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Tiêu đề Therapeutic approaches for prion and Alzheimer’s diseases
Tác giả Thomas Wisniewski, Einar M. Sigurdsson
Trường học New York University School of Medicine
Chuyên ngành Neurology, Pathology, Psychiatry
Thể loại Minireview
Năm xuất bản 2007
Thành phố New York
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The basic pathomechanism in both disorders is related to a conformational change of normally expressed proteins: amyloid-b Ab in AD and the prion protein PrP in Keywords Alzheimer’s dise

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Therapeutic approaches for prion and Alzheimer’s diseases Thomas Wisniewski1,2,3and Einar M Sigurdsson2,3

1 Department of Neurology, New York University School of Medicine, NY, USA

2 Department of Pathology, New York University School of Medicine, NY, USA

3 Department of Psychiatry, New York University School of Medicine, NY, USA

Introduction

Alzheimer’s disease (AD) and prion disease belong to

a category of conformational disorders showing

sub-stantial overlap in pathologic mechanism [1–3] The basic pathomechanism in both disorders is related to a conformational change of normally expressed proteins: amyloid-b (Ab) in AD and the prion protein (PrP) in

Keywords

Alzheimer’s disease; metals; mucosal

vaccination; prion; vaccine

Correspondence

T Wisniewski, New York University School

of Medicine, Departments of Neurology,

Psychiatry and Pathology, Millhauser

Laboratories, Room HN419, 560 First

Avenue, New York, NY 10016, USA

Fax: +1 212 263 7528

Tel: +1 212 263 7993

E-mail: thomas.wisniewski@med.nyu.edu

(Received 9 March 2007, revised 3 May

2007, accepted 4 May 2007)

doi:10.1111/j.1742-4658.2007.05919.x

Alzheimer’s and prion diseases belong to a category of conformational neu-rodegenerative disorders [Prusiner SB (2001) N Eng J Med 344, 1516–1526; Sadowski M & Wisniewski T (2007) Curr Pharm Des 13, 1943–1954; Beekes M (2007) FEBS J 274, 575] Treatments capable of arresting or at least effectively modifying the course of disease do not yet exist for either one of these diseases Alzheimer’s disease is the major cause of dementia in the elderly and has become an ever greater problem with the aging of Western societies Unlike Alzheimer’s disease, prion diseases are relatively rare Each year only approximately 300 people in the USA and approxi-mately 100 people in the UK succumb to various forms of prion diseases [Beekes M (2007) FEBS J 274, 575; Sigurdsson EM & Wisniewski T (2005) Exp Rev Vaccines 4, 607–610] Nevertheless, these disorders have received great scientific and public interest due to the fact that they can be transmis-sible among humans and in certain conditions from animals to humans The emergence of variant Creutzfeld–Jakob disease demonstrated the trans-missibility of the bovine spongiform encephalopathy to humans [Beekes M (2007) FEBS J 274, 575] Therefore, the spread of bovine spongiform encephalopathy across Europe and the recently identified cases in North America have put a large human population at risk of prion infection It is estimated that at least several thousand Britons are asymptomatic carriers

of prion infections and may develop variant Creutzfeld–Jakob disease in the future [Hilton DA (2006) J Pathol 208, 134–141] This delayed emer-gence of human cases following the near elimination of bovine spongiform encephalopathy in the UK may occur because prion disease have a very prolonged incubation period, ranging from months to decades, which depends on the amount of inoculum, the route of infection and the genetic predisposition of the infected subject [Hilton DA (2006) J Pathol 208, 134– 141] Therefore, there is a great need for effective therapies for both Alzhei-mer’s disease and prion diseases

Abbreviations

ACT, a1-antichymotrypsin; AD, Alzheimer’s disease; Ab, amyloid-b; apoE, apolipoprotein E; BBB, blood–brain barrier; BSE, bovine

spongiform encephalopathy; CAA, congophilic amyloid angiopathy; CNS, central nervous system; CWD, chronic wasting disease;

DC, dendritic cell; GSSS, Gerstmann–Stra¨usler–Scheinker syndrome; PrP, prion protein; sAb, soluble Ab; sCJD, sporadic CJD;

Tg, transgenic; vCJD, variant Creutzfeld–Jakob disease.

