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Tiêu đề Val216 decides the substrate specificity of a-glucosidase in Saccharomyces cerevisiae
Tác giả Keizo Yamamoto, Akifumi Nakayama, Yuka Yamamoto, Shiro Tabata
Trường học Nara Medical University
Chuyên ngành Biochemistry
Thể loại báo cáo khoa học
Năm xuất bản 2004
Thành phố Japan
Định dạng
Số trang 7
Dung lượng 362,23 KB

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Nội dung

Chimeric enzymes constructed from isomaltase by exchanging with maltase fragments were characterized by their substrate specificities.. When the con-sensus region II, which is one of the

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Val216 decides the substrate specificity of a-glucosidase

Keizo Yamamoto1, Akifumi Nakayama2, Yuka Yamamoto1,* and Shiro Tabata1

1

Department of Chemistry, Nara Medical University, Japan;2Nara Prefectural Institute for Hygiene and Environment, Japan

Differences in the substrate specificity of a-glucosidases

should be due to the differences in the substrate binding and

the catalytic domains of the enzymes To elucidate such

differences of enzymes hydrolyzing a-1,4- and

a-1,6-glu-cosidic linkages, two a-glucosidases, maltase and isomaltase,

from Saccharomyces cerevisiae were cloned and analyzed

The cloned yeast isomaltase and maltase consisted of 589

and 584 amino acid residues, respectively There was 72.1%

sequence identity with 165 amino acid alterations between

the two a-glucosidases These two a-glucosidase genes

were subcloned into the pKP1500 expression vector and

expressed in Escherichia coli The purified a-glucosidases

showed the same substrate specificities as those of their

parent native glucosidases Chimeric enzymes constructed

from isomaltase by exchanging with maltase fragments were

characterized by their substrate specificities When the

con-sensus region II, which is one of the four regions conserved in family 13 (a-amylase family), is replaced with the maltase type, the chimeric enzymes alter to hydrolyze maltose Three amino acid residues in consensus region II were different in the two a-glucosidases Thus, we modified Val216, Gly217, and Ser218 of isomaltase to the maltase-type amino acids by site-directed mutagenesis The Val216 mutant was altered

to hydrolyze both maltose and isomaltose but neither the Gly217 nor the Ser218 mutant changed their substrate specificity, indicating that Val216 is an important residue discriminating the a-1,4- and 1,6-glucosidic linkages of substrates

Keywords: family 13; a-glucosidase; Saccharomyces cere-visiae; site-directed mutagenesis; substrate specificity

Glucosyl hydrolases (EC 3.2.1.-) are key enzymes of

carbohydrate metabolism that were found in the three

major kingdoms, and are categorized into 57 structural

families [1,2] Family 13 (a-amylase family) includes

enzymes such as a-amylase, a-glucosidase, pullulanase,

cyclodextrin glucanotransferase, and 1,4-a-D-glucan

branching enzyme, specifically acting on a-1,4- and

a-1,6-O-glucosidic linkages [1] Many primary structures

of the members of family 13 from various origins are now

available, and have been compared to each other The

existence of four highly conserved regions (regions I–IV)

and three acidic residues located in the conserved regions as

catalytic residues has been reported [3–7] Furthermore,

computing secondary structure analysis indicated that

specific structural features of the catalytic (b/a)8-barrel

domain exist in these enzymes [8–10]

The relationship of sequence and structure to substrate

specificity in family 13 enzymes, particularly a-amylase,

cyclomaltodextrinase, and neopullulanase, has been well

studied [11–13] Despite the fact that many a-glucosidases with diverse substrate specificities have been purified and cloned from mammals, plants, and microorganisms, it is still not clear which amino acid residues of a-glucosidase recognize the difference between a-1,4- and a-1,6-glucosidic bonds contained in saccharides

Yeast contains two a-glucosidases, a-1,4-glucosidase (E.C 3.2.1.20, maltase) and oligo-1,6-glucosidase (E.C 3.2.1.10, isomaltase), which act preferentially on maltose or isomaltose and methyl a-D-glucopyranoside (a-mg), respectively The expression of these enzymes is controlled by different polymeric genes, MAL or MGL, separately [14–16] Maltase (the MAL6 product of Saccharomyces carlsbergensis) preferentially hydrolyzed maltose but neither isomaltose nor a-mg, whereas isomaltase hydrolyzes isomaltose and a-mg but not maltose [17,18] Thus, we focused on the structure–function relationship of the two a-glucosidases from Saccharomyces as a model in respect of the difference in their substrate specificities The yeast genome directory which was constructed by Goffeau et al revealed the existence of many homologous open reading frames of a-glucosidase [19] The complete nucleotide sequence of the MAL gene of Saccharomyces has been determined [20], whereas it is not clear which open reading frame corresponds to the MGL gene

