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Tài liệu Báo cáo khóa học: A multi-protein complex containing cold shock domain (Y-box) and polypyrimidine tract binding proteins forms on the vascular endothelial growth factor mRNA Potential role in mRNA stabilization pptx

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A The sequence of the VEGF 5¢-UTR V1 RNA probe is shown and consensus CSD and PTB protein binding site sequences are indicated.. Results The VEGF 5¢-UTR binds cytoplasmic and recombinant

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A multi-protein complex containing cold shock domain (Y-box)

Potential role in mRNA stabilization

Leeanne S Coles1,*, M Antonetta Bartley1,*, Andrew Bert1, Julie Hunter1, Steven Polyak2, Peter Diamond1, Mathew A Vadas1,3and Gregory J Goodall1,3

1

Division of Human Immunology, The Hanson Institute, Institute of Medical and Veterinary Science;2Division of Biochemistry, Department of Molecular Biosciences, The University of Adelaide;3Department of Medicine, The University of Adelaide,

North Terrace, Adelaide, South Australia, Australia

Vascular endothelial growth factor (VEGF) is a key

regu-lator of angiogenesis and post-transcriptional regulation

plays a major role in VEGF expression Both the 5¢- and

3¢-UTR are required for VEGF post-transcriptional

regu-lation but factors binding to functional sequences within

the 5¢-UTR have not been fully characterized We report

here the identification of complexes, binding to the VEGF

mRNA 5¢- and 3¢-UTR, that contain cold shock domain

(CSD) and polypyrimidine tract binding (PTB) RNA

binding proteins Analysis of the CSD/PTB binding sites

revealed a potential role in VEGF mRNA stability, in both

noninduced and induced conditions, demonstrating a

gen-eral stabilizing function Such a stabilizing mechanism had

not been reported previously for the VEGF gene We further

found that the CSD/PTB-containing complexes are large

multiprotein complexes that are most likely preformed in

solution and we demonstrate that PTB is associated with the

VEGFmRNA in vivo Complexformation between CSD proteins and PTB has not been reported previously Analysis

of the CSD/PTB RNA binding sites revealed a novel CSD protein RNA recognition site and also demonstrated that CSD proteins may direct the binding of CSD/PTB com-plexes We found the same complexes binding to an RNA-stabilizing element of another growth factor gene, suggesting

a broader functional role for the CSD/PTB complexes Finally, as the VEGF gene is also regulated at the tran-scriptional level by CSD proteins, we propose a combined transcriptional/post-transcriptional role for these proteins in VEGF and other growth factor gene regulation

Keywords: cold shock domain proteins; Y-boxprotein; polypyrimidine tract binding protein; mRNA stabilization; vascular endothelial growth factor

VEGF is an essential regulator of angiogenesis that acts on

vascular endothelial cells to induce proliferation and

promote cell migration [1–3] Disregulated VEGF

expres-sion is implicated in a number of diseases that are

characterized by abnormal angiogenesis [1–6] In the case

of solid tumors, the overexpression of VEGF, produced in

response to activated oncogenes, growth factors or low

oxygen conditions (hypoxia), plays a major role in

promo-ting tumor angiogenesis and progression [1–3,7] Both the

cancer cells themselves and nontumor support cells, such as

fibroblasts, are sources of VEGF [8] In contrast, in the case

of coronary artery disease, inadequate VEGF expression rather than VEGF overexpression, plays a role in disease progression A number of cell types, including cardiac myocytes, fibroblasts and endothelial cells produce VEGF

in response to hypoxia, but this natural response is not sufficient to prevent the further progression of heart disease [9–11] It is therefore important to understand the mecha-nisms of VEGF regulation to develop means to control VEGF expression

Post-transcriptional regulation plays a major role in VEGF expression, with regulation occurring at the level of splicing, mRNA stability and translation [2,7] The VEGF mRNA is normally unstable and its stability is increased in response to cytokines and stress conditions such as hypoxia [7,11–14] Regions in both the 5¢- and 3¢-UTR have been shown to be involved in VEGF mRNA stabilization [7,12,13,15–18] The presence of an internal ribosome entry site (IRES) in the VEGF 5¢-UTR ensures continual translation of the VEGF mRNA in stress conditions that normally decrease cap-dependent translation [19–21] Little

is known about the factors involved in VEGF post-transcriptional regulation Factors such as HuR and hnRNPL have been implicated in hypoxic stability via their

Correspondence to L S Coles, Division of Human Immunology,

The Hanson Institute, Institute of Medical and Veterinary Science,

Frome Road., Adelaide, South Australia, 5000, Australia.

Fax: + 61 88 2324092, Tel.: + 61 88 2223432,

E-mail: leeanne.coles@imvs.sa.gov.au

Abbreviations: CSD, cold shock domain; IRES, internal ribosome

entry site; VEGF, vascular endothelial growth factor.

*These authors contributed equally to this work.

(Received 16 October 2003, revised 14 December 2003,

accepted 16 December 2003)

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actions on the VEGF 3¢-UTR [17,18] but factors involved in

stability or translational regulation have not been identified

on the 5¢-UTR

The single-strand RNA and DNA binding, cold shock

domain (CSD) (also known as Y-box) proteins, play

diverse roles in both transcriptional and

post-transcrip-tional regulation of growth factor and stress response

genes [22–29] CSD proteins have several family members

which are defined by the presence of a central highly

conserved 70 amino acid region called the cold shock

domain [24,25,29] The central domain is required for

sequence-specific RNA binding, while the adjacent

C-terminal domain has a more nonspecific role in

stabilizing binding [24–27] There are two types of

nongerm cell CSD proteins and these are called dbpB

(also known as YB-1, MSY-1, chkYB-1b, EF1A, p50 and

FRGY1) and dbpA (MSY4, chkYB-2 and YB2/RYBa)