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prion disease (Fig 1) [4,5] This occurs without an

alteration in the amino-acid sequence of the proteins

Ab is a 40–43 amino acid peptide, which, in AD,

self-assembles into toxic oligomers and fibrils that

accumu-late in the brain, forming plaques and deposits in the

walls of meningocephalic vessels [6,7] The same

pep-tide can be detected in most physiological fluids, such

as serum or cerebrospinal fluid, where it is called

sol-uble Ab (sAb) [7] PrPC (C-cellular) is a 209 amino

acid, cell membrane anchored protein expressed at

highest levels by neurons and follicular dendritic cells

of the immune system In the setting of prion disease,

this protein undergoes a transformation to toxic PrPSc

(Sc-scrapie) [8–10] Fibrillar Ab and PrPSchave a high

b-sheet content which renders them insoluble, resistant

to proteolytic degradation and toxic to neurons

Neu-rological symptoms in AD and prion disease are

directly related to loss of neurons and synaptic

connec-tions Oligomeric and fibrillar Ab can be directly

neurotoxic and⁄ or can promote formation of

neuro-fibrillary tangles [7] Both fibrillar Ab and PrPSc are

capable of forming amyloid deposits The presence of

amyloid deposits is necessary for making the diagnosis

of AD [11,12] Abundant amyloid deposits composed

of PrPSc (full length or fragments) are a neuropatho-logical hallmark of variant Creutzfeld–Jakob disease (vCJD), Gerstmann–Stra¨usler–Scheinker syndrome (GSS), and kuru [13] They are also present in 10% of sporadic CJD (sCJD) cases [9]

A number of proteins may actively promote the con-formational transformation of these disease specific pro-teins and stabilize their abnormal structure Examples

of such proteins in AD include apolipoprotein E (apoE), especially its E4 isoform [13,14], a1-antichymotrypsin (ACT) [15] or C1q complement factor [16,17] (Fig 1)

In their presence, the formation of Ab fibrils in a solution of sAb is much more efficient [13,15] These

‘pathological chaperone’ proteins have been found histologically and biochemically in association with fibrillar Ab deposits [18] but not in preamyloid aggre-gates, which are not associated with neuronal loss [19] Similarly, in prion disease, extensive data points toward the existence of an unidentified protein X actively involved in the conversion of PrPCinto PrPSc[20]

AD and prion diseases exist as sporadic and inher-ited illnesses In addition, prion disease can be trans-mitted from one subject to another In experimental model settings, some evidence also exists for the infec-tivity of AD [21,22] An important event in the patho-mechanism of AD is thought to be reaching a critical concentration of sAb and⁄ or chaperone proteins in the brain, at which point the conformational change occurs [23] This leads to the formation of Ab aggre-gates, initiating a neurodegenerative cascade In sporadic AD, this occurs due to an age-associated overproduction of Ab, impaired clearance from the brain, and⁄ or influx into the central nervous system (CNS) of sAb circulating in the serum [24] Inherited forms of AD are associated with various genetic defects, resulting in overproduction of total sAb, or more fibrillogenic Ab 1–42 species [25]

Sporadic prionoses like sCJD are thought to result from the spontaneous conversion of PrPC into PrPSc [26] The mechanisms that stabilize PrPCstructure are largely unknown but, once PrPSc assumes its patholo-gical conformation, it can bind to PrPC and induce a conformation change This starts a self-perpetuating vicious cycle allowing PrPScto replicate without DNA, using the host cell’s PrPC as a template [9,26] Most inherited prionoses such as GSS or inherited forms of CJD are the result of a point mutation in PrPC that increases the propensity for it to assume an abnormal conformation Virtually all genetic defects implicated

in familial forms of AD and prionoses are inherited in

an autosomal dominant fashion Unlike AD, prionoses can be easily transmitted between subjects of the same

Protofibrils Fibrils Increased

Aggregated

Toxic

CONFORMATIONAL DISORDERS

Mainly

Random Coil

Monomers

Non-Toxic

Alzheimer’s Disease

A β Plaque Neurofibrillary

Tangle

Prionoses

Neuronal loss Spongiform changes

Pathological Chaperones

Metals

Fig 1 Conversion of sAb peptide or PrP C to their pathological

b-sheet conformers is a key step in the pathogenesis of AD and

pri-onoses, respectively In AD, these b-sheet rich structures consist

of oligomers, protofibrils and fibrils that form plaques within the

brain parenchyma or deposit in the cerebrovasculature A

compar-able entity in prion diseases consists of the proteinase K resistant

scrapie form of the prion protein (PrP Sc ) that, in certain prion

dis-eases, fibrillizes and deposits as plaques within the brain This

pro-cess is facilitated by various pathological chaperones as well as

several metals The aim of most therapeutic interventions for these

conformational disorders is to reduce the amount of the substrate

(sAb, PrP C ) and ⁄ or its availability for this structural alteration;

interfere with the conversion either directly or indirectly (via the

pathological chaperones or metals); and promote removal of the

disease-associated conformers.