In this study, we cloned the genes encoding isomaltase and maltase by means of a RT-PCR method and expressed them in Escherichia coli Subsequently, from a comparison

of the primary structures of the two a-glucosidases, chimeric enzymes were constructed by exchange parts of maltase and isomaltase genes including any one of the four conserved

Correspondence to K Yamamoto, Department of Chemistry, Nara

Medical University, Shijo, Kashihara, Nara 634–8521, Japan.

Fax/Tel.: +81 744 29 8810, E-mail: kama@naramed-u.ac.jp

Abbreviations: a-mg, methyl a- D -glucopyranoside; a-pNPG,

p-nitro-phenyl a- D -glucopyranoside.

Enzymes: a-1,4-glucosidase (maltase) (E.C 3.2.1.20);

oligo-1,6-glucosidase (isomaltase) (E.C 3.2.1.10).

*Present address: Department of General Medicine, Nara Medical

University, Japan.

(Received 2 April 2004, revised 17 June 2004, accepted 5 July 2004)

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regions for family 13 members In addition, we constructed

mutants of isomaltase by replacing three amino acid

residues after Asp215 in consensus region II with residues

of the maltase type using site-directed mutagenesis The

substrate specificities of all mutant enzymes were examined

We found that one amino acid residue in consensus region

II decided the substrate specificity of isomaltase

Materials and methods

Materials

The yeast strains used were Saccharomyces cerevisiae

D-346 (ATCC 56960) and 727–14C (ATCC 56959) The

bacterial strains and plasmids used were Escherichia coli

JM109, KP3998 [21], pUC18 and pKP1500 [21]

Hydroxyapatite (Gigapite) was purchased from

Seika-gaku Kogyo and hydroxyapatite (Micro-Prep Ceramic

Hydroxyapatite, type I) was from Bio-Rad Maltose,

isomaltose, a-mg, and p-nitrophenyl a-D-glucopyranoside

were from Nakalai Tesque, Japan A site-directed

muta-genesis kit (QuickchangeTM) was obtained from Stratagene

and the bicinchoninic acid protein assay reagent was from

Pierce Chemicals La-Taq polymerase was purchased from

Takara Syuzo and restriction endonucleases and T4 DNA

ligase were from Takara Syuzo, or New England Biolabs

Reverse transcriptase was used from the ExpandTM

Reverse Transcriptase kit from Boehringer Mannheim

The Marathon kit was purchased from Clontech

Labor-atory Oligonucleotides were synthesized by Takara Syuzo

Custom Service

Assay method for enzyme activity a-glucosidase activity

was determined by measuring the release of p-nitrophenol

from p-nitrophenyl a-D-glucopyranoside (a-pNPG)

accord-ing to the method described previously [22] When maltose,

isomaltose, and methyl a-D-glucopyranoside (a-mg) were

used as substrates, the enzyme activity was determined as

the rate of hydrolysis of the substrate by measuring the

release of glucose according to the enzymatic method of

NADP+reduction using hexokinase and

glucose-6-phos-phate dehydrogenase [23]

Cloning of the isomaltase gene fromS cerevisiae

The production of maltase and isomaltase of S cerevisiae

was induced by adding maltose and a-mg to the culture

medium, respectively [22] In the case of the cloning of the

isomaltase gene, total RNA was prepared from S cerevisiae

D-346 grown on a medium including 3% (w/v) a-mg by the

method of Chomczynski & Sacchi [24] The mRNA was

purified from the total RNA using Oligotex-dT 30 (Super)

