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Tiêu đề Insulin-like growth factor 1 signaling regulates cytosolic sialidase Neu2 expression during myoblast differentiation and hypertrophy
Tác giả Alessandro Fanzani, Francesca Colombo, Roberta Giuliani, Augusto Preti, Sergio Marchesini
Trường học University of Brescia, Department of Biomedical Sciences and Biotechnology, Unit of Biochemistry
Chuyên ngành Biomedical sciences and biotechnology
Thể loại Research article
Năm xuất bản 2006
Thành phố Brescia
Định dạng
Số trang 13
Dung lượng 0,93 MB

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sialidase Neu2 expression during myoblast differentiation and hypertrophy Alessandro Fanzani, Francesca Colombo, Roberta Giuliani, Augusto Preti and Sergio Marchesini Department of Biome

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sialidase Neu2 expression during myoblast differentiation and hypertrophy

Alessandro Fanzani, Francesca Colombo, Roberta Giuliani, Augusto Preti and Sergio Marchesini Department of Biomedical Sciences and Biotechnology, Unit of Biochemistry, University of Brescia, Italy

Skeletal muscle hypertrophy plays an important role

during postnatal development and occurs in response

to physical exercise [1], resulting in an increase in fiber

size accompanied by the increased expression of

insulin-like growth factor 1 (IGF-1) [2,3] Since IGF-1

overexpression in the skeletal muscle of transgenic

mice triggers an increase in muscle size [4–6], the emer-ging idea is that IGF-1 is sufficient to induce muscle hypertrophy Administration of IGF-1 to cultured muscle cells elicits a biphasic response, first promoting cell proliferation and then enhancing myogenic differ-entiation [7,8], reproducing the events occurring during

Keywords

AKT; IGF-1; myoblast; Neu2 sialidase;

gangliosides

Correspondence

A Fanzani, University of Brescia,

Department of Biomedical Sciences and

Biotechnology, viale Europa 11,

25123 Brescia, Italy

Fax: +39 030 3701157

Tel: +39 030 3717568

E-mail: fanzani@med.unibs.it

(Received 5 May 2006, revised 12 June

2006, accepted 13 June 2006)

doi:10.1111/j.1742-4658.2006.05380.x

Cytosolic sialidase (neuraminidase 2; Neu2) is an enzyme whose expression increases during myoblast differentiation Here we show that insulin-like growth factor 1 (IGF1)-induced hypertrophy of myoblasts notably increa-ses Neu2 synthesis by activation of the phosphatidylinositol 3-kinase/AKT/ mammalian target of rapamycin (P13K/AKT/mTOR) pathway, whereas the proliferative effect mediated by activation of the extracellular regulated kinase 1⁄ 2 (ERK1 ⁄ 2) pathway negatively contributed to Neu2 activity Accordingly, the differentiation L6MLC⁄ IGF-1 cell line, in which the forced postmitotic expression of insulin-like growth factor 1 stimulates a dramatic hypertrophy, was accompanied by a stronger Neu2 increase Indeed, the hypertrophy induced by transfection of a constitutively activa-ted form of AKT was able to induce high Neu2 activity in C2C12 cells, whereas the transfection of a kinase-inactive form of AKT prevented myo-tube formation, triggering Neu2 downregulation Neu2 expression was strictly correlated with IGF-1 signaling also in C2 myoblasts overexpressing the insulin-like growth factor 1 binding protein 5 and therefore not responding to endogenously produced insulin-like growth factor 1 Although Neu2-transfected myoblasts exhibited stronger differentiation, we demonstrated that Neu2 overexpression does not override the block of dif-ferentiation mediated by PI3 kinase and mTOR inhibitors Finally, Neu2 overexpression did not modify the ganglioside pattern of C2C12 cells, sug-gesting that glycoproteins might be the target of Neu2 activity Taken together, our data demonstrate that IGF-1-induced differentiation and hypertrophy are driven, at least in part, by Neu2 upregulation and further support the significant role of cytosolic sialidase in myoblasts

Abbreviations

AKT or PKB, protein kinase B; caAKT, constitutively active form of AKT; DM, differentiating medium; GM, growth medium; IGF-1, insulin-like growth factor 1; IGFBP5, insulin-like growth factor 1-binding protein; IRS-1, insulin receptor substrate 1; kiAKT, kinase-inactive form of AKT;

LY, LY294002; Neu2, neuraminidase 2; HS, horse serum; MAP kinase, mitogen-activated protein kinase; mTOR, mammalian target of rapamycin; PD, PD098059.