DbpB and dbpA CSD proteins are ubiquitously expressed

and are highly conserved across species Highly conserved

germ cell-specific CSD proteins also exist such as MSY-2

and FRGY2 [22–25,29] In addition there are CSD-related

proteins such as UNR (upstream of N-ras) which contains

multiple conserved CSD domains [30] CSD proteins

stabilize growth factor/stress response mRNAs in response

to stress signals [31–33] and also act as general mRNA

stabilizers [34–37] In addition, CSD and CSD-related

proteins have been shown to play a role in cap-dependent

and [26,27,38–42] IRES-dependent [43–46] translation and

in RNA splicing [47,48] In the case of the GM-CSF

(granulocyte-macrophage colony stimulating factor)

growth factor gene, CSD proteins have been shown to

play a combined role at both the transcriptional and

post-transcriptional levels [22,23,49,50] As we have recently

shown a role for CSD proteins in regulation of the VEGF

gene at the transcriptional level [51], and given the diverse

functions of CSD proteins, relevant to VEGF expression,

we investigated a role for CSD proteins in VEGF

post-transcriptional regulation

We now show here that CSD proteins can bind to both

the 5¢- and 3¢-UTR of the VEGF mRNA We find that

CSD proteins form a cytoplasmic complexon VEGF

mRNA that also contains the multifunctional

single-strand RNA/DNA binding protein, PTB [43–46,52–57],

and that the binding of this complexmay be involved in

general VEGF mRNA stabilization The

CSD/PTB-con-taining cytoplasmic complexalso forms on a stability

element in the interleukin-2 (IL-2) 5¢-UTR suggesting a

similar mechanism of regulation of stability of growth

factor mRNAs

Materials and methods

Plasmid constructs

The pGEM44, pGEM46 and pGEM47 constructs were

generated by cloning segments of the mouse VEGF

5¢-UTR, that were amplified by PCR from the pfVEGF

construct [15], into pGEM4Z (Promega) The pGEM44,

46 and 47 constructs contain, respectively, mouse VEGF

5¢-UTR sequences +1 to +325, +461 to +727 and +735 to

+1014 (relative to the transcription start site at +1) [58]

(Fig 1) The pGEMV1 construct, containing the VEGF

5¢-UTR CSD site 1 sequences (+150 to +185) was constructed by cloning double strand oligonucleotides (with EcoRI 5¢- and HindIII 3¢-ends) into pGEM4Z pGEMV37,

39, 15, 17 and 19 were similarly constructed, except that they contained mutant versions of the CSD site 1 sequences

Fig 1 The VEGF 5¢-UTR binds cytoplasmic and recombinant CSD proteins (A) Schematic of the mouse VEGF 5¢-UTR The sequences and coordinates (relative to the mRNA start site +1) [58] of consensus CSD binding sites (CSD site 1,2) are indicated The coordinates of RNA probe sequences are also indicated RNA probes were derived from pGEM44, pGEM46 and pGEM47, respectively (B) Balb/c 3T3 fibroblast cytoplasmic extracts were incubated without competitor (–)

or with unlabeled single-strand DNA competitor oligonucleotides containing wild-type (CSDwt) and mutant (CSDmut) CSD binding sites [49–51] 32 P-Labeled RNA probes (44 and 46) were then imme-diately added and RNase T1 digested complexes analyzed by gel shift assay Cytoplasmic complexes CC44a, CC44b and CC46 and unbound RNA probe are indicated (C) Cytoplasmic extracts were preincubated with anti-CSD polyclonal Ig (CSD), with preimmune serum (PI) or left untreated (–), followed by addition of the labeled VEGF 44 RNA probe in a gel shift assay Increasing amounts of anti-CSD Ig were added Pre-immune sera was used at the maximal concentration used for the anti-CSD Ig Cytoplasmic complexes CC44a and CC44b are indicated (D) Recombinant GST-dbpB/YB-1 was incubated with labeled 44, 46 and 47 RNA probes Complexes were competed with wild-type (CSDwt) or mutant (CSDmut) CSD binding site single-strand DNA competitors or left untreated (–).

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(Figs 2 and 3) pGEMV25 and pGEMV27 were

construc-ted by cloning wild-type and mutant double strand

oligo-nucleotides containing the IL-2 5¢-UTR +1 to +35

sequences [31] (Fig 4) pGEMVC1 was constructed by

cloning double strand oligonucleotides containing the

VEGF 3¢-UTR CSD site 3 (+1712 to +1747, relative to

the stop codon at +1, of the mouse VEGF 3¢-UTR) [59]

into pGEM4Z pGEMVC2 and VC3 contained mutations

in the CSD site 3 sequence (Fig 6)

The pfVEGF construct contained a reconstructed, tagged VEGF cDNA sequence [15], composed of the entire VEGF mouse 5¢-UTR (+1 to +1014), the coding region for the 164 amino acid form of VEGF and the VEGF 3¢-UTR (+4 to +2195) The major polyadenylation site is at +1861 [59] A

Fig 2 The VEGF 5¢-UTR CSD-containing cytoplasmic complexes also

contain PTB (A) Schematic of the VEGF 5¢-UTR CSD site 1 The

coordinates for the VEGF RNA probes 44 and V1 are indicated

rel-ative to the start of the VEGF mRNA (+1) [58] (B) Balb/c 3T3

fibroblast cytoplasmic extract was incubated with labeled VEGF 44 or

V1 RNA probes, followed by RNase T1 digestion in a gel shift assay.

The 44 and V1 RNA probes are derived from pGEM44 and

pGEMV1, respectively Cytoplasmic complexes CC44a and CCV1

and unbound RNA probe are indicated (C) Cytoplasmic complexes

CC44 and CCV1, in gel shift assay gels, were exposed to UV light to

cross-link proteins in each complexto RNA Cross-linked proteins

were then analyzed by SDS/PAGE and the sizes of cross-linked

pro-teins were calculated by subtraction of the molecular weight of bound

RNA probe The sizes of cross-linked proteins are indicated

Cross-link analysis is not quantitative as different proteins will crossCross-link to

different extents (D) Cytoplasmic extracts were incubated with

unlabe-led wild-type or mutant CSD (CSDwt, mut) or PTB (PTB wt, mut) [52]

binding site single-strand DNA oligonucleotides, or left untreated (–).

Labeled V1 RNA probe was then immediately added and complexes

analyzed in a gel shift assay The CCV1 complexis indicated (E)

Cytoplasmic extracts were preincubated with an anti-PTB monoclonal

antibody (PTB), with a control anti-GM-CSF monoclonal antibody

(GM), or without antibody (–) Labeled V1 RNA probe was then

added and complexes analyzed in a gel shift assay.

Fig 3 Sequence requirement for VEGF 5¢-UTR CCV1 CSD/PTB complex formation-PTB complexes form on the VEGF mRNA in vivo (A) The sequence of the VEGF 5¢-UTR V1 RNA probe is shown and consensus CSD and PTB protein binding site sequences are indicated The 3¢ consensus PTB site is also found, in this report, to bind recombinant CSD protein (labeled CSD*) The sequences of mutant RNA probes are given under the V1 sequence Only those bases that are changed in the mutant probes are indicated The RNA probes were generated from pGEMV1, V37, V39, V15, V17 and V19 constructs, respectively (B) Balb/c 3T3 fibroblast cytoplasmic extracts were incubated with labeled wild-type (V1) and mutant VEGF 5¢-UTR CSD site 1 RNA probes in a gel shift assay The CCV1 cytoplasmic complex

is indicated (C) Recombinant GST-dbpB/YB-1 and GST-PTB were incubated with labeled wild-type (V1) and mutant (V37, V39) VEGF 5¢-UTR RNA probes in a gel shift assay The recombinant protein complexes are indicated (D) PTB binding to VEGF mRNA in vivo was investigated using an RNA immunoprecipitation assay Cytoplasmic RNA/protein complexes (prepared in the presence of RNase inhibi-tors) were immunoprecipitated with anti-PTB monoclonal Ig (PTB), with an IgG2 isotype control (control), or without antibody (–) VEGF mRNA in RNA extracted from immunoprecipitated complexes was detected by RT-PCR The VEGF PCR product is indicated.