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species Transmissibility of prionoses between different

species is generally ineffective due to differences in the

PrP sequence The phenomenon protecting one species

from acquiring a prion disease from another is called

‘the species barrier’ Therefore, scrapie (a prionosis

affecting sheep) is not transmissible to humans The

species barrier does not provide absolute protection;

therefore, transmission of scrapie to cattle and

trans-mission of bovine spongiform encephalopathy (BSE)

from cattle to humans results in the emergence of

vCJD In transmissible prionoses, exogenous PrPSc

present in the inoculum is responsible for the

conform-ational transformation of host PrPC Upon entering an

organism, PrPSc initially replicates within the

lym-phoreticular organs, including the spleen, lymph nodes

and tonsils, for months to years prior to neuroinvasion

and the onset of neurological symptoms Therefore,

infected but asymptomatic individuals are a reservoir

of infectious material This occurs because PrPC is

expressed by follicular dendritic cells and other

lym-phoid cells [27] Accumulation of PrPScin the

lympha-tic organs of presymptomalympha-tic humans infected with

BSE has been demonstrated by immunohistochemistry

[28] PrPSc replication is possible because it does not

elicit an immune response [29] This is related to the

inability of the immune system to distinguish between

PrPCand PrPSc

Vaccination approaches for AD

Vaccination was the first treatment approach

demon-strated to have genuine impact on disease process, at

least in animal models of AD Vaccination of AD

transgenic (Tg) mice with Ab1–42 or Ab homologous

peptides coinjected with Freund’s adjuvant prevented

the formation of Ab deposition and, as a consequence,

eliminated the behavioral impairments that are related

to Ab deposition [30–35] Similar effects on Ab load

and behavior have been demonstrated in AD Tg mice

by peripheral injections of anti-Ab monoclonal serum

indicating that the therapeutic effect of the vaccine

is based primarily on eliciting a humoral response

[36,37] The striking biological effect of the vaccine in

preclinical testing and the apparent lack of side-effects

in AD Tg mice encouraged Elan⁄ Wyeth to launch

clin-ical trials with a vaccine designated as AN1792 which

contained preaggregated Ab1–42 and QS21 as an

adju-vant This type of vaccine design was aimed to induce

a strong cell-mediated immune response because QS21

is known to be a strong inducer of Th-1 lymphocytes

[38] The initial safety testing of AN1792 in phase I of

the trial did not demonstrate any adverse effects The

phase II of the trial was prematurely terminated when

6% of vaccinated patients manifested symptoms of acute meningoencephalitis [38,39] An autopsy per-formed on one of the affected patients revealed an extensive cytotoxic T-cell reaction surrounding some cerebral vessels; however, analysis of the Ab load in the brain cortex suggested that Ab clearance had occurred [40] It appeared that the immune reaction triggered by AN1792 was a double-edge sword, where the benefits of a humoral response against Ab were overshadowed in some individuals by uncontrolled cytotoxicity [41] Not all patients who received AN1792 responded with antibody production The majority mounted a humoral response and showed a modest but statistically significant cognitive benefit demonstrated as an improvement on some cognitive testing scales compared to baseline and a slowed rate

of disease progression compared to patients who did not form antibodies [42] The follow-up data from the

‘Zurich’s cohort’, who are a subset of the Elan⁄ Wyeth trial followed by Dr Nitsch’s group [42,43], indicated that the vaccination approach may be beneficial for human AD patients but that the concept of the vaccine has to be redesigned

It appears that a humoral response elicited by the vaccine has at least two mechanisms of action and both

of these are thought to be involved in amyloid clearance [44,45] Conformational selective anti-Ab serum may target Ab deposits in the brain [43] leading to their disassembly [46,47] and elicit Fc mediated phagocytosis

by microglia cells The second mechanism by which anti-Ab serum likely prevents Ab deposition is the cre-ation of a ‘peripheral sink’ effect, where the removal of excess sAb circulating in the blood stream leads to sAb being drawn out from the brain [31,34, 47,48] This per-ipheral sink mechanism is likely to be the dominant means of reducing Ab peptides in the brain

The cause(s) for the toxicity in 6% of the Elan trial patients are not entirely known; however, from the available clinical and limited autopsy data, it is thought that an excessive Th-1 cell-mediated response within the brain was to blame [49] The concept of a redesigned AD vaccine puts emphasis on avoiding this cell-mediated response in the following ways: (a) avoiding stimulation of Th-1 lymphocytes so the vaccine could potentially elicit a purely humoral res-ponse; (b) using nontoxic and nonfibrillogenic Ab homologous peptides, so that the immunogen can not produce any direct toxicity; and (c) enhancing the peripheral sink effect rather than central action Passive transfer of exogenous anti-Ab monoclonal serum appears to be the easiest way to fulfill the goal of providing anti-Ab serum without risk of uncontrolled Th-1 mediated autoimmunity AD Tg model mice