(Takara Syuzo) according to the manufacturer’s

instruc-tions Double-stranded cDNA was constructed from

poly(A) RNA with the oligo-dT primer using the ExpandTM

Reverse Transcriptase kit The N-terminal amino acid

sequence, TISSAHPETEPK, which was determined from

purified yeast isomaltase, matched the ORF YGR287c on

chromosome VII of S cerevisiae [19] Therefore, the

iso-maltase gene was amplified from the cDNA library by PCR

using the N-terminal sequence of ORF YGR287c and

oligo-dT as primers The 1.8 kb RT-PCR product was ligated to

plasmid pUC 18 after digestion with SmaI and introduced

into E coli JM109 The insert was sequenced by the dideoxy method [25] using the Dye Terminator Cycle Sequencing FS Ready Reaction kit (Applied Biosystems) To verify the 5¢ end sequence, 5¢ RACE was performed using the Marathon kit with the AP1 primer and a gene-specific primer (5¢-AGATTGCCTTTCTACAGTCTTCATTC-3¢) accord-ing to the manufacturer’s protocol The 5¢-RACE product was sequenced by a direct sequencing method

Subcloning into the pKP1500 expression vector Forward and reverse primers were designed based on the 5¢- and 3¢-terminal nucleotide sequences of the isomaltase gene (MGL) for cloning into plasmid pKP1500 The forward primer 5¢-ATGACTATTTCTTCTGCACAT CCAGAGACAGAAC-3¢ contains the initiation codon, while the reverse primer 5¢-CTTTCTGCAGACTCA TTCGCTGATATATATTC-3¢ linked a PstI restriction site

to the termination codon PCR was carried out on the isomaltase gene cloned above PCR products were digested with PstI Simultaneously, pKP1500 was digested with EcoRI and PstI, and then the EcoRI site was blunted by the use of a Blunting kit (Takara Syuzo) The vector and the insert MGL gene were ligated with T4 ligase followed by transformation into E coli JM109 The cells were plated on Luria–Bertani agar supplemented with 40 lgÆmL)1 5-bromo-4-chloro-3-indolyl-a-D-glucopyranoside (Boehrin-ger Mannheim), 50 lgÆmL)1ampicillin, and 1 mM isopro-pyl thio-b-D-galactoside and then one day later several blue colonies appeared One of the clones expressing isomaltase was selected The plasmid containing the isomaltose gene was designated pYIM

Cloning of the maltase gene fromS cerevisiae For cloning of the maltase gene, S cerevisiae 727–14C was grown in medium containing 3% (w/v) maltose The mRNA and cDNA were prepared using the same procedure

as described above

The gene-specific primers were synthesized based on the information of Hong & Marmur [20] The reverse primer was modified by introducing a HindIII site seven bases down-stream from the stop codon PCR with La-Taq polymerase was carried out on the cDNA prepared from S cerevisiae 727–14C The 1.8 kb PCR fragment was digested with HindIII Plasmid pKP1500 was digested with EcoRI and HindIII, and then the EcoRI site was blunted by the use of a Blunting kit (Takara Syuzo) The fragment was inserted into the pKP1500 vector and the resulting plasmid was intro-duced into E coli KP3998 Several transformants containing the 1.8 kb insert were selected and sequenced The plasmid carrying the maltase gene was designated pYMA

Expression of recombinant enzymes inE coli and purification of the enzymes

The E coli transformant carrying pYIM (or pYMA) was inoculated into PYG medium [21] supplemented with

50 lgÆmL)1of ampicillin and incubated at 37C Isopropyl thio-b-D-galactoside (final 1 mM) was added when cell density at A660 reached 0.5 and the culture was further incubated for 12 h

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Cells were resuspended in 50 mM Tris/HCl buffer