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polylinker is positioned between the coding region and the

3¢-UTR sequences to distinguish pfVEGF mRNA from

endogenous VEGF mRNA pfVEGFdel contains deletions

of the site 1, 2 and 3 CSD sites (Fig 7) The sequences +156

to +179 (CSD site 1) and +650 to +666 (CSD site 2) of the

5¢-UTR were deleted and the sequences +1727 to +1740

(CSD site 3) of the 3¢-UTR were deleted

Construction of the expression vector producing

recom-binant GST-dbpB/YB-1 (pGEXBT) has been described

previously [49,51] pGEXPTB, for production of

recombin-ant GST-PTB, was constructed by cloning of a 1.6kb EcoRI

fragment from pcDNA3PTB (gift from T Cooper, Baylor

College of Medicine, Houston, TX, USA), coding for

human PTB, into pGEX4T-2

Oligonucleotides Oligonucleotides for cloning into pGEM4Z and for use as competitors in gel shift assays were synthesized by Gene-works (Adelaide, Australia) and purified from nondenatur-ing polyacrylamide gels Snondenatur-ingle-strand oligonucleotides for competition of CSD protein-containing complexes were from the human granulocyte-macrophage-colony stimula-ting factor (GM-CSF) gene The wild-type (CSDwt) and mutant sequences (CSD site mutant; CSDmut) have been described previously (GM- and GMm23-, respectively) [49–51] The CSD wild-type sequence binds both dbpA and dbpB CSD proteins The wild-type (PTBwt) and mutant PTB (PTBmut) competitor single-strand DNA oligonucleo-tides are from the transferrin gene (DR1 sense and DR1 sense mut1, respectively) [52]

RNA probe preparation

32P-labeled RNA probes for gel shift analysis or RNase protection assays were generated by in vitro transcription from linearized plasmid templates (pGEM4Z constructs) using SP6 (for pGEM44,46,47) or T7 (for pGEMV1, V25 and VC1) RNA polymerase (Promega) and [32P]UTP[aP] Probes for RNase protection assays were processed as previously described [15] Probes for gel shift assays were purified from nondenaturing polyacrylamide gels and eluted into RNase-free water at 56C

Preparation of recombinant and cytoplasmic proteins The Escherichia coli strain MC1061 transformed with pGEXBT or pGEXPTB was induced with isopropyl thio-b-D-galactoside to produce recombinant GST-dbpB/YB-1 and GST-PTB [49,51] The fusion proteins for gel shift analysis were purified on glutathione-Sepharose beads (Promega) Cytoplasmic extracts were produced according

to the method of Schrieber et al [60]

FPLC gel filtration of cytoplasmic extracts Cytoplasmic extract from Balb/c 3T3 fibroblasts was applied at a flow rate of 0.35 mLÆmin)1to a Superdex200 column (10 mm diameter, 20 mL bed volume) pre-equili-brated with buffer containing 150 mM KCl, 20 mM Tris/ HCl pH 7.6, 20% glycerol, 1.5 mMMgCl2, 2 mM dithio-threitol, 0.4 mMphenylmethanesulfonyl fluoride and 1 mM

Na3VO4 The CCV1 complexwas eluted with the same buffer and 0.5 mL fractions collected The molecular mass

of the complexwas estimated from the column by comparison with the elution volumes of c-globulin, bovine serum albumin, ovalbumin, myoglobin and vitamin B12 Antibodies

The anti-CSD antibody is a rabbit polyclonal Ig raised against a peptide conserved in dbpA and dbpB/YB-1 CSD proteins across species [49,51] The anti-PTB Ig is a mouse monoclonal antibody (BB7; gift from D Black, UCLA, Los Angeles, CA, USA) A mouse monoclonal anti-(GM-CSF) Ig (gift from A Lopez, Hanson Institute, IMVS, Adelaide, Australia) and an IgG2 monoclonal

Fig 4 CCV1 complex formation on the IL-2 5¢-UTR stability element

in fibroblasts and Jurkat T cells (A) Sequence of the IL-2 5¢-UTR

wild-type probe V25 with consensus CSD and PTB sites indicated The

region +1 to +22 is involved in IL-2 mRNA stabilization in T cells

[31] The V27 mutant sequence is shown with only those bases differing

from the wild-type sequence shown (B) Balb/c 3T3 fibroblast

cyto-plasmic extracts were incubated with labeled VEGF (V1) and IL-2

(V25,V27) 5¢-UTR RNA probes, and analyzed by gel shift The CCV1

cytoplasmic complexis indicated (C) The Balb/c 3T3 CCV1

com-plexes binding to the VEGF (V1) and IL-2 (V25) RNA probes (after

RNase T1 digestion) were exposed to UV light, in gel shift gels, to

cross-link proteins to RNA Cross-linked proteins were sized by SDS/

PAGE The sizes of cross-linked proteins were calculated by

subtrac-tion of molecular masses of bound RNA probes (D) Balb/c 3T3

fibroblast and Jurkat T cell cytoplasmic extracts were incubated with

labeled VEGF (V1) and IL-2 (V25) RNA probes, digested with RNase

T1 and analyzed in a gel shift assay The CCV1 cytoplasmic complexis

indicated (E) The Jurkat T cell CCV1 cytoplasmic complexbinding to

the IL-2 V25 RNA probe was analyzed by UV cross-link analysis as

described above The sizes of cross-linked proteins are indicated.