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the repair of damaged tissue In particular, myoblast

proliferation is triggered by activation of the

extra-cellular regulated kinase (ERK) pathway, whereas

myoblast hypertrophy occurs after activation of the

phosphatidylinositol 3-kinase (PI3K)–AKT pathway

[9,10] Another critical regulator of myoblast

hypertro-phy is mammalian target of rapamycin (mTOR)

[11,12], whose activation by AKT elicits the

phos-phorylation of two known regulators of protein

syn-thesis, P70S6K and the eukaryotic initiation factor

4E-binding protein PHAS-1 (PHAS/4EBP1) [13,14],

thereby promoting increased protein translation

Among the four forms of mammalian sialidases,

neuraminidase 2 (Neu2) (EC 3.2.1.18) is unique with

regard to cellular localization and tissue expression

Whereas the lysosomal form Neu1 [15–17], the

ganglio-side sialidase Neu3 [18] and the recently cloned Neu4

[19] are membrane-bound enzymes with broad tissue

expression, Neu2 has a cytosolic localization and its

expression is relatively high only in the skeletal muscle

[20] The involvement of Neu2 in myoblast

differenti-ation has been proposed for the first time using L6 rat

myoblasts [21]; in addition, we recently suggested a

cru-cial role for Neu2 in C2C12 myoblasts, demonstrating

its increase during myoblast differentiation and that its

overexpression enhances myotube formation [22]

The purpose of this work was to establish whether

IGF-1 is critical in myoblasts for Neu2 expression,

using pharmacologic inhibitors of the PI3K–AKT–

mTOR and ERK pathways and obtaining cells either

expressing the constitutively activated AKT or its

dominant negative form Neu2 expression was further

investigated using L6E9 myoblasts, in which forced

postmitotic expression of IGF-1 stimulates a dramatic

hypertrophy [23], and using C2 myoblasts

overexpress-ing IGF-bindoverexpress-ing protein-5 (IGFBP5), in which IGF-1

signaling is selectively repressed [24] Neu2

transfect-ants, characterized by enhanced differentiation, were

treated with inhibitors of the PI3 kinase–AKT–mTOR

pathway to evaluate the effects on myotube formation;

finally, parental and Neu2-transfected cells were

sub-jected to ganglioside analysis to determine whether the

endogenous sialidase activity was able to modify the

cellular content of sialolipids

Results

Neu2 expression increases during IGF-1-induced

hypertrophy of myoblasts

It is well known that IGF-1 is able to induce both

myoblast proliferation through the activation of the

Ras–Raf–Mek–Erk pathway and cell differentiation⁄

hypertrophy through activation of the PI3 kinase– AKT–mTOR pathway [9]

Accordingly, IGF-1 treatment (5 ngÆmL)1) of C2C12 myoblasts triggered the simultaneous phosphorylation

of ERK1⁄ 2 and AKT proteins (Fig 1A) Subsequently, AKT phosphorylation led to activation of mTOR, detected as phosphorylation of the downstream target p70S6K (Fig 1A) When we used pharmacologic inhib-itors to block selectively these pathways (Fig 1A), ERK1⁄ 2 phosphorylation was prevented in the pres-ence of 30 lm PD098059 (PD), whereas AKT phos-phorylation was blocked in the presence of 20 lm LY294002 (LY), a known inhibitor of PI3 kinase activ-ity In addition, the inhibition of mTOR activity was achieved in the presence of 5 ngÆmL)1 rapamycin, as revealed by the absence of the phosphorylated form of p70S6K As shown in Fig 1B, C2C12 cells grown in differentiating medium (DM) until day 5 fused into multinucleated myotubes, whereas the cells grown in

DM supplemented with IGF-1 (5 ngÆmL)1) developed a marked cell hypertrophy While simultaneous treatment with IGF-1 and PD did not change the rate of cell hypertrophy, myotube formation was completely pre-vented by treatment with LY The block of differenti-ation was obtained even in the presence of rapamycin (data not shown), an inhibitor of mTOR activity, con-firming the relevance of the PI3 kinase–AKT–mTOR pathway in this process The rate of cell hypertrophy was quantified by myotube diameter analysis (Fig 1B, right panel): in the presence of IGF-1 or IGF-1 supple-mented with PD, the average myotube diameter was about two-fold compared to parental cells differenti-ated in DM alone, whereas in the presence of LY no myotubes were observed

Under these experimental conditions, Neu2 expres-sion was investigated by RT-PCR analysis (Fig 1C) and enzymatic assay (Fig 1D) Neu2 transcript upreg-ulation was observed in myoblasts grown in the pres-ence of IGF-1 compared to DM alone, with the upregulation being reinforced in the presence of IGF-1 supplemented with PD In addition, treatment with LY

or rapamycin strongly repressed Neu2 transcription Accordingly, the enzymatic assay showed very low Neu2 activity in proliferating cells cultured in growth medium (GM), whereas myoblasts grown in DM exhibited high Neu2 activity Interestingly, a further increase of Neu2 activity was observed during myotube hypertrophy obtained in the presence of IGF-1; more-over, the effects of IGF-1 were considerably reinforced

in the presence of IGF-1 supplemented with PD, sug-gesting that ERK1⁄ 2 phosphorylation negatively con-tributes to Neu2 expression Finally, the treatments either with LY or rapamycin completely prevented