(pH 7.5) and sonicated The cell-free extract was applied

to a QAE-Toyopearl column equilibrated with 50 mMTris/

HCl (pH 7.5) and the column was washed with the same

buffer containing 20 mMNaCl The enzyme was eluted with

a linear gradient of NaCl (20–150 mM) in the same buffer

Active fractions were pooled and applied to a column of

Gigapite equilibrated with 20 mMsodium phosphate buffer

(pH 7.0) The enzyme was eluted with a linear gradient

of sodium phosphate buffer up to 150 mM The active

fractions were collected and dialyzed against 40 mMsodium

phosphate buffer (pH 6.8), then subjected to

chromato-graphy on hydroxyapatite (Micro-Prep Ceramic

Hydroxy-apatite type I) The purified enzyme was eluted at 250 mM

phosphate buffer (pH 6.8) by a linear gradient of

40–320 mMphosphate

Construction of chimeric enzymes from recombinant

maltase and isomaltase

Chimeric enzymes were constructed by exchanging

nucleo-tide fragments between the maltase and isomaltase genes at

a single restriction site on the plasmid or by inserting a

fragment which was introduced at a unique restriction site

by PCR

Chimeric enzymes MAa/IMb and IMa/MAb were

con-structed by exchanging two MunI/BglII fragments of pYIM

and pYMA which were cleaved at single restriction sites

with both of these restriction enzymes The chimeric

enzyme, Mun/Bpu was constructed by inserting a fragment,

which was amplified by PCR with the forward

pri-mer 5¢-AGAAGCCATTGCTGAGCAATTTTTGTTC-3¢

(underlining indicates the Bpu1102I restriction site) and the

reverse primer 5¢-AAAAAGCTTGCACTAATTTTATTT

GAC-3¢ (underlining indicates the HindIII restriction site and

stop codon, respectively) and pYMA as a template, into IMa/

MAb at Bpu1102I/HindIII Other chimeric enzymes, Mun/

Bst, Mun/Pst, and Pst/Bst were constructed by the same

method described for the Mun/Bpu chimera The chimeric

enzymes are shown in a schematic diagram in Fig 2

Site-directed mutagenesis

Site-directed mutagenesis (Asp215fi Ala,Val216 fi Thr,

Gly217fi Ala, and Ser218 fi Gly of isomaltase) was

carried out by the use of the Quick ChangeTMSite-Directed

Mutagenesis kit and DNA from pYIM as a template and

two additional mutagenic oligonucleotide primers for each

amino acid substitution according to the instruction

man-ual The sites to which the mutation was introduced were

sequenced to confirm that only the expected mutation had

occurred

Results and Discussion

Cloning of yeast a-glucosidases

Two a-glucosidase genes, encoding isomaltase and maltase,

were isolated from an S cerevisiae cDNA library using the

PCR technique In the case of isomaltase, the N-terminal

amino acid sequence, TISSAHPETEPK, matched ORF

YGR287c on chromosome VII of S cerevisiae [19]

More-over, six peptides, including the N-terminal amino acid sequence (TISSAHPETEPK, GSAWTFDEK, NGPRI

PWEGR) obtained from the native isomaltase were in accord with their nucleotide sequences of the ORF Based on this information, a 1.8 kb fragment was amplified from the cDNA library by PCR using 5¢-sequence of the ORF and oligo dT as primers, and was inserted into pUC18 Sequen-cing of the 1.8 kb insert revealed an open reading frame of

1770 bp including a stop codon, TGA The 589 amino acid protein deduced from the ORF was completely identical to the amino acid sequence deduced from ORF YGR287c The sequence data for isomaltase is available from the DNA Data Bank of Japan with accession number AB109221

The entire coding region of the insert was amplified by PCR and subcloned into the pKP1500 expression vector, and the resulting plasmid was introduced into E coli JM109 Expression of the gene was screened by a plate assay using 5-bromo-4-chloro-3-indolyl-a-D -glucopyrano-side Several blue colonies were found to hydrolyze a-pNPG The expression of isomaltase in these clones was confirmed by their ability to hydrolyze isomaltose and a-mg but not maltose The plasmid containing the isomaltase gene was designated pYIM

The maltase gene was also isolated from the DNA library

of S cerevisiae by PCR using gene specific primers The amplified 1.8 kb fragment was inserted into plasmid pKP1500 and the resulting plasmid was transformed into

E coli KP3998 DNA sequence analysis of the fragment gave 100% identity to the MAL6 gene [15] The plasmid containing the maltase gene was designated pYMA Figure 1 shows a comparison of amino acid sequences between maltase and isomaltase There is 72.1% of sequence identity with 165 amino acid alterations

Assessment of recombinant enzymes in comparison with native a-glucosidases

We assessed the two recombinant a-glucosidases in terms of substrate specificity and immunological identity and com-pared them to their native enzymes The two recombinant a-glucosidases showed the same substrate specificities as those of their parent glucosidases, namely, maltase hydro-lyzed maltose but not isomaltose and a-mg, whereas isomaltase hydrolyzed isomaltose and a-mg but not malt-ose Upon double immunodiffusion, rabbit antiserum against native isomaltase produced a single precipitation line without spurs with recombinant isomaltase (data not shown) When the two recombinant enzymes reacted with antisera against native maltase and isomaltase, the recom-binant enzymes showed the same dose–response as the native enzymes by antiserum neutralization (data not shown) These results indicate that the two recombinant a-glucosidases are identical to their parent enzymes Substrate specificities of chimeric enzymes The comparison of the primary structures of the members

of family 13 from various origins has revealed the existence

of four highly conserved regions I, II, III, and IV [3–7] Thus, for the design of chimeric a-glucosidases, the a-glucosidase genes in the two plasmids, pYMA and pYIM,