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antibody isotype control (Silensus, Boronia, Victoria,

Aus-tralia) were used as controls for the anti-PTB antibody in gel

shift assays and RNA immunoprecipitations, respectively

RNA gel shift analysis, competitions and antibody

analysis

RNA gel shifts were performed using 32P-labeled RNA

probes in a 10 lL reaction mixof 0.5· TM buffer [49–51]

containing 200 mMKCl, 1 lg poly(dI.dC), 100 ng tRNA,

1 lg bovine serum albumin and either 1 lg cytoplasmic

extract or 25 ng recombinant protein (dbpB or

GST-PTB) Reactions were incubated at 4C for 20 min,

followed by treatment with or without RNase T1

(Worth-ington Biochemical Corp., NJ, USA) and analyzed on

6% nondenaturing polyacrylamide gels Competition with

single-strand DNA oligonucleotides was performed by

addition of protein and 50 ng of unlabeled probe, followed

by immediate addition of the 32P-labeled RNA probe

Antibody blocking experiments were performed by

incuba-ting protein and antibody for 5 min before adding the

32P-labeled probe Antibodies did not degrade RNA probes

under the gel shift conditions used

UV cross-linking

Cytoplasmic extracts were bound to 32P-labeled RNA

probes in a 25 lL gel shift reaction and fractionated on a

6% polyacrylamide gel as described above The gel was

exposed to UV light (340 nm) for 15 min and retarded

complexes were excised after exposure overnight to X-ray

film Protein in excised bands was analyzed by 12% SDS/

PAGE as described previously [49–51]

RNA immunoprecipitation assay

Balb/c 3T3 fibroblast extracts were prepared, as described

above, in the presence of RNase inhibitors (Promega) and

incubated with or without anti-PTB monoclonal Ig or with

an IgG2 isotype control for 60 min RNase inhibitors were

required to prevent the loss of RNA from extracts Protein

A sepharose CL-4B (Pharmacia, Biosciences, Uppsala,

Sweden) was added and further incubated for 60 min

Sepharose was extracted for bound RNA (TRIzol

reagent, Invitrogen) RNA was reverse transcribed using

Superscript II (Promega) and a PCR assay for VEGF

cDNA was performed using oligonucleotides from the

mouse VEGF cDNA of 5¢-CACAGACTCGCGTTGCA-3¢

and 5¢-TGGGTGGGTGTGTCTAC-3¢ PCR products

were analyzed by agarose gel electrophoresis The VEGF

PCR product is approximately 400 bp

Cell culture, stable transfection and cell stimulation

Mouse Balb/c 3T3 fibroblasts and rat C6 glioma cells were

grown in Dulbecco’s modified Eagle’s medium with 10%

fetal bovine serum Jurkat T cells were cultured in RPMI

media with 10% fetal bovine serum For cytoplasmic

extracts, cells were grown in normoxic conditions (normal

oxygen; 20% O2) For the production of stably transfected

cell lines, C6 glioma cells were transfected with linearized

pfVEGF or pfVEGfdel plasmids using lipofectamineTM

2000 (Gibco BRL Life Technologies, Melbourne, Australia) according to the manufacturer’s directions Cells were grown for 24–48 h and selected in 400 lgÆmL)1G418 [15] Serum stimulation of stably transfected cell lines was as described previously [15] Hypoxic conditions (1% O2) were generated in a hypoxic chamber (Edwards Instrument Company, Sydney, Australia)

Analysis of mRNA stabilityin vivo Stable transfectants (pfVEGF or pfVEGFdel) were serum stimulated (time 0) and concurrently incubated under normoxic or hypoxic conditions for 1, 1.5, 2, 3 or 4 h Serum stimulation provides a brief pulse of transcription from the c-fos promoter in pfVEGF/pfVEGFdel con-structs, allowing subsequent degradation of the mRNA to

be monitored as previously described by us in analysis of the pfVEGF construct [15] This system allows determination

of mRNA stability directly, rather than using indirect means such as nonspecific inhibitors of transcription RNA was isolated from treated cells using TRIzolrreagent (Invitro-gen) according to the manufacturers instructions, and pfVEGF/pfVEGFdelmRNA was detected by RNase pro-tection analysis using a32P-labeled transcript covering the polylinker sequence in the pfVEGF/pfVEGFdel constructs

as previously described [15] Neomycin phosphotransferase (neo) mRNA expressed from pfVEGF/pfVEGFdel con-structs was detected as described [15] Protected RNAs were separated on denaturing polyacrylamide gels and the amounts of specific32P-labeled protected pfVEGF/pfVEGF-del or neo mRNAs were quantitated by PhosphoImager analysis (Molecular Dynamics, Sunnyvale, CA, USA) Levels of pfVEGF/pfVEGFdel mRNA (with time 0 levels subtracted) were normalized with respect to the levels of neo mRNA at each time point

Results

The VEGF 5¢-UTR binds cytoplasmic and recombinant CSD proteins

Sequence specific RNA binding sites for CSD proteins have been determined in a few genes but a consensus sequence has not been established Analysis of the prota-mine 1 (Prm1) 3¢-UTR has revealed a preferred binding site

of 5¢-U/C/A–C/A–C–A–U/C–C–A/C/U-3¢ for mouse CSD proteins [38–40] This sequence is consistent with a prefer-red sequence for Xenopus CSD proteins (FRGY1/2) of 5¢-AACAUCU-3¢ [61] and with a 5¢-ACCACC-3¢ sequence from the Rous Sarcoma virus LTR that binds chicken CSD proteins [41]

Given a potential role for CSD proteins in VEGF post-transcriptional regulation, the VEGF 5¢-UTR was exam-ined for CSD protein binding sites Two potential sites at +157 and +650 were observed These were named CSD site

1 and CSD site 2 and have sequences of 5¢-AACCU CU-3¢ and 5¢-AACUUCU-3¢, respectively (Fig 1A) No other potential CSD protein binding sequences were observed

To determine if the VEGF 5¢-UTR could bind cytoplas-mic CSD complexes,32P-labeled RNA probes 44 (+1 to +325) and 46 (+461 to +727) covering the potential CSD sites (Fig 1A) were bound to cytoplasmic extracts from

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Balb/c 3T3 fibroblasts and analyzed by gel shift assay