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treated this way had a significantly reduced Ab level and

demonstrated cognitive benefit [36,37] The major

draw-backs of this approach are the high cost, limited half-life

of monoclonal antibodies (2–21 days depending on class

and isoform) and the potential for inducing serum

sick-ness with resultant complications such as renal failure

or lymphomas Nevertheless, clinical trials for passive

immunization trials are underway Alternative

approa-ches for passive immunization which are less likely to be

associated with toxicity, are use of Fv fragments or

mimetics of the active antibody binding site

Another potential source of toxicity in association

with passive immunization is cerebral hemorrhage The

mechanism of this hemorrhage is thought to be

inflam-mation in association with cerebral amyloid deposits

(congophilic amyloid angiopathy; CAA) that weakens

the blood vessel wall Several reports have shown an

increase in microhemorrhages in different AD mouse

models following passive intraperitoneal immunization

with different monoclonal antibodies with high affinity

for Ab plaques and CAA [50–52] The risk of

micro-hemorrhage following active immunization in animal

models has not been fully assessed It has not been

a problem in our own active immunization studies

[34,35], but has been reported in one study [53]

Furthermore, the clinical trial data from the limited

number of autopsied cases suggests that vascular

amyloid was not being cleared and that hemorrhage

may have been increased [54–56] In one of these

autopsies, numerous cortical bleeds, which are

typically rare in AD patients, were evident [55] In

addition, the association of T lymphocytosis and

cuffing with the cerebral vessel Ab in these autopsies

suggests a potential role of CAA and an excessive

Th-1 response in the genesis of the inflammatory

side-effects [57] This is an important issue because CAA is

present in virtually all AD cases, with approximately

20% of AD patients having ‘severe’ CAA [58]

Furthermore CAA is present in approximately 33% of

cognitively normal elderly, control populations [59–61]

Understanding the antigenic profile of Ab peptide,

allows engineering of modifications that favor a

humoral response and reduce the potential for a Th-1

mediated response This approach has been termed

altered peptide ligands Computer models have

predic-ted that Ab1–42 has one major antibody binding site

located on its N-terminus and two major T-cell epitopes

located at the central and C-terminal hydrophobic

regions encompassing residues 17–21 and 29–42,

respectively [62–64] Therefore, their elimination or

modification provides a double gain by eliminating

tox-icity, as well as the potential for T-cell stimulation

Sigurdsson et al [34] immunized AD Tg mice with

K6Ab1–30[E18E19], a nontoxic Ab-homologous peptide, where the first above mentioned T-cell epitope was modified and the second removed Polyamino acid chains coupled to its N-terminus aimed to increase the immunogenicity and solubility of the peptide AD Tg mice vaccinated with this peptide produced mainly an IgM class antibodies and low or absent IgG titer These animals showed behavioral improvement and a partial reduction of Ab deposits [34,35] One of the advantages

of this design is that IgM, with a molecular mass of

900 kDa, does not penetrate the blood–brain barrier (BBB) and therefore is unlikely to be associated with any immune reaction in the brain Like passive immun-ization, this type of vaccine focuses its mechanism of action on the peripheral sink Furthermore, the IgM response is reversible because it is T-cell independent; hence memory T-cells that could maintain the immune response are not generated Therefore, this vaccine method may potentially be safer than typical active immunization

Mucosal vaccination can be an alternative way to achieve a primarily humoral response This mechanism

is based on the presence of lymphocytes in the mucosa

of the nasal cavity and of the gastrointestinal tract This type of response produces primarily S-IgA antibodies but, when the antigen is coadministrated with adjuvants such as cholera toxin subunit B or heat-labile Escheri-chia coli enterotoxin, significant IgG titer in the serum may be achieved [65,66] A marked reduction of Ab bur-den in AD Tg mice immunized this way using Ab as an antigen has been already demonstrated [66,67] Interest-ingly, this type of mucosal immunization has recently been shown to be highly effective for prion infection [68,69,70] This promising approach requires further exploration, especially using nonfibrillar and nontoxic

Ab homologous peptides as an antigen Mucosal immunization offers a great potential advantage in that

a more limited humoral immune response can be obtained, with little or no cell-mediated immunity

Inhibition of Ab fibrillization Formation of Ab fibrils and deposition of Ab in the brain parenchyma or in the brain’s vessels occurs in the setting of increased local Ab peptide concentra-tions [71] Initially, condiconcentra-tions do not favor aggrega-tion of fibrils; however, once a critical nucleus has been formed, aggregation with fast kinetics is favored Any available monomer can then become entrapped in

an aggregate or fibril Several compounds, such as Congo red [71], anthracycline [73], rifampicin [74], anionic sulphonates [75], or melatonin [76], can inter-act with Ab and prevent its aggregation into fibrils