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were divided into five portions taking into account the four

consensus regions Figure 2 is a schematic representation of

a number of the chimeric enzymes Chimeric enzymes were

characterized based on substrate specificities for maltase,

isomaltase, a-mg, sucrose, and a-pNPG, and the Km for

a-pNPG MAa/IMb and IMa/MAb were constructed by a

recombination of the N-terminal fragment containing

consensus region I of isomaltase and maltase, respectively

The recombination had no effect on either the substrate

specificities or the Kmfor a-pNPG (Table 1) In the Mun/

Bam chimera, the amino acids from 488 to the C-terminus

of IMa/MAb were substituted by the corresponding amino

acids of maltase (residues 485–584) The substitution of the

C-terminal fragment of IMa/MAb also had no effect on the

substrate specificities We further dissected the C-terminal

region of IMa/MAb by preparing chimeras with

switch-over points at residues 332 and 231 (Mun/Bpu and Mun/

Bst, respectively) The specific activity for isomaltose of

Mun/Bpu and Mun/Bst were about 10 and 80 times lower

than that of isomaltase, respectively The Kmfor a-pNPG of

Mun/Bpu was the same as that of isomaltase, whereas the

Kmfor a-pNPG of Mun/Bst was about 50 times lower than

that of isomaltase Thus, fragments including consensus

regions III and IV may affect the substrate affinity of the

a-glucosidases To investigate the role of the fragment

containing consensus region II, two chimeras, Mun/Pst and

Pst/Bst, were constructed In the Mun/Pst chimera, a 27

amino acid fragment of Mun/Bst including consensus

Fig 1 Comparison of amino acid sequences

between maltase and isomaltase Identical and

similar amino acid residues are designated by

* and Æ, respectively Four highly conserved

regions of family 13 are underlined.

Fig 2 Schematic diagram of the chimeric enzymes Isomaltase se-quence is represented as an open bar and maltase sese-quence is repre-sented as a shaded bar MunI, PstI, BstBI, and Bpu1102I are restriction sites used for the construction of chimeric enzymes I, II, III, and IV indicate the location of four highly conserved regions of family 13.

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region II was replaced by the corresponding fragment of

pYMA The substrate specificities of Mun/Pst changed

completely to those of maltase type However, the

charac-teristics of Pst/Bst which contained only the 27 amino acid

fragment of pYIM in pYMA were the same as those of

Mun/Bst Therefore, these results indicate that the fragment

including consensus region II contributes to the

determin-ation of the substrate specificity of a-glucosidase

Site-directed mutagenesis

There were six amino acid differences between the two

a-glucosidases in the fragment including consensus region

II Three out of the six alterations were similar, thus, we

targeted the other three amino acid residues in consensus

region II for site-directed mutagenesis The Val216, Gly217,

and Ser218 in consensus region II of isomaltase were

substituted to the corresponding amino acid residues of

maltase, Thr, Ala, and Gly, respectively The mutant

enzymes G217A and S218G did not exhibit different

substrate specificity to that of isomaltase but their Kmfor

a-pNPG tended toward maltase (Table 2) Mutant V216T

could hydrolyze the a-1,4-glucosidic linkage retaining the isomaltase type substrate specificity and its hydrolyzing ratio of maltose/isomaltose was 1 : 1 As shown in Table 2, doubly and triply mutated enzymes including V216T (V216T/G217A, V216T/S218G, and V216T/G217A/

Table 1 Substrate specificities of the chimeric enzymes The enzyme was incubated with 0.5 M substrate in 100 lL of 0.1 M sodium phosphate buffer,

pH 7.0 at 30 C for 5 min The reaction was stopped by addition of 100 lL of 0.5 M Tris/HCl buffer, pH 7.5, then released glucose was assayed For a-pNPG, an increase of absorbance at 410 nm was measured in 5 m M a-pNPG in 0.1 M sodium phosphate buffer, pH 7.0 at 30 C.

Enzyme

Specific activity (lmolÆmin)1Æmg)1enzyme)

K m for a-pNPG (m M )

Table 2 Kinetic parameters of wild-type isomaltase and site-directed

mutants The consensus region II of isomaltase was mutated to the

maltase type by site-directed mutagenesis For example, V216T was

made by exchanging Val216 of isomaltase with Thr of maltase.

