suggest that, at least partially, the CCK-induced electrophoretic mobility shift is correlated with an increase in the phosphorylated tyrosine content of CrkII In this regard, it is well documented that CrkII itself, unlike other adapter proteins, is tyrosine phosphorylated in response to growth factors EGF, nerve growth factor, insulin-like growth factor and also by sphingosin 1-phos-phate [15,16,22,23], engagement of T-cell receptor or B-cell antigen receptor [24,25] Tyrosine kinases, such as the cytoplasmic c-Abl and the EGF receptor, phosphorylate CrkII in tyrosine [19,21] However we cannot rule out other possibilities that would explain the CrkII electrophoretic mobility shift induced by CCKin our study

According to this model of inhibition of CrkII complex formation, regulated by the intramolecular binding of SH2 to phosphorylated Tyr221, there is an established sequence of mechanisms regulating CrkII complex formation where (a) different proteins have to be phosphorylated on tyrosine residues to allow the complex formation with CrkII through the SH2 domain of this adapter protein; (b) CrkII is phosphorylated on Tyr221 to allow (c) the intramolecular SH2 domain bind to it, which results in (d) inhibition of the intermolecular interactions of CrkII mediated by the SH2 domain and (e) subsequent blockade of the downstream CrkII-mediated pathways [30] Based on our results, we propose that a similar sequential model of the regulation of CrkII function by CCKmay occur in rat pancreatic acini: (a) CCKstimulates the rapid tyrosine phosphorylation of proteins such as p130Casand paxillin [6,7]; (b) immediately afterwards, CCKpromotes the rapid formation of CrkII– p130Casand CrkII–paxillin complexes, probably complexing

to the SH2 domain of CrkII (rate is maximal at 1 min and declines after 5 mins; (c) the CrkII electrophoretic mobility shift appears visible within 1 min and is maximal at 5 min

Fig 7 Effect of PP2, a specific inhibitor of Src

family tyrosine kinases, and its inactive analog,

PP3 on the CCK-8 induction of CrkII

elec-trophoretic mobility shift in rat pancreatic acini.

Pancreatic acini were pretreated 2 h at 37 C

in either absence or presence of 20 l M PP2

(lanes 4–6) or 20 l M PP3 (lanes 7–9) Acini

were further incubated 5 or 40 min with 10 n M

CCK-8 and then lysed Results shown are

representative of three experiments in

dupli-cate Results in the lower panel are means ±

SEM of four experiments expressed as a

per-centage of CrkII (upper band) with respect to

total CrkII (upper and lower band).

**P < 0.01.

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incubation with CCK If we suppose that this mobility shift is

at least partially due to the tyrosine phosphorylation of

CrkII, as suggested from this study, then at 5 min, the SH2

domain of CrkII could be intramolecularly bound to

phosphorylated tyrosine resulting in a blockade of any CrkII

protein complex mediated via the SH2 domain In agreement

with this model, we have found that CrkII association with

p130Casor paxillin is almost completely disrupted at 5 min,

which is in concordance with this temporal sequence model of

CrkII functional mechanism Thus, changes in CrkII

phos-phorylation state, visualized by the subsequent

electro-phoretic mobility shift, would explain the CCK-mediated

regulation of CrkII–protein complex formation by a

mech-anism of open-closed configuration similar to that described

for Src family members [12]

Concerning the function of the CrkII protein complexes,

in rat-1 fibroblasts over-expressing human insulin receptor

(HIRc cells), a potential role of CrkII–p130Cas complex

formation (via the SH2 domain of CrkII) has been

suggested in the regulation of mammalian actin

cytoskele-ton [30] Several studies have recently suggested that CrkII

may regulate cytoskeleton organization through activation

of the Rho/Rac family of small GTPases [30]

Electrophoretic mobility shift of CrkII was a rapid

consequence of the stimulation of rat pancreatic acini with

CCKand was dependent on the CCKconcentration At

present, little is known about the intracellular pathways

coupling receptor activation to CrkII, especially in the case

of the GPCRs such as the CCKA receptor It is well

established that the CCKconcentration range that regulates

CrkII also causes activation of CCKAreceptor [1] activating

PLC, resulting in the subsequent PKC activation, inositol

phosphate generation and intracellular calcium release [1,2],

and also activates several transduction pathways such as

p125FAK, PYK2, paxillin and p130Castyrosine

phosphory-lation [6–8]