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in vitro, thereby reducing toxicity It has been further

identified that certain nonfibrillogenic, Ab homologous

peptides can bind to Ab and break the formation of

b-sheet structure [77–80] Therefore, these peptides

were termed b-sheet breakers Several modifications

were used to extend serum half-life and increase BBB

permeability of these peptides Permanne et al [81],

using a BBB permeable five amino-acid long peptide

(iAb5), were able to demonstrate a reduction of Ab

load in AD Tg mice that received this peptide compared

with age-matched control group which received placebo

Of interest, a similar concept of b-sheet breakers has

been shown to be applicable to prion disease [82]

Extensive evidence suggests that the most toxic forms

of Ab are oligomeric aggregates [83] There is also

evi-dence implicating oligomeric aggregates in the

medi-ation of PrPSctoxicity and infectivity [84,85] Recently,

compounds and antibodies have been developed that

specifically target Ab oligomers [86–88] Similar

approa-ches are being developed for prion oligomers

Ab homologous peptides can aggregate and form

fibrils spontaneously in vitro; however, in vivo this

pro-cess appears more dependant on the presence of Ab

pathological chaperones This group of proteins

promotes conformational transformation at certain

concentrations by increasing the b-sheet content of

these disease specific proteins and stabilizes their

abnormal structure [89,90] Examples of such proteins

in AD include apoE, especially its E4 isoform [18,91],

ACT [20] or C1q complement factor [21,22] In

their presence, the formation of Ab fibrils in a solution

of sAb monomers becomes much more efficient

[18,20] These ‘pathological chaperone’ proteins have

been found histologically and biochemically in

associ-ation with fibrillar Ab deposits [23,89,92,93] but not in

preamyloid aggregates that are not associated with

neuronal toxicity [24,94] Inheritance of the apoE4

isoform has been identified as the major identified

genetic risk factor for sporadic, late-onset AD [95] and

correlates with an earlier age of onset and greater Ab

deposition, in an allele-dose-dependent manner

[19,95,96] In vitro, all apoE isoforms can propagate

the b-sheet content of Ab peptides promoting fibril

formation [92], with apoE4 being the most efficient

[18] The critical dependence of Ab deposition in

plaques on the presence of apoE has also been

confirmed in AD Tg APPV717F⁄ apoE– ⁄ –

mice which have a delayed onset of Ab deposition, a reduced Ab

load, and no fibrillar Ab deposits Compared to

APPV717F⁄ apoE+⁄ +Tg mice, APPV717F⁄ apoE+⁄ – mice

demonstrate an intermediate level of pathology

[97–100] Neutralization of the chaperoning effect of

apoE would therefore potentially have a mitigating

effect on Ab accumulation ApoE hydrophobically binds to the 12–28 amino acid sequence of Ab, form-ing SDS insoluble complexes [101–103] Ma et al [104] have demonstrated that a synthetic peptide homolog-ous to 12–28 amino-acid sequence of Ab can be used

as a competitive inhibitor of the binding of full length

Ab to apoE, resulting in reduced fibril formation

in vitro and increased survival of cultured neurons The introduction of several modifications to Ab12–28

by replacing a valine for proline in position 18, making this peptide nontoxic and nonfibrillogenic, as well as end-protection by amidation and and acetylation of the C- and N-termini, respectively, to increase serum half-life, have allowed us to use this peptide therapeu-tically in the APPK670N⁄ M671L⁄ PS1M146L double Tg mice model Tg mice treated with Ab12–28P for

1 month demonstrated a 63.3% reduction in Ab load

in the cortex (P¼ 0.0043) and a 59.5% (P ¼ 0.0087) reduction in the hippocampus comparing to age-matched control Tg mice that received placebo [105,106] The treated Tg mice also had a cognitive benefit [105,106] No antibodies against Ab were detec-ted in sera of treadetec-ted mice; therefore, the observed therapeutic effect of Ab12–28P cannot be attributed to

an antibody clearance response This experiment demonstrates that compounds blocking the interaction between Ab and its pathological chaperones may be beneficial for treatment of Ab accumulation in AD [14,105,106] Whether similar approaches can be used for prion disease remains to be determined