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A B

G F

H C

Fig 1 Insulin-like growth factor 1 (IGF-1)-induced hypertrophy enhances Neu2 expression in murine myoblasts (A) 5 ngÆmL)1IGF-1 induces phosphorylation of ERK1 ⁄ 2, AKT and p70S6K proteins ERK1 ⁄ 2 phosphorylation was prevented in the presence of 30 l M PD098059 (PD), AKT phosphorylation in the presence of 20 l M LY294002 (LY), and p70S6K phosphorylation in the presence of 5 ngÆmL)1rapamycin West-ern blots against total ERK1 ⁄ 2 and tubulin were performed to verify equal loading of protein samples (B) C2C12 myoblasts were grown for

6 days in the presence of the indicated treatments and subjected to Giemsa staining Mean myotube diameters are shown in a graph on the right and expressed in arbitrary units (n ¼ 10, *P < 0.05) (C) Neu2 transcript expression obtained by RT-PCR analysis in the presence of the indicated treatments until day 5 The data were normalized by loading the total RNA as control (D) Neu2 enzymatic assay performed using C2C12 cells cultured for 6 days in the presence of the indicated treatments (n ¼ 3, *P < 0.05) (E) Neu2 activity was evaluated in C2C12 cells cultured in differentiating medium (DM) until day 4 in the presence of two different concentrations of PD (10 and 30 l M ) alone

or supplemented with 5 ngÆmL)1IGF-1 (n ¼ 3, *P < 0.05) (F, G, H) Morphology (F), time-course of Neu2 enzymatic activity (G) and RT-PCR analysis of Neu2 transcript expression (H) obtained for L6MLC ⁄ IGF-1 cells compared to untreated and IGF-1-treated L6E9 cells (n ¼ 3,

*P < 0.05).

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Neu2 activity, suggesting that the PI3 kinase–AKT–

mTOR pathway is crucial for Neu2 expression

The effects of PD treatment on Neu2 activity were

further examined (Fig 1E); in particular, C2C12 cells

cultured in DM for 4 days in the presence of different

concentrations of PD (10–30 lm) showed an increase

of Neu2 activity compared to cells grown in DM

alone, suggesting that the lower PD concentration is

sufficient to inhibit the ERK1⁄ 2 phosphorylation

induced by endogenously secreted IGF-1 As

expec-ted, Neu2 activity further increased in the presence of

PD supplemented with exogenous IGF-1, with the

major effect obtained in the presence of 30 lm PD,

confirming that the higher Neu2 activity is achieved

only when the proliferative effect of IGF-1 is

neutral-ized To uncouple the proliferative effects of IGF-1

on muscle cells, we used L6MLC⁄ IGF-1 cells [23], a

myogenic cell line in which IGF-1 expression is forced

only after myoblast withdrawal from the cell cycle

and commitment to differentiation As shown in

Fig 1F, at day 6 L6MLC⁄ IGF-1 cells exhibited

pro-nounced myotube hypertrophy compared to L6E9

cells treated with IGF-1 (5 ngÆmL)1), whereas

untreated L6E9 cells exhibited a low rate of

differenti-ation Accordingly, hypertrophied L6MLC⁄ IGF-1

cells showed significantly higher Neu2 activity

com-pared to IGF-1-treated cells (Fig 1G) In particular,

L6MLC⁄ IGF-1 cells exhibited a peak of Neu2

enzy-matic activity at day 6 that correlated with a very

high degree of hypertrophy Indeed, the

transcrip-tional profile revealed a high level of Neu2 induction

in L6MLC⁄ IGF-1 cells compared to IGF-1-treated or

untreated cells (Fig 1H) These data strongly suggest

that the highest Neu2 expression is obtained when

IGF-1 fully exerts its myogenic effect without

stimula-ting cell proliferation

Constitutive AKT activation is per se sufficient

to drive Neu2 expression

It is well known that the expression of an AKT

activa-ted form is able to induce myoblast differentiation and

hypertrophy, mainly through the activation of mTOR

protein [11,12] To better characterize the signaling

pathway triggering Neu2 upregulation, C2C12 cells

were transfected using either the constitutively

activa-ted form of AKT (caAKT) or its kinase-inactive form

(kiAKT) [13]