(Fig 1B) The 44 and 46 probes formed strong complexes

with cytoplasmic proteins (CC44a, b and CC46,

respect-ively) and these complexes were readily competed by a

single-strand DNA oligonucleotide (CSDwt) from the

GM-CSFgene that is known to bind CSD proteins [49,50] These

complexes were less readily competed by a mutant version

of the GM-CSF CSD oligonucleotide (CSDmut),

suggest-ing the presence of CSD proteins (Fig 1B) In support of

this, formation of complexes on the 44 RNA probe were

blocked by preincubation of extracts with increasing

amounts of an anti-CSD polyclonal Ig (CSD), whereas

preimmune serum (PI) had no effect (Fig 1C) Cytoplasmic

complexes containing CSD proteins can therefore bind the

VEGF 5¢-UTR

To further support a role for CSD proteins binding the

VEGF 5¢-UTR, it was observed that a recombinant CSD

protein GST-dbpB/YB-1 could bind to both the 44 and 46

RNA probes but not to a probe which does not contain

a potential CSD site (probe 47; +735 to +1014) The 47

probe contains sequences required for mouse VEGF IRES

activity [19,20] As for cytoplasmic complexes, GST-dbpB/

YB-1 binding was specifically competed by the CSD wt

oligonucleotide (Fig 1D) Both cytoplasmic and

recombin-ant CSD protein complexes are therefore forming on the

VEGF 5¢-UTR

The VEGF 5¢-UTR CSD-containing cytoplasmic complexes

also contain PTB

To localize the binding site for the major complexon the 44

RNA probe (CC44a), Balb/c 3T3 fibroblast cytoplasmic

extract was bound, in a gel shift assay, to a shorter

32P-labeled RNA probe, containing the proposed CSD

binding site 1 (V1; +150 to +185, Fig 2A) A single major

complex(CCV1) formed on the V1 probe and migrated in a

similar position to the CC44a complexon the 44 RNA

probe (Fig 2B) To verify that the CC44a and CCV1

complexes were the same, complexes were analyzed by UV

cross-linking (Fig 2C) The CC44a and CCV1 complexes,

that had been separated in a gel shift gel, were exposed

to UV light to cross-link proteins in complexes to their

respective RNA probes Cross-linked proteins were then

separated by SDS/PAGE and the sizes of cross-linked

proteins were calculated by subtraction of molecular masses

of bound RNA fragments The number and size of proteins

cross-linked to RNA was identical for the 44 and V1 RNA

probes We similarly found that the 46 RNA probe binding

complex(CC46), that contains the CSD site 2, gave an

identical cross-link pattern (data not shown)

As expected the CSD-containing cytoplasmic complexes

binding to the CSD site 1 (and CSD site 2) contained a

protein of 50 kDa, consistent with the size of the CSD

protein, dbpB (also known as YB-1/p50) [42] Additional

proteins in the complexhad sizes of 60, 27 and 12 kDa The

single CSD-containing cytoplasmic RNA/protein complex

therefore contains at least four different proteins It has been

reported that PTB, another single-strand RNA/DNA

binding protein [43–46,52–57] can bind to a 50 base region

spanning the CSD site 1 sequence in the human VEGF

5¢-UTR [21] Given that we have detected a 60 kDa protein

of the approximate size for PTB (57 kDa), we further

investigated the CSD site 1, CCV1 complex The presence of PTB protein in the CCV1 complexwas confirmed in a gel shift assay, by competition of the CCV1 complexwith an unlabeled single-strand DNA oligonucleotide probe from the transferrin gene (PTB wt), that binds PTB [52] The CCV1 complexwas not readily competed by a transferrin gene oligonucleotide with a mutant PTB site (PTB mut) (Fig 2D) We confirmed using recombinant proteins that the PTB wt oligonucleotide could not bind CSD proteins and hence was specific for PTB (data not shown) The presence of PTB was further confirmed by preincubation of cytoplasmic extract with an anti-PTB monoclonal Ig (PTB) before binding to V1 RNA probe in a gel shift assay The formation of the CCV1 complexwas blocked by the anti-PTB Ig (anti-PTB) but not by an irrelevant monoclonal antibody (anti-GMCSF; GM) (Fig 2E)

Taken together, this data demonstrates that the CSD-containing cytoplasmic complexforming on the VEGF 5¢-UTR contains PTB in addition to further unknown proteins of 27 and 12 kDa The ability of anti-CSD and PTB antibodies and DNA competitors to effectively compete complexformation demonstrates the dependence

on the presence of both CSD and PTB proteins to form the CCV1 complex

VEGF 5¢-UTR CCV1 complex formation requires the consensus 5¢-ACCUCUU-3¢ sequence and a downstream 5¢-UUUUCUU-3¢ sequence

To determine the sequences required for CCV1 complex formation on the VEGF 5¢-UTR CSD site 1 RNA probe (V1), Balb/c 3T3 fibroblast cytoplasmic extract was bound

to mutant versions of the V1 probe (Fig 3A) and analyzed

in a gel shift assay (Fig 3B) Mutations were made in the predicted CSD protein binding site, 5¢-ACCUCUU-3¢, and also in an adjacent sequence containing a potential PTB site 5¢-UUUUCUU-3¢ 5¢-UCUU-3¢ sequences flanked by pyrimidine residues are commonly found in PTB binding sites [52–55,57] Mutation of either sequence, by a block mutation (V37, V39) or by mutation of the central UC residues to AA (V15, V17) reduced CCV1 binding, suggesting a role for both sequences in complexformation Consistent with this, a double mutation (V19) abolished CCV1 complexformation (Fig 3B)

To investigate the individual roles CSD and PTB proteins may play in directing CCV1 complexbinding to the 5¢-ACCUCUU-3¢ and 5¢-UUUUCUU-3¢ sequences, recombinant CSD dbpB/YB-1) and PTB (GST-PTB) binding to wild-type (V1) and mutant (V37, V39) RNA probes was examined (Fig 3C) Consistent with CCV1, GST-dbpB/YB-1 binding was reduced by mutation

of both sites (V37, V39) whereas PTB binding was only slightly reduced by mutation of the 3¢-pyrimidine-rich sequence (V39) The presence of the adjacent poly U stretch may provide an alternative contact site for the recombinant PTB protein CSD proteins may play a larger role in directing CCV1 complexformation than PTB via their ability to bind both the predicted CSD site, 5¢-ACCUC UU-3¢, and the downstream 5¢-UUUUCUU-3¢ sequence required for CCV1 complexformation

To confirm that PTB-containing complexes can form on the VEGF mRNA in vivo an RNA immunoprecipitation

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assay was performed Cytoplasmic RNA/protein complexes

from Balb/c 3T3 fibroblasts were immunoprecipitated with

an anti-PTB monoclonal antibody and RNA extracted

from immunoprecipitated complexes was assayed by

RT-PCR for mouse VEGF mRNA sequences (Fig 3D)

Cytoplasmic extracts, for immunoprecipitation, were made

in the presence of RNase inhibitors to prevent RNA loss

VEGFmRNA was readily detected by RT-PCR in samples

immunoprecipitated with anti-PTB monoclonal Ig (PTB)

VEGFmRNA was not, however, detected in

immunopreci-pitations performed with an IgG2 monoclonal antibody

isotype control or without the addition of antibody (–)

An IL-2 5¢-UTR stability element binds the same

cytoplasmic complex as the VEGF 5¢-UTR

The IL-2 5¢-UTR contains sequences, at +1 to +22, that are

required for mRNA stabilization in T cells Both

dbpB/YB-1 and another RNA binding protein, nucleolin, bind to this

region and are involved in stabilization [31] Inspection of

the IL-2 5¢-UTR stability element revealed a sequence,

5¢-ACUCUCUU-3¢, at +4 to +11, that was very similar to

the VEGF CSD site 1 CSD consensus sequence (Fig 4A)