Prion disease Interest in prion disease has greatly increased subse-quent to the emergence of BSE in England and the resulting appearance of vCJD in human populations BSE arose from the feeding of cattle with prion con-taminated meat and bone meal products, whereas vCJD developed following entry of BSE into the human food chain [107,108] Since the original report

in 1995, a total of 201 probable or confirmed cases of vCJD have been diagnosed, 165 in Great Britain, 21 in France, four in Ireland, three in the USA, two in the Netherlands and one each in Italy, Canada, Japan, Saudi Arabia, Portugal and Spain Most of the patients from these countries resided in the UK during

a key exposure period of the UK population to the BSE agent It has proven difficult to predict the expec-ted future numbers of vCJD Mathematical analysis has given a range from 1000 to approximately 136 000 individuals who will eventually develop the disease This broad range reflects a lack of knowledge regard-ing the time of incubation and the number of patients

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who could be infected from a given dosage of BSE

agent Because the vCJD agent is present at high levels

in the lymphatic tissue, screening for PrPSc was

per-formed on sections from lymph nodes, tonsils, and

appendices archives in the UK Three out of 12 674

randomly selected cases showed evidence of subclinical

infection, leading to a prediction that approximately

4000 vCJD further cases may occur in the UK [109]

However, there is much uncertainty about such a

pre-diction because it is not known whether all subclinical

infections will progress and also whether such

screen-ing of lymphoid tissue would capture all subclinical

cases The initially predicted epidemic of vCJD does

not seem to be materializing because the number of

cases in the UK has declined from a peak of 28 in

2000 to five cases in 2006 [107] A complicating factor

for estimating future numbers of vCJD is the

docu-mentation of several transfusion associated cases

These occurred after incubation periods of 6–8 years

One of these disease associated donations was made

more than 3 years before the donor became

sympto-matic, suggesting that vCJD can be transmitted from

silently infected individuals [110] The estimated risk

for new cases of vCJD in other European countries

looks more optimistic In the UK, 200 000 cases of

BSE were reported (it is estimated that four times this

number entered the food chain), compared to

approxi-mately 5600 BSE cases in other European countries

(with the highest numbers being 1590, 1030 and 986 in

Ireland, Portugal and Frances, respectively) This

sug-gests a significantly lower exposure of these

popula-tions to BSE prions A few cases of BSE have also

been reported in other parts of the world, such as

Japan, the USA and Canada

Of greater concern in North America is chronic

wast-ing disease (CWD) This disease is now endemic in

Colorado, Wyoming and Nebraska and continues to

spread to other parts in the USA, initially in the

Mid-west but now detected as far East as New York State

[111,112] Most vulnerable to CWD infection are white

tailed deer and the disease is now found in areas with a

large population of these animals, which indicates that

its prevalence can be expected to increase substantially

in the future The occurrence of CJD among three

young deer hunters from this same region raised the

spe-culation of transmission of the CWD to humans [113]

However, autopsy of these three subjects did not reveal

the extensive amyloidosis characteristic of vCJD and

CWD [114] However like BSE, CWD is transmissible

to nonhuman primates and transgenic mice expressing

human PrPC[115,116] Therefore, the possibility of such

transmission needs to be closely monitored CWD is

similar to BSE in that the peripheral titers of the prion

agent are high PrPSchas been detected in both muscle and saliva of CWD infected deer [117,118]

Vaccination as a therapeutic approach for prionoses

The prion protein is a self-antigen; hence, prion infec-tion is not known to elicit a classical immune response

In fact, the immune system is involved in the peri-pheral replication of the prion agent and its ultimate access to the CNS [29,68] This involvement is further supported by the observation that immune suppression with, for example, splenectomy or immunosuppressive drugs, increases the incubation period This interval, during which time the prion agent replicates peripher-ally, without producing any symptoms, is quite long, lasting many months in experimental animals and up

to 56 years in documented human cases associated with cannibalistic exposure to the prion agent [119] Lymphatic organs such as the spleen, tonsils, lymph nodes or gut associated lymphoid tissue contain high concentrations of PrPSc long before PrPSc replication starts in the brain [27,120,121] Cells found to be par-ticularly important for peripheral PrPScreplication are the follicular dendritic cells (DC) and the migratory bone-marrow derived DC [121,122] DC from infected animals are capable of spreading the disease [122] An emerging therapeutic approach for prion infection is immunomodulation [68,70,123]

Currently, there is no treatment that would arrest and⁄ or reverse progression of prion disease in non-experimental settings, although many approaches have been tried [124] Partly due to the success in AD models discussed above, similar experiments with anti-PrP serum were initiated in prion infectivity cul-ture models as well as active and passive immuniza-tion studies in rodent models Earlier in vivo studies showed that infection with a slow strain of PrPSc blocked expression of a more virulent fast strain of PrP, mimicking vaccination with a live attenuated organism [125] In tissue culture studies, anti-PrP serum and antigen binding fragments directed against PrP were shown to inhibit prion replication [126–128] Although we first demonstrated that active immunization with recombinant PrP delayed the onset

of prion disease in wild-type mice, the therapeutic effect was relatively modest and, eventually, all the mice succumbed to the disease [129] This limited therapeutic effect may be explained by the observa-tion that antibodies generated against prokaryotic PrP often do not have a high affinity towards PrPC [130], although, in our studies, the increase in the incubation period correlated well with the antibody