After transfection, caAKT cells differentiated faster

than parental cells, developing hypertrophy as revealed

by morphology (Fig 2A) On the contrary, kiAKT

cells did not differentiate at all, as evidenced by the

weak positivity to myotube staining Myotube

dia-meter analysis (Fig 2A, right panel) confirmed the increase in fiber size of caAKT cells of about three-fold compared to parental cells, whereas kiAKT cells formed few myotubes with a reduced diameter As a consequence, stronger phosphorylation of AKT was observed in caAKT cells compared to parental cells, thus leading to enhanced phosphorylation of p70S6K (Fig 2B), whereas in kiAKT cells, activation of AKT and p70S6K was undetectable (Fig 2B) As shown in Fig 2C, a remarkable increase of Neu2 transcript was observed by RT-PCR analysis in caAKT cells com-pared to parental cells, whereas kiAKT cells exhibited reduced Neu2 expression In addition, caAKT myo-blasts revealed about a three-fold induction of Neu2 enzymatic activity compared to parental cells, whereas kiAKT cells exhibited very low Neu2 activity (Fig 2D) As caAKT cells treated with rapamycin did not exhibit Neu2 activity (data not shown), sustained activation of the AKT–mTOR pathway seems to be crucial for Neu2 expression

To determine whether IGF-1 was able to drive Neu2 expression through AKT-independent pathways, kiAKT cells were treated with IGF-1 and subjected to Neu2 activity analysis As shown in Fig 2E, IGF-1 treatment induced AKT phosphorylation in parental cells, whereas IGF-1-treated kiAKT cells showed a very low level of AKT phosphorylation; indeed, as shown in Fig 2F, Neu2 enzymatic activity was unde-tectable in kiAKT cells stimulated with IGF-1, whereas parental cells grown either in DM or in DM supplemented with IGF-1 exhibited Neu2 activity These data confirmed that Neu2 expression is depend-ent on AKT activation during IGF-1-induced differen-tiation of myoblasts

Neu2 expression is strictly dependent

on IGF-1 signaling

To establish whether Neu2 expression was strictly dependent on IGF-1 signaling, we used C2BP5 cells, a well-characterized cell model consisting of C2 myo-blasts overexpressing IGFBP5 and therefore not responding to endogenously produced IGF-1 [24] C2BP5 myoblasts failed to differentiate properly when grown in DM (Fig 3A), even in the presence of strong upregulation of endogenous IGF-1 transcript (Fig 3B) On the contrary, treatment of the cells with R3-IGF-1 (a mutated form of IGF-1 tat does not bind IGFBP5) was able to restore myotube formation (Fig 3A), as confirmed by strong expression of myo-genin (Fig 3C) In addition, as seen in C2C12 cells, simultaneous treatment with R3-IGF-1 and PD did not interfere with myoblast differentiation, whereas

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the treatments with LY completely prevented myotube

formation (Fig 3A) Thus, strong Neu2 transcript

upregulation was found to be strictly dependent on

the restoration of IGF-1 signaling (Fig 3D); in fact,

C2BP5 cells treated with increasing doses of R3-IGF-1

(15 and 30 ngÆmL)1) exhibited a proportional increase

of Neu2 expression, as revealed by RT-PCR ana-lysis Indeed, during the differentiation induced by R3-IGF-1 (30 ngÆmL)1), the Neu2 enzymatic activity increased approximately four-fold compared to cells

A

D

F

E

Fig 2 Neu2 upregulation is dependent on AKT activation (A) Parental C2C12 myoblasts, constitutively active AKT (caAKT) cells and kinase-inactive (kiAKT) cells were grown in differentiating medium (DM) for 48 h, and the myotubes were visualized by Giemsa staining Mean my-otube diameters are represented in the graph on the right and expressed in arbitrary units (n ¼ 10, *P < 0.05) (B) caAKT cells grown in DM for 48 h showed stronger phosphorylation of AKT and p70S6K compared to parental C2C12 cells, whereas phosphorylation was undetecta-ble in kiAKT cells Immunoblot analysis was performed using anti-phospho-AKT (Ser473) and anti-phospho-P70S6K (Thr389) The data were normalized using tubulin as control (C) Neu2 transcript upregulation is dependent on AKT activity Neu2 transcript analysis was performed

by semiquantitative RT-PCR, using cells grown for 48 h in DM, and the data were normalized by loading the total RNA as control (D) Neu2 enzymatic assay performed on parental, caAKT and kiAKT cells grown for 48 h in DM (n ¼ 3, *P < 0.05) (E) Immunoblot analysis against the phospho-AKT form (Ser473) was performed on untreated C2C12 cells and on parental and kiAKT cells treated with insulin-like growth factor 1 (IGF-1) for 15 min The data were normalized using tubulin as control (F) Neu2 enzymatic activity of kiAKT cells treated until day 5 with IGF-1 and compared to C2C12 cells grown either in DM or in DM supplemented with IGF-1 (n ¼ 3, *P < 0.05).