The ability of the IL-2 sequence to bind the CCV1 complex

was tested in a gel shift assay using Balb/c 3T3 fibroblast

cytoplasmic extract (Fig 4B) An RNA probe containing

the +1 to +35 IL-2 5¢-UTR sequences (V25) bound a

similarly migrating complexto that observed on the VEGF

V1 probe (CCV1), and this complexwas abolished by

mutation of the 5¢-ACUCUCUU-3¢ sequence (V27) The

V27 block mutation is reported to reduce IL-2 mRNA

stability in T cells [31] UV cross-link analysis of the IL-2

complexrevealed that it was identical to the VEGF 5¢-UTR

CCV1 complex(Fig 4C) An identical complexfrom

fibroblast extracts can therefore form on both the VEGF

and IL-2 genes

For the CCV1 complexto be of relevance to the

regulation of expression of the IL-2 gene, it was important

to determine if the complexcould be formed using T cell

extracts Binding of the IL-2 V25 probe to Jurkat T cell

cytoplasmic extracts revealed the formation of a complex

comigrating with the fibroblast CCV1 complex(Fig 4D)

UV cross-linking demonstrated that the fibroblast and

T-cell complexes were identical (Fig 4E) The CCV1

complextherefore forms on a functional element in the

IL-2 5¢-UTR in T cells

The VEGF 5¢-UTR CCV1 complex may be preformed

To determine if cytoplasmic CSD/PTB-containing VEGF

5¢-UTR complexes can form in the absence of RNA, Balb/c

3T3 fibroblast extract was fractionated by FPLC gel

filtration and the fractions incubated with wild-type (V1)

or mutant (V19; Fig 3) VEGF CSD site 1 RNA probes in a

gel shift assay (Fig 5) CCV1 complexformation, binding

to the V1 probe, was observed in fractions with an

approximate molecular mass range of 400–490 kDa

(frac-tions 6, 7) No other complexes were observed across the

range of fractions analyzed (from 10 to 1000 kDa) (data not

shown) CCV1 complexformation, in fractions 6 and 7, was

abolished by the V19 mutation, verifying the nature of these

complexes (Fig 5) These data indicate that the CCV1

complexis preformed in solution The presence of a higher order preformed complexsuggests the possibility that CSD and PTB may interact Consistent with this, CSD proteins have been shown to interact with a number of partner proteins in solution [22,23]

Involvement of the VEGF 3¢-UTR in binding CSD and PTB proteins

As sequences in the 3¢-UTR are also involved in post-transcriptional regulation of VEGF expression, the mouse VEGF 3¢-UTR [59] was examined for potential CSD protein binding sites A single site at +1727, relative to the stop codon at +1, was observed with a sequence of 5¢-AACAUCA-3¢ This sequence is an exact match to the preferred binding site for mouse CSD proteins [38,40] and,

as for the VEGF 5¢-UTR sites, has a potential PTB site, 5¢-UCUU-3¢, immediately downstream at +1736 (Fig 6A)

We used gel shift assays to examine whether a CSD/PTB complexbinds to this region in the 3¢-UTR An RNA probe (VC1) containing sequences +1712 to +1747 of the mouse VEGF 3¢-UTR was bound to Balb/c 3T3 fibroblast cytoplasmic extracts and two major complexes were observed The faster migrating complex(CCVC1) was competed more readily with wild-type (wt) than mutant (mut) PTB and CSD protein binding oligonucleotides, suggesting that this complexcontains PTB and CSD proteins (Fig 6B) As expected, mutation of either the potential CSD site (VC2) or the PTB site (VC3) reduced the formation of the CCVC1 complex(Fig 6C) Consistent with this, recombinant GST-PTB and GST-dbpB/YB-1 bound to the VC1 probe and PTB and CSD protein binding were reduced by mutations in the PTB (VC3) and CSD protein (VC2) binding sites, respectively As was observed for the 5¢-UTR, CSD binding was also reduced by mutation

of the potential PTB site (VC3) (Fig 6D)

Fig 5 Gel filtration fractionation of the VEGF 5¢-UTR CCV1 com-plex Balb/c 3T3 fibroblast cytoplasmic extract was fractionated by FPLC gel filtration and fractions assayed by incubation with labeled VEGF 5¢-UTR wild-type (V1) and mutant (V19) RNA probes in a gel shift assay Consecutive 0.5 mL fractions containing CCV1 binding activity are shown The approximate sizes of protein fractions, deter-mined by comparison to elution profiles of protein standards, is given

in kDa The CCV1 complexis indicated.

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Hence as for the 5¢-UTR, both the potential CSD and

PTB 3¢-UTR sites are required for cytoplasmic complex

(CCVC1) formation, with recombinant PTB primarily

contacting the downstream PTB site and CSD protein

contacting both sites

TheVEGF mRNA CSD/PTB binding sites play a role

inVEGF mRNA stability

The binding of common cytoplasmic complexes to the IL-2

5¢-UTR stability element and the VEGF CSD/PTB sites,

suggested a possible role for these sites in VEGF mRNA

stability CSD proteins have been shown to be involved in

both inducible mRNA stabilization, as is observed for the

IL-2 mRNA [31–33], and general mRNA stabilization

[34–37] PTB proteins may also play a role in general

mRNA stabilization [62]

To investigate a role for the VEGF mRNA CSD/PTB

sites, we analyzed the in vivo stability of mRNAs produced

from constructs containing tagged VEGF mRNA coding

Fig 6 CSD and PTB proteins bind to the VEGF 3¢-UTR (A)

Sequence of the VEGF 3¢-UTR CSD site 3 RNA probe (VC1) The

sequences represent +1712 to +1747 of the mouse VEGF 3¢-UTR,

relative to the stop codon at +1 [59] Consensus CSD and PTB binding

sequences are indicated CSD* indicates that recombinant CSD

pro-tein can also contact the PTB site Mutant RNA probe sequences

(VC2, VC3) are shown with only those bases that differ from the wild

type indicated RNA probes were generated from pGEMVC1, VC2

and VC3 constructs (B) Balb/c 3T3 fibroblast cytoplasmic extract was

incubated with wild-type and mutant CSD (CSDwt,mut) or PTB

(PTBwt,mut) binding site single-strand DNA competitors or left

untreated (–) Labeled VC1 probe was then immediately added and

complexes analyzed in a gel shift assay The CCVC1 complex and

unbound RNA probe are indicated (C) Cytoplasmic extracts were

incubated with VEGF 3¢-UTR wild-type (VC1) and mutant (VC2,

VC3) RNA probes and analyzed in a gel shift assay (D) Recombinant

GST-dbpB/YB-1 and GST-PTB were incubated with VEGF 3¢-UTR

wild-type (VC1) and mutant (VC2,VC3) RNA probes Recombinant

complexes are indicated.