PKC activation is probably not part of an intracellular

pathway that mediates CCK-stimulated CrkII

electropho-retic mobility in pancreatic acini, as demonstrated by the

lack of effect of TPA or the PKC inhibitor, GF109203X

(data not shown) Moreover, simultaneous PKC and

intracellular calcium stimulation did not affect CrkII

electrophoretic mobility In the present study, we have

demonstrated that intracellular calcium increase by itself did

not cause a change on CrkII electrophoretic migration but

the presence of intracellular calcium did play a permissive

role because its presence was necessary for CCKto

stimulate CrkII mobility shift

In the present study we have found that PP2, a specific

inhibitor of Src family kinases [28,29], produced a significant

inhibition of CCK-stimulated CrkII electrophoretic

mobil-ity shift This effect was specific as pretreatment with PP3,

an inactive analog of PP2 [28,29], had no effect at all on

CrkII migration induced by CCKstimulation Thus, our

results support the conclusion that CCKinduces CrkII

electrophoretic mobility shift by an intracellular pathway

that is at least partially mediated by the Src family of

tyrosine kinases in rat pancreatic acini Src family tyrosine

kinase inhibitors have been demonstrated to abolish CrkII

phosphorylation induced by sphingosine 1-phosphate [31]

This observation reinforces our idea that the electrophoretic

mobility shift of CrkII is related directly with its tyrosine

phosphorylation Various GPCRs, including CCKA [32], activate Src family kinases [33] In addition, v-Src and v-Crk transformed cells display elevated tyrosine phosphorylation

on proteins related with CrkII and focal adhesions, inclu-ding p130Cas, p125FAKand paxillin [10,33]

The CrkII electrophoretic mobility shift was also observed after stimulation with agonists of pancreatic receptors (belonging to the GPCR family) other than CCK(such as bombesin and carbachol) Interestingly, EGF

or agonists of receptors coupled to an increase in cAMP did not change the electrophoretic mobility of CrkII The lack

of effect of EGF is not due to an inefficient dose as we have shown previously in pancreatic acini that 10 nM EGF induced a maximal increase in EFG-receptor, p125FAKand paxillin tyrosine phosphorylation [34]

The physiological importance of CrkII electrophoretic mobility shifts induced by CCKbecame more relevant when

we demonstrated that it occurred in the intact animal Exogenous CCKmarkedly altered CrkII electrophoretic mobility in the intact animal at a dose that has been demonstrated to regulate the initiation phase of protein synthesis in rat pancreas in vivo [35] At present, our results support the idea that CrkII is probably an important intracellular mediator of CCKphysiological actions in vivo, although its role mediating the physiological effects of CCK

in the intact pancreas deserves future research

In summary, results in this study support the conclusion that activation of the G-protein coupled CCKA receptor

in vivoin rat pancreatic acini promotes the function of CrkII, resulting in complex formation (CrkII–paxillin and CrkII– p130Cas) Formation of both CrkII complexes in vivo is dependent on the incubation time with CCKand follows

an opposite kinetic than the electrophoretic mobility shift observed after CCKtreatment CrkII complex formation is maximal when the majority of CrkII is present in the lower band (at 1 min) and is disrupted when the majority of CrkII

is present in the upper slower migrating band (at 5 min) Intracellular calcium probably plays a permissive role in the CCK-induced electrophoretic mobility shift of CrkII, which

is also partially mediated by the Src family of tyrosine kinases The molecular nature of this mobility shift remains unclear but the fact that it occurred in the intact animal reinforces the idea of a relevant physiological role of CrkII in mediating some CCKactions in the exocrine pancreas in vivo

Acknowledgements

We thank Mercedes Go´mez for her technical assistance J.A Tapia was supported by a Postdoctoral Grant from Direccion General de Universidades (MECD), Spain This work was supported by DGICYT grant PB97-0370, and Junta de Extremadura, Consejeria de Sanidad grants 02/10 and 03/63.

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