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grown in DM (Fig 3E) As seen in C2C12 cells,

treat-ment with R3-IGF-1 and PD significantly enhanced

Neu2 activity compared to IGF-1 treatment alone,

whereas in the presence of R3-IGF-1, supplemented

with either LY or rapamycin, Neu2 expression was

completely prevented

PI3 kinase and mTOR inhibitors block the

enhanced differentiation of Neu2-overexpressing

cells

We previously reported that Neu2 overexpression

enhances myoblast differentiation of C2C12 cells,

trig-gering marked cell hypertrophy [22] In order to show

whether C2C12 myoblasts transfected with rat Neu2

cDNA (Fig 4A) could override the pharmacologic

inhibition of differentiation, untreated or

IGF-1-trea-ted Neu2 clones were added with either LY or

rapa-mycin (Fig 4B) After 48 h in DM, Neu2 clones

developed an elongated shape and a pronounced

ten-dency to form myotubes; in the same manner, the

clones that were treated with IGF-1 showed a similar

morphology, except that there were many proliferating cells The treatment of Neu2-transfected cells with either LY or rapamycin prevented myotube formation also in presence of IGF-1, suggesting that Neu2 over-expression cannot override LY⁄ rapamycin inhibition

of differentiation

Neu2 overexpression does not affect the ganglioside pattern in C2C12 myoblasts Although the ability of Neu2 to hydrolyze gangliosides

in vitro has been reported [25], the target of Neu2 activity during myoblast differentiation is still unknown To investigate this, we used Neu2 clones to evaluate possible modifications of the ganglioside pat-tern (Fig 4C) Surprisingly, both transfected and par-ental cell lines exhibited a similar pattern, with GM3 ganglioside as a major component, and GM2 and GD1a gangliosides present in lower amounts In addi-tion, C2C12 myoblasts were grown in the presence of

a selective inhibitor of ganglioside biosynthesis, P4 [26], and characterized for their proliferation and

A

B

C

E D

Fig 3 Neu2 expression is strictly depend-ent on insulin-like growth factor 1 (IGF-1) signaling (A) C2BP5 cells were grown after confluence until day 4 in differentiating med-ium (DM) or DM supplemented with

15 ngÆmL)1R3-IGF-1 with or without 10 l M PD098059 (PD) or 20 l M LY294002 (LY) The cells were visualized by Giemsa stain-ing (B) RT-PCR analysis of endogenous IGF-1 transcript in C2BP5 cells grown in DM for 48 h (C) Western blot analysis of myogenin in C2BP5 cells cultured for 48 h

in growth medium (GM), DM or DM supple-mented with 15 ngÆmL)1R3-IGF-1 (D) RT-PCR analysis of Neu2 transcript in C2BP5 cells grown for 72 h in DM or DM supple-mented with two different concentrations of R3-IGF-1 The data were normalized by load-ing the total RNA as control (E) Neu2 enzy-matic activity was detected in C2BP5 cells only when R3-IGF-1 was added to restore myotube formation The enzymatic assays were performed using cells grown for 96 h

in DM with R3-IGF-1 (30 ngÆmL)1) alone or supplemented with 30 l M PD, 20 l M LY, or

5 ngÆmL)1rapamycin (n ¼ 3, *P < 0.05).

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A B

C

E

D

Fig 4 Neu2-induced differentiation is blocked by PI3 kinase and mammalian target of rapamycin (mTOR) inhibitors, and Neu2 overexpres-sion does not affect the ganglioside pattern of C2C12 myoblasts (A) C2C12 cells were stably transfected with a vector harboring the rat Neu2 cDNA and tested for Neu2 transcript expression and for the increase of sialidase activity compared to untransfected cells (B) Neu2-overexpressing clones grown for 48 h in differentiating medium (DM) or DM supplemented with insulin-like growth factor 1 (IGF-1) were treated with either LY294002 (LY) or rapamycin and analyzed by Giemsa staining for their morphology (C) Ganglioside pattern obtained by TLC analysis Gangliosides were visualized in parental C2C12 cells and in C2C12 cells overexpressing Neu2 sialidase In addition, the ganglio-sides were undetectable in myoblasts after treatment with P4, a synthetic inhibitor of glycosphingolipid biosynthesis (D) C2C12 cells were treated with P4 and then subjected to [ 3 H]thymidine incorporation to quantify the rate of proliferation (n ¼ 3, *P < 0.05) (E) morphology of C2C12 cells and Neu2-overexpressing clones, differentiated in either DM or DM supplemented with P4 until day 5 Mean myotube diame-ters are represented in a graph on the right and expressed in arbitrary units (n ¼ 10, *P < 0.05).