Fig 7 Deletion of the VEGF CSD/PTB sites affects VEGF mRNA stability in normoxic and hypoxic conditions (A) Diagrammatic rep-resentation of the pfVEGF [15] and pfVEGFdel constructs The c-fos promoter and sequences encoding the mouse VEGF mRNA are indicated A poly linker is located between the protein coding and 3¢-UTR sequences as a tag for detection of pfVEGF and pfVEGFdel mRNA The sequences deleted from the CSD sites 1 (+156 to +179),

2 (+650 to +666) and 3 (+1727 to +1740) in the pfVEGFdel con-struct are indicated with dashes (B) Stable transfectants, containing pfVEGF or pfVEGFdel were serum stimulated at time 0 to induce a brief pulse of RNA expression from the c-fos promoter from which mRNA degradation can be followed [15] Cells were simultaneously treated (at time 0) under normoxic or hypoxic conditions and the levels

of pfVEGF/pfVEGfdel mRNA expressed from constructs determined

by RNase protection assay mRNA levels were normalized with respect to neo mRNA Serum stimulation increased transfected mRNA levels approximately 10-fold in both the pfVEGF and pfVEGFdel stable transfectants and was maximal at the 1 h time point The levels of pfVEGF and pfVEGFdel mRNAs were approxi-mately 1.7-fold the levels of endogenous VEGF mRNA in respective cell lines at this time (data not shown) The percentage mRNA remaining, relative to the mRNA levels at the 1 h time point (given as 100%), is shown as a linear plot for experiments performed under normoxic and hypoxic conditions Data is the average of five experi-ments RNase protection gel data is shown below the linear plot for one representative experiment Three repeats were performed for each time point The pfVEGF, pfVEGFdel and neo transcripts are indi-cated (C) Presentation of data in (B) as a log plot.

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sequences with either wild-type or deleted CSD/PTB sites

(pfVEGF and pfVEGFdel, respectively) (Fig 7A) We have

reported previously the use of pfVEGF in stabilization

experiments [15] pfVEGF or pfVEGFdel stable

transfect-ants were serum stimulated and simultaneously exposed to

hypoxic or normoxic conditions Transfected wild-type or

mutant VEGF mRNA levels were then assayed by RNase

protection assay at time intervals following serum

stimula-tion to determine the stability of respective mRNAs

(Fig 7B,C)

It can be seen in Fig 7(B,C) that degradation of the

wild-type VEGF mRNA (pfVEGF) occurs less rapidly than for

the mutant mRNA (pfVEGF del) under both normoxic and

hypoxic conditions, indicating that the CSD/PTB sites play

a role in stabilizing the VEGF mRNA in both noninduced

and hypoxia-induced conditions The wild-type pfVEGF

mRNA is 1.3-fold more stable than the CSD/PTB site

deleted mRNA Mutation of the CSD/PTB sites, however,

had no effect on the ability of hypoxia to increase mRNA

stability relative to that seen under normoxic conditions

Both wild-type and mutant VEGF mRNAs were stabilized

approximately 1.4-fold by hypoxia The VEGF CSD/PTB

sites therefore are not involved in induced stabilization in

response to hypoxia but appear to be involved in general

stabilization of the VEGF mRNA Interestingly the

pres-ence of the CSD/PTB sites confers a similar degree of

increased stability to the VEGF mRNA to that produced

under hypoxic conditions

Discussion

Inappropriate or inadequate expression of VEGF plays a

key role in the progression of a number of diseases [1–6] It is

therefore important to determine the processes involved in

regulation of VEGF expression We had previously shown

that cold shock domain (CSD) (or Y-box) proteins

regu-lated VEGF expression at the transcriptional level in the

nucleus [51] We show here that CSD proteins may also play

a role in post-transcriptional regulation of VEGF

expres-sion in the cytoplasm, in conjunction with another

single-strand RNA/DNA binding protein, PTB

Conserved CSD/PTB binding sites in theVEGF mRNA

5¢- and 3¢-UTR

The 5¢- and 3¢-UTR of the VEGF mRNA are involved in

post-transcriptional regulation [7,11–15,17,17–21] and we

have identified CSD/PTB protein binding sites in both

these regions Two sites were found in the 5¢-UTR (CSD

sites 1 and 2) and one site was found in the 3¢-UTR (CSD

site 3) (Fig 8A) All three sites contain a sequence that is

similar to a preferred RNA binding sequence determined

for the mouse CSD proteins MSY1, 2 and 4 [38–40] This

preferred sequence is consistent with the RNA binding

sites identified for chicken, frog and human CSD proteins

[31,41,47,61] (Fig 8B) The VEGF sequences all show a

substitution of the fourth position of the preferred mouse

sequence from an A to a C or U residue Potential PTB

binding sequences, 5¢-UCUU-3¢ (flanked by U/C residues)

[52–55,57], were located immediately downstream of the

consensus CSD sequences in both the 5¢- and 3¢-UTR

CSD/PTB sites An additional potential PTB site

over-lapped the consensus CSD sequence in the VEGF 5¢-UTR site 1 (Fig 8A)

Consistent with the presence of potential PTB binding sites, cytoplasmic complexes binding to the VEGF 5¢- and 3¢-UTR sites contained both CSD and PTB proteins and it was observed that both the consensus CSD sequence and the downstream PTB sequence, within these sites, were required for full complexformation The ability of both antibody and oligonucleotide competitors to reduce or abolish complexformation demonstrated that CSD and PTB proteins were simultaneously bound to VEGF RNA The ability of CSD and PTB proteins to bind to the 5¢- and 3¢-UTR sequences was further demonstrated by the binding

of recombinant PTB and dbpB/YB-1 CSD protein to these sites Importantly, we found that PTB-containing com-plexes could be detected on the VEGF mRNA in vivo PTB binding was primarily affected by the mutation of the downstream PTB consensus sequences, while surprisingly, recombinant CSD binding was affected by mutation of either the consensus CSD site or the downstream PTB sequence CSD proteins therefore recognize not only the expected consensus RNA sequence but also the VEGF PTB binding sequences The binding of CSD proteins to PTB

Fig 8 Comparison of CSD protein RNA binding sites (A) The sequences of the VEGF 5¢- and 3¢-UTR CSD site 1, 2 and 3 sequences are shown and consensus CSD (5¢) and PTB (3¢) protein binding sites are underlined Both sequences are required for cytoplasmic CSD/PTB complexformation and recombinant CSD protein binding (B) A comparison of CSD protein RNA binding sites is shown relative to a preferred sequence derived for the mouse MSY1/2/4 CSD proteins [38–40] Bases in binding sites that vary from this sequence are indi-cated in lower case The sequences are for chicken chkYB-1b/2 pro-teins [41], for Xenopus FRGY1/2 propro-teins derived using the selex procedure [61], for dbpB/YB-1 binding to CD44 pre-mRNA [47], dbpB/YB-1 binding to the IL-2 5¢-UTR [31] and the VEGF 5¢-UTR CSD site 1 MSY1, ChkYB-1b and FRGY1 are dbpB/YB-1 proteins MSY-4 and chkYB-2 are dbpA proteins, and MSY2 and FRGY2 are germ cell-specific CSD proteins.