Enzyme

Specific activity (lmolÆmin)1Æmg)1

a-pNPG (m M ) Maltose Isomaltose

V216T/G217A/S218G 6.18 0.57 0.49

Fig 3 Sequence alignment of a-glucosidases of known substrate spe-cificity in the consensus region II Asp residue of the catalytic nucleo-phile is labeled with an arrow and the next residue is highlighted in bold Shown are: Sce D-346, S cerevisiae isomaltase (this study); Bth,

B thermoglucosidasius oligo-1,6-glucosidase [27]; Bce, B cereus suc-rase-isomaltase [28]; Bco, B coagulans sucsuc-rase-isomaltase [29]; Bsp1, Bacillus sp DG0303 a-glucosidase [30], Bsp2, Basillus sp F5 sucrase-isomaltase [31]; Bfl, B flavocaldarius oligo-1,6-glucosidase [32]; Spn, Streptococcus pneumoniae a-1,6-glucosidase [33]; Bsu, B subtilis suc-rase-isomaltase-maltase [34]; Bsp3, Bacillus sp a-glucosidase [35], Tcu, Thermomonospora curvata a-glucosidase [36]; Sce727–14C, S cerevis-iae maltase (this study); Sca, S carlsbergensis maltase [20]; Cal,

C albicans maltase [37]; Hpo, Hansenula polymorpha maltase [38].

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S218G) exhibited a change in the hydrolyzing ratio of

maltose/isomaltose to 5 : 1, 3 : 1, and 10 : 1, respectively

These facts indicate that the three residues in consensus

region II, particularly Val, plays an important role in

distinguishing between the a-glucosidic linkages of a-1,4

and a-1,6

McCarter and Withers [26] indicated that Asp214 on

the consensus region II of maltase is the catalytic

nucleophile Because the Asp214 of maltase is equivalent

to the Asp215 of isomaltase, a mutant with the residue

altered to Ala was tested for its activity on a-pNPG

None of the mutants including D215A had activity on

a-pNPG and a-mg although the proteins were detected

with antiserum against isomaltase by immunoblotting

(data not shown) Thus, the Asp215 of isomaltase is one

of three active acidic residues which are completely

conserved in a-glucosidase group

Amino acid sequence alignment

Figure 3 shows the amino acid sequence alignment of the

consensus region II of a-glucosidases of known substrate

specificity In the case of a-glucosidases hydrolyzing the

a-1,6-glucosidic linkage, the amino acid residue following

the catalytic nucleophile is Val On the other hand, the

corresponding residue of a-glucosidases which acting on

the a-1,4-glucosidic linkage but does not a-1,6-linkage is

Thr X-ray crystallographic analysis of B cereus

oligo-1,6-glucosidase revealed that Val200 following the

cata-lytic nucleophile Asp199 locates on the long loop region

followed by Nb4, and the side chain of Val200 faces

toward the inside of the catalytic cleft [39] Figure 4 shows

the hypothetical structure of the active site of S cerevisiae

isomaltase in complex with isomaltose or maltose using

the crystal structure of B cereus oligo-1,6-glucosidase [39]

as the starting model In the case of wild-type isomaltase,

isomaltose fit to the active site, whereas maltose cannot

bind to the active site because the side chain of Val216

interfere with binding of a 4-linked glucose The CG1 of

Val216 is too close to the O3¢ of maltose On the other

hand, both isomaltose and maltose can bind to the V216T mutant because the steric hindrance between OG1 of Thr216 and O3¢ of maltose is canceled by the rotation of the side chain of Thr216 The results indicate that the amino acid residue just after the catalytic nucleophile in consensus region II must be involved in the recognition of a-glucosidic linkages

In conclusion, this work was successful in identifying the region and residue important in the determination of the substrate specificity of a-glucosidases The identification of V216T and doubly and triply mutated enzymes altered in substrate specificity will serve as a basis for progress toward further understanding the structure-function relationship of family 13 a-glucosidases

References

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Fig 4 Hypothetical model structure of the active site of isomaltase in complex with isomaltose or maltose (A) Wild type (B) V216T mutant The models were constructed by the use of the program HOMOLOGY from the Insight II (Accelrys Inc., San Diego, CA, USA) The crystal structure of

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