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differentiation rate As shown in Fig 4C, gangliosides

were undetectable in myoblasts incubated for 72 h in

the presence of P4 Under these conditions,

prolifer-ation rate was decreased about two-fold compared to

untreated myoblasts, as revealed by thymidine

incor-poration (Fig 4D) However, myoblasts grown in the

presence of P4 retained the capacity to differentiate,

and Neu2-overexpressing cells exhibited stronger

myo-tube formation compared to parental cells, even when

treated with P4 (Fig 4E), as confirmed by myotube

diameter analysis (right panel) These data suggest that

different substrates, such as sialoglycoproteins, could

be the target of Neu2 enzymatic activity in myoblasts

Discussion

The current study establishes for the first time that

Neu2 expression is strictly dependent on IGF-1

signa-ling in myoblasts IGFs (IGF-1 and IGF-2) are

syn-thesized primarily in the liver, but are also produced

locally in tissues, including skeletal muscle, where they

can exert autocrine or paracrine effects [27] In

partic-ular, whereas IGF-2 appears to play a mitogenic role

primarily during embryogenesis and regeneration

[28,29], IGF-1 has been reported to be essential for

muscle differentiation and hypertrophy [1–3] Unlike

other growth factors, IGF-1 is able to exert pleiotropic

effects on muscle cells, first supporting myoblast

repli-cation through mitogen-activated protein (MAP)

kin-ase activation, and subsequently promoting myogenic

differentiation through the PI3 kinase–AKT pathway

The data presented here demonstrate that the signaling triggered by IGF-1 modulates Neu2 expression in myo-blasts We were able to dissect the contribution of the IGF-1-induced pathways to Neu2 expression (Fig 5);

in particular, the highest Neu2 activity was obtained

by IGF-1 treatment with concomitant inhibition of ERK1⁄ 2 phosphorylation, suggesting that this path-way contributes to Neu2 downregulation, whereas activation of the PI3 kinase–AKT–mTOR pathway sti-mulated strong Neu2 upregulation

When we measured Neu2 activity in L6MLC⁄ IGF-1 cells, we found a stronger increase of Neu2 enzymatic activity compared to parental L6E9 cells treated with exogenous IGF-1 Thus, Neu2 is highly expressed only when IGF-1 exerts its myogenic effect after myoblast withdrawal from the cell cycle and commitment to dif-ferentiation These observations suggest that during IGF-1-induced regeneration of muscle cells following myofiber injury, the largest contribution of Neu2 activ-ity might be related to the postmitotic effects of IGF-1 after cell migration, presumably during the formation

of new fibers We next examined the contribution of AKT to Neu2 expression The activation of AKT has been extensively suggested as a key event in myoblast differentiation and hypertrophy [14,30,31] For exam-ple, AKT is able to promote increased protein syn-thesis by direct activation of p70S6K and PHAS-1⁄ 4E-BP1 through mTOR [13,14,32,33] or through inhi-bition of mTOR-independent targets such as glycogen synthase kinase 3b [13,34] Here we show a dramatic increase of Neu2 activity during C2C12 cell hypertro-phy induced by transfection of a constitutively active form of AKT On the contrary, the transfection of its kinase-inactive form almost completely prevented Neu2 activity, also after treatment with IGF-1, sug-gesting that AKT is a key regulator of Neu2 expres-sion Interestingly, when we used rapamycin to block mTOR activity in myoblasts overexpressing the active form of AKT, complete suppression of Neu2 synthesis was observed, suggesting that Neu2 expression is com-pletely dependent on mTOR activity To determine whether Neu2 regulation was strictly dependent on IGF-1 signaling, we used C2 myoblasts stably trans-fected with IGFBP5 [35]; these cells, unable to differ-entiate properly in response to endogenous secreted IGF-1 [23], exhibited Neu2 enzymatic activity only when myotube formation was restored by addition of the analogous form R3-IGF-1, thus confirming that Neu2 expression is dependent on IGF-1 signaling Although Neu2 overexpression was able to enhance myotube formation in C2C12 cells, treatment of Neu2 transfectants with inhibitors of PI3 kinase and mTOR proteins prevented myotube formation, suggesting that

IGF-1 receptor

myoblast plasma membrane

Differentiation Hypertrophy

Neu2 up-regulation Neu2 down-regulation

Proliferation

myotube formation

p70s6k mTOR AKT P13-k IRS-1 Ras Raf

Mek

Erk1/2

Fig 5 Intracellular signaling pathways regulating Neu2 expression

in myoblasts Insulin-like growth factor 1 (IGF-1) receptor

autop-hosphorylation activates, through insulin receptor substrate 1 (IRS-1)

recruitment, different downstream signals, triggering both myoblast

proliferation and differentiation ⁄ hypertrophy In particular, activation

of the Ras–Raf–Mek–Erk pathway stimulates proliferation,

contribu-ting to Neu2 downregulation On the contrary, activation of the

PI3K–AKT–mTOR–P70S6K pathway leads to myoblast differentiation

and hypertrophy, inducing strong Neu2 expression, which could play

a crucial role during myotube formation.