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titers against PrPC Our follow-up passive anti-PrP

immunization study confirmed the importance of the

humoral response, showing that anti-PrP serum is

able to prolong the incubation period [131]

Subse-quently, other investigators, using a much higher

anti-body dosage, were able to completely prevent disease

onset in mice exposed to PrPSc provided that passive

immunization was initiated within 1 month of

expo-sure [132] This type of approach could be used

immediately following accidental exposure in humans

to prevent future infection However, passive

immun-ization has not been found to be effective closer to

the clinically symptomatic stages of prion infection

Also, passive immunization would be an approach

that is too costly for animal prion diseases

In the development of immunotherapeutic

approa-ches targeting a self-antigen, designing a vaccine

avoid-ing auto-immune related toxicity is a major concern

The emerging data from AD targeting immunization is

that toxicity is due to excessive cell-mediated immunity

within the CNS, whereas the therapeutic response is

linked to humoral immunity In addition, toxicity

could be partially related to the immunogen and⁄ or to

the adjuvant used; in the human AD vaccination trial,

fibrillar Ab1–42 was used as an immunogen This

pep-tide is well characterized to be toxic Hence, we have

been promoting the use of nonamyloidogenic

deriva-tives as immunogens for protein conformational

disor-ders, including AD and prion disease [31,34,38] How

significant an issue direct toxicity of the immunogen

may be for prion vaccination remains unclear Unlike

the Ab peptide used for vaccination in AD models,

direct application of recombinant PrP has not been

shown to be toxic However, this issue has not been

investigated as thoroughly as in the Alzheimer’s field

and remains controversial Several lines of evidence

suggest that intracellular accumulations of PrPSc

pro-mote neurodegeneration [133]

A potential ideal means of using immunomodulation

to prevent prion infection is by mucosal immunization

One important reason for this is that the gut is the

major route of entry for many prion diseases such as

CWD, BSE and vCJD Furthermore, mucosal

immun-ization can be designed to induce primarily a humoral

immune response, avoiding the cell-mediated toxicity

that was seen in the human AD vaccine trial In

addi-tion, mucosal vaccination has the advantage that it is

unlikely to induce significant immune response within

the brain Although it has been shown that reduced

levels or absence of CNS PrPCby, for example,

condi-tional ablation by genetic manipulation of neuronal

PrPC [134] can prevent clinical prion infection, it is

likely that the immunological targeting of neuronal

PrP would be associated with inflammatory toxicity Recently, we have been developing prion vaccines that target gut associated tissue, the main site of entry of the prion agent One of our approaches is to express PrP in attenuated Salmonella strains as a live vector for oral vaccination, which has resulted in prevention

or significant delay of prion disease in mice [69] Live attenuated strains of Salmonella enterica have been used for many years as vaccines against salmonellosis and as a delivery system for the construction of multi-valent vaccines with a broad application in human and veterinary medicine [135] A main advantage for this system is that the safety of human administration of live attenuated Salmonella has been extensively con-firmed in humans and animals [136,137] Ruminants and other veterinary species can be effectively immun-ized by the oral route using attenuated Salmonella, to induce humoral mucosal responses [138,139] We are currently exploring ways to increase the efficacy even further In these studies, the mucosal IgA anti-PrP titer correlates well with the delay or prevention of prion infection, further supporting the importance of the humoral response for the therapeutic effect Salmonella target M-cells, antigen sampling cells in the intestines, which may also be important for uptake of PrPSc [27,68,121] Hence, this approach is more targeted than prior vaccination studies, likely explaining the improved efficacy By exploring other strains of attenu-ated Salmonella, using different bacteria or oral adjuvants, and⁄ or by altering the expression levels or sequence of the PrP antigen, it is likely that the percentage of uninfected animals can be improved Our recent work utilizing this approach indicates that complete protection to clinical prion infection via an oral route is possible Overall, this approach holds great promise as an inexpensive prophylactic immuno-therapy to prevent the spread of prion disease, partic-ularly in animals at risk and perhaps eventually in certain high risk human populations