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sequences has not previously been reported The ability of

CSD proteins to recognize both types of sequence suggests

that CSD proteins may direct formation of the CSD/PTB

cytoplasmic complexes on the VEGF 5¢-and 3¢-UTR

Functional role of VEGF CSD/PTB binding sites

The stability of VEGF mRNA is increased by stress

conditions such as hypoxia [7,11–14,17,18] in response to

a number of signaling pathways [12,14,16] Investigation of

stabilization mechanisms in noninduced or normoxic

con-ditions has not previously been reported Our data

presen-ted here suggests that the VEGF CSD/PTB sites may be

involved in such mechanisms We observed, that deletion of

the VEGF 5¢- and 3¢-UTR CSD/PTB site sequences, results

in reduced VEGF mRNA stability in both normoxic and

hypoxic conditions while the degree of stabilization of the

VEGFmRNA under hypoxic conditions was not affected

It appears therefore that CSD/PTB complexes may be

playing a general protective role for the VEGF mRNA in

normoxic growing cells, but that they are not involved in

increased stabilization in response to hypoxia Consistent

with this finding, CSD proteins have been shown to play a

role in both induced [31–33] and general [34–37] mRNA

stabilization Recent data suggests that PTB proteins may

also play a role in this latter type of mRNA stabilization

[62] Factors such as HuR and hnRNPL proteins, have been

implicated in VEGF mRNA stabilization through binding

to the 3¢-UTR, but this is the first report of identification of

potential post-transcriptional regulatory factors binding to

the VEGF 5¢-UTR [17,18] CSD and PTB proteins may

function to stabilize structures required to enhance mRNA

stability, as proposed for other post-transcriptional roles

mediated by CSD and PTB proteins [42,45] As the second

5¢-UTR CSD/PTB site is downstream of a reported

alternative transcription start site, the presence of two

CSD/PTB sites in the VEGF 5¢-UTR may be to ensure that

at least one of these sites will be present in alternative forms

of the VEGF mRNA [63]

Given that CSD and CSD-related proteins can play a role

in both cap-dependent [26,27,42] and IRES-driven

transla-tion [43–46] it is possible that the CSD/PTB sites play a role

in translation as well as stabilization of the VEGF mRNA

A combined role in mRNA stability and translation has

been observed for the YB-1 and MSY-2 CSD proteins

[35–37] Sequence-specific CSD binding sites involved in

translational regulation have been found in both 5¢- and

3¢-UTR sequences [38–41] PTB proteins are also involved

in translational regulation and it has been demonstrated

that PTB in combination with a CSD-related protein,

UNR, is involved in IRES function [43–46] The CSD/PTB

sites are, however, outside the regions defined for IRES

activity in the mouse and human VEGF 5¢-UTR sequences

[19–21], hence a cap-dependent translational role would be

more likely for the VEGF CSD/PTB binding regions

Higher order CSD/PTB complex formation

We have shown that the VEGF 5¢-UTR

CSD/PTB-containing complexes are multiprotein complexes

contain-ing proteins of the appropriate size for PTB (60 kDa), the

dbpB/YB-1 CSD protein (50 kDa) and two additional

smaller unidentified factors (27 and 12 kDa), giving a combined molecular mass  180 kDa DbpB/YB-1 (also called MSY-1, chkYb-1b, p50 and FRGY1) is one of two ubiquitously expressed CSD proteins The other being represented by dbpA (also called MSY-4, chkYB-2 and YB2/RYBa) [22–25,29] Both CSD and PTB proteins have been shown to functionally interact with a number of partner proteins e.g [23,43] but the dbpA or dbpB/YB-1 CSD proteins have not previously been reported to complex, or interact, with PTB Although not investigated here, a role for dbpA in the CSD/PTB complexes can not

be ruled out, as dbpA and dbpB/YB-1 have very similar functions [38–41] The large CSD-related UNR protein, with a size of 97 kDa is, however, unlikely to be part of the complex

Our data also demonstrates that the VEGF 5¢-UTR cytoplasmic CSD/PTB complexis preformed in solution This indicates that the preformed CSD/PTB complex, with

an approximate size of 400–490 kDa, may contain addi-tional proteins to those detected by UV cross-link analysis (the combined size of cross-linked components is only

180 kDa) Alternatively the 400–490 kDa complexmay contain two molecules of each protein identified by UV cross-linking This is likely as CSD and PTB proteins have

in fact been found to be able to bind to RNA and DNA as dimers as well as monomers [28,29,42,51,56]

Comparison of the sequence requirements for CSD/PTB complexformation with the binding of recombinant dbpB/ YB-1 and PTB, suggests that CSD proteins may direct the binding of the multiprotein complexto the VEGF RNA, as discussed above Consistent with this, using recombinant proteins, we have found that dbpB/YB-1 enhances the binding of PTB to VEGF RNA (M A Bartley & L S Cole, unpublished observation) Similarly the CSD-related protein, UNR, has been shown to direct the binding of PTB to IRES sequences [45] CSD proteins have also been shown to affect the ability of transcription factors to bind to DNA [23]

Broader role for CSD/PTB complexes in growth factor gene regulation

We found that the CSD/PTB complexes binding to the VEGF 5¢-UTR bound to similar sequences in the IL-2 5¢-UTR (Fig 8B) The IL-2 sequence that binds the CSD/ PTB complexhas previously been shown to be part of a stability element that responds to the JNK signaling pathway

in T cells [31] We confirmed that the CSD/PTB complexes could in fact form in T cells Both the dbpB/YB-1 CSD protein and another RNA binding protein, nucleolin, were found to be required for the induced IL-2 mRNA stabiliza-tion [31] It therefore appears likely that dbpB/YB-1 may be able to partner with multiple proteins on the IL-2 5¢-UTR stability element and that these complexes may respond to different signaling events or operate under different condi-tions The CSD/PTB complexes, for example, could be involved in general protection of the IL-2 mRNA until appropriate signaling pathways are activated, whereby CSD proteins could partner with nucleolin to bring about enhanced stabilization A similar mechanism could be occurring on the VEGF mRNA, where CSD/PTB complexes protecting VEGF mRNA under normal growing conditions

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