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Neu2 overexpression cannot override LY⁄ rapamycin

inhibition of differentiation

Taken together, our data suggest that

IGF-1-induced differentiation and hypertrophy are associated

with Neu2 upregulation, supporting the idea that the

presence of a cytosolic sialidase is significant during

myotube formation In accord with this hypothesis, it

has been reported that the inhibition of Neu2

transla-tion by additransla-tion of antisense oligonucleotides strongly

decreases myotube formation in L6 rat myoblasts [21]

The ability of sialidases to work on glycoconjugates

has been long known, suggesting that modulation of

these substrates is a crucial step in physiologic and

pathologic states [36,37] Despite the reported Neu2

ability to hydrolyze gangliosides and glycoproteins

in vitro [25], the target of this enzyme in myoblasts is

still unknown It has been previously reported that

Neu2 transfection decreases GM3 ganglioside in B16

melanoma cells, diminishing invasiveness and cell

motility [38], whereas transfection in human carcinoma

epidermoid A431 cells led to increased epidermal

growth factor receptor autophosphorylation and cell

proliferation caused by the decrease in GM3 [39]

According to these observations, we sought to

deter-mine whether Neu2 overexpression could modify the

ganglioside pattern in C2C12 cells Surprisingly, no

differences were found in ganglioside pattern between

parental and transfected cells, in particular with regard

to GM3 ganglioside A decrease in GM3 was observed

during C2C12 differentiation (data not shown), but

even in this case we did not detect differences

com-pared to Neu2 transfectants As the inhibition of

gan-glioside biosynthesis significantly decreased the

proliferation rate of myoblasts, thus leading to

differ-entiation, the reduction of ganglioside content could

play a prodifferentiating role in myoblasts It is

poss-ible that local modulation of some gangliosides could

be important for myoblast differentiation, but in our

experimental conditions we were unable to detect

even-tual differences due to Neu2 activity However, we

cannot rule out the possibility that Neu2 activity could

be restricted to glycosphingolipids associated with the

cytoskeleton [40,41] or soluble and organelle

mem-brane-bound gangliosides [42,43], thus rendering the

analysis quite difficult Interestingly, Neu2 trasfectants

maintained the ability to enhance myotube formation

even during the inhibition of ganglioside biosynthesis,

suggesting that different substrates, such as

glycopro-teins, could be a potential target for Neu2 in

myo-blasts The ability of the Neu2 enzyme to hydrolyze

a2,3-sialylglycoproteins has been reported, suggesting a

potential role in the turnover of glycoproteins resident

in the cytosolic compartment Interestingly, a cytosolic

N-glycanase has been found to release free glycans from asparagine-linked glycopeptides exported out of the endoplasmic reticulum to the cytosol [44,45] In this context, cytosolic glycans may be substrates for Neu2 activity In addition, there is a recent report of a dramatic increase of recombinant Neu2 enzymatic activity in the presence of Ca2+ [46] As Ca2+ has a crucial role in correct myoblast differentiation, it is likely that local variations in Ca2+ concentration enhance Neu2 enzymatic activity in the cytosolic com-partment

Finally, since IGF signaling plays a crucial role in the physiologic and pathologic states of the muscle [47], it is of interest to establish whether Neu2 impair-ment occurs during atrophy caused by muscle diseases

A recent paper, in fact, describes the downregulation

of sialidase Neu2 in a mouse model of human dysfer-linopathy [48,49], indicating that altered Neu2 expres-sion may impair muscle regeneration In concluexpres-sion, our data shed new light on the mechanisms triggering the increase of cytosolic sialidase expression during myoblast differentiation and hypertrophy, and suggest that further investigations would be useful to elucidate the target of Neu2 activity in muscle cells

Experimental procedures

Cell lines

The mouse C2C12 myoblasts maintained at subconfluent density at 37C in 5% CO2 were cultured in DMEM high glucose (Sigma-Aldrich, Milan, Italy) supplemented

100 lgÆmL)1 penicillin⁄ streptomycin antibiotic (Sigma-Aldrich), defined as growth medium (GM) Confluent cells were transferred to DM containing DMEM supplemented with 2% horse serum (HS) and the medium was changed every day To induce myoblast hypertrophy, C2C12 cells were grown in DM, and 72 h postconfluence 5 ngÆmL)1 IGF-1 (Sigma-Aldrich) was added in order to stimulate myotube formation

The L6E9 line is a subclone of the parental rat neonatal myogenic line that does not express IGF-1 but that has IGF-1 receptors L6E9 cells were maintained in GM consist-ing of DMEM supplemented with 20% fetal bovine serum, and differentiated at 80% confluence either in DM consist-ing of DMEM supplemented with 1% fetal bovine serum or

in DM supplemented with 5 ngÆmL)1 IGF-1 L6MLC⁄ IGF-1 cells are L6E9 cells stably transfected with a vector harboring a muscle-specific IGF-1 [23], whose expression is activated by myosin light chain promoter only after myo-blasts have withdrawn from the cell cycle and have commit-ted to differentiation Hypertrophy of L6MLC⁄ IGF-1 cells was achieved by growing the cells in DM alone