Metal chelation for prion and AD Metal chelation is emerging as an important therapeu-tic approach for AD, which is currently in clinical trial [140,141] This approach for AD is reviewed elsewhere

in this minireview series Importantly, modulation of metal levels, in particular copper, has been shown to

be important for the conversion of PrPC to PrPSc, highlighting another similarity between AD and prion diseases [10] Copper binding is thought to be part of the normal function of PrPC[142–144] The binding of copper to PrPC gives the complex antioxidant activity [145,146]; hence, it has been suggested that the reduced

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copper binding of PrPSc with a consequent reduction

of antioxidant activity is part of the pathogenesis of

prion disease [147] This hypothesis has been supported

by the finding that copper is reduced up to 50% in the

brains of sporadic CJD patients [148] How copper

binding influences the PrPC to PrPSc conversion is

complex [10,149] We were the first to show that,

sim-ilar to studies in AD Tg models, metal chelation can

be used therapeutically [150] in prion infection Our

studies indicated that penicillamine, a copper chelator,

prolongs the incubation period of scrapie in mice

[150] Consistent with this observation, the presence of

copper has also been shown to stabilize the PrPSc

con-formation using preformed fibrils [151–158], as well as

to induce aggregation of the prion peptide 106–126

[159] Some tissue culture studies of prion infection

have also suggested that copper chelators are suitable

candidates for antiprion drugs [160] However, there

are conflicting reports indicating that the interaction

between copper and PrP is likely to be quite complex

For example, copper has been shown to inhibit the

in vitro conversion of recombinant PrP into amyloid

fibrils but, also in contrast, to enhance the

protein-ase K resistance of preformed fibrils [157] These

findings indicate that copper may have a dual and

opposite effect on prion propagation It may both

inhibit prion replication and prevent clearance of

potentially infectious forms of the prion protein

Furthermore, copper treatment has also been shown to

inhibit PrPSc amplification in reactions where brain

derived PrPCwas used as a seed [161], as well as

delay-ing the onset of clinical disease in scrapie infected

hamsters [162] In addition, it has been shown that

physiological levels of copper promote internalization

of PrPC[163] The interaction between PrPCand

cop-per was found to be the overriding factor in

stimula-ting the internalization response with other metals

showing no effect The decrease in detectable levels of

PrPC at the cell surface following copper treatment

was found to be the result of internalization rather

than loss into the surrounding environment [163]

Such internalization would limit the exposure of

PrPC to conversion from exogenous PrPSc; however,

because cytoplasmic forms of PrP have been linked to

neurodegeneration [133], increased internalization

could also be deleterious in some settings Copper has

also been shown to have immunomodulatory effects

[164] and, as discussed earlier, the immune system can

have profound effects on prion infection Hence, it

appears that the deleterious or beneficial role of copper

in prion infection might vary depending on which

function predominates under the distinct experimental

conditions being used Nevertheless, it is clear that a

greater understanding of the role of metal binding in prion infection presents a therapeutic opportunity

Conclusions Immunization appears to be an effective therapeutic method for prevention of Ab deposition and cognitive decline in AD, provided that cell-mediated auto-immune toxicity can be avoided The second genera-tion AD vaccines, which are under development, are based on nontoxic and nonfibrillar Ab homologous peptides that are modified to eliminate the potential for inducing cellular immunity, and elicit primarily a humoral response Other related approaches include direct administration of antibodies that target Ab These interventions would likely favor a peripheral sink effect, clearing soluble Ab from the blood stream and inducing efflux of Ab from the brain Additional potentially synergistic therapeutic approaches for AD would include blocking the interaction of Ab with its

‘pathological chaperones’ such as apoE, as well as use

of b-sheet breaker compounds Immunization approa-ches could be used for sporadic AD, familial AD, and

AD associated with Down’s syndrome The effective-ness of treatment would depend on its initiation early

in the disease course Therefore, such a treatment needs to coincide with the development of a procedure for the detection and monitoring of Ab deposits Both active and passive immunization appear to be effective in prevention of prion infections in animal models Further studies are needed to develop specific protocols applicable for human use Active immuniza-tion, using especially mucosal immunization could be used to prevent spread of BSE through the oral route, whereas passive immunization protocols would

be more appropriate for subjects accidentally infected with prion contaminated material (e.g blood transfu-sion or organ transplant) Effective immunization for prion infections works through prevention of entry of PrPSc via the gut and⁄ or neutralization of PrPSc replicating in the peripheral lymphoreticular system Metal chelation is another promising therapeutic approach for AD, which is currently undergoing clinical trials Similar approaches are just emerging for prion diseases However, a greater understanding

of the role of copper and other metals in the PrPCto PrPSc conversion is needed before this therapeutic strategy can be effectively harnessed for prion infection

Acknowledgements This manuscript is supported by NIH grants: AG15408, AG20245, AG20197 and the Alzheimer’s Association

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