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C2BP5 cells were cultured according to previously

described conditions [24] in the presence of G418

(400 lgÆmL)1) C2BP5 cells are C2 myoblasts stably

trans-fected with mouse insulin-like growth factor 1 binding

pro-tein-5 cDNA, which renders the cells unresponsive to

endogenous IGF-1 These cells undergo minimal

differenti-ation without the inclusion of exogenous R3-IGF-1, an

IGF-1 analog lacking the IGFBP-binding region and

there-fore able to induce differentiation Pharmacologic

treat-ments of myoblasts were performed using 10–30 lm

PD098059 (Sigma) to inhibit ERK1⁄ 2 phosphorylation,

20 lm LY294002 (Sigma) to inhibit PI3 kinase activity, and

5 ngÆmL)1rapamycin (Sigma) to inhibit mTOR activity

To visualize myotubular structures, cells were washed

three times in NaCl⁄ Pi before fixing for 10 min in 100%

methanol at) 20 C Cells were stained with Giemsa

react-ive (Sigma-Aldrich) for 2–3 h and again washed in

NaCl⁄ Pi To quantify the myotube diameter in

differenti-ating myoblasts, 10 fields were chosen randomly and 10

myotubes were measured per field The average diameter

per myotube was the mean of 10 mesurements taken along

the length of the myotube

Stable transfections

To obtain Neu2 transfectants, C2C12 myoblasts were

trans-fected with a pCDNA expression vector harboring the rat

Neu2 cDNA using Lipofectamine 2000 reagent (Invitrogen,

Milan, Italy) according to the manufacturer’s instructions;

the cells were cloned after 10–15 days of selection in G418

antibiotic (0.5 mgÆmL)1, Promega, Milan, Italy) and used

for a few passages To obtain C2C12 myoblasts expressing

either a constitutive active form of AKT or its dominant

negative form, the cells were transfected using a pBABE

vector in which a myristoylated AKT or a kinase-inactive

AKT mutated at the ATP-binding site (K179M) were

cloned [13] After transfection by Lipofectamine 2000

rea-gent, the mix of stable transfectants was obtained after

10 days of selection in puromycin antibiotic (2 lgÆmL)1,

Sigma) and used for a few passages

RNA extraction and RT-PCR analysis

Total RNA was obtained by Tri-reagent extraction (Sigma)

The pellet of RNA was resuspended in RNase-free water,

and digested with 1 unit of DNAase (DNA-free; Ambion,

Huntingdon, UK) for 1 h at 37C, according to the

manu-facturer’s instructions Two micrograms of total RNA was

retrotranscribed with 400 units of MMLV-RT (Promega)

for 1 h at 37C, and the RT template was used for PCR

amplification

For RT-PCR analysis of murine cytosolic Neu2 sialidase

expression, primers 5¢-CGAGCCAGCAAGACGGATGA

G-3¢ (sense) and 5¢-GGCTCTACAAGCTTACTCACTAC

CCGG-3¢ (antisense) were used, and the amplified products

were normalized by loading an equal amount of extracted RNA for each sample For the screening of Neu2 transfect-ants, PCR analysis was performed using the primers for the rat Neu2 cDNA in order to avoid amplification of the endogenous murine Neu2 mRNA, as previously described [22] For RT-PCR analysis of rat cytosolic Neu2, primers 5¢-CCGTCCAGGACCTCACAGAG-3¢ (sense) and 5¢-TC ACTGAGCACCATGTACTG-3¢ (antisense) were used

Sialidase assay

A confluent 100 mm plate was washed with NaCl⁄ Pi, and the cells harvested in 350 lL of 0.25 m sucrose⁄ 1 mm EDTA containing a mix of protease inhibitors (Complete Mini Pro-tease Inhibitors; Roche Molecular Biochemicals, Monza, Italy) were then sonicated at 4C for 10 s The mixture was centrifuged at 600 g (Heraeus Megafuge 1.0R, DJB Labcare Ltd., Newport Pagnell, UK) for 10 min at 4C, and the supernatant was ultracentrifuged at 105 000 g (Beckmann Coulter L80 S.p.A., Milan, Italy) for 60 min at 4C The supernatant was used as the cytosolic fraction and assayed for sialidase activity The assay mixture contained 60 nmol

of the substrate 4-methylumbelliferyl N-acetylneuraminic acid (Sigma-Aldrich), 100 lg of BSA and aliquots of cytoso-lic fractions (50–100 lg of proteins) in a final volume of 0.2 mL of 50 mm sodium acetate buffer (pH 5.8) After incu-bation at 37C for 3 h, the reaction was terminated by addi-tion of 0.8 mL of 0.25 m glycine buffer (pH 10.4), and the amount of 4-methylumbelliferone released was determined fluorometrically with an excitation wavelength of 365 nm and an emission wavelength of 450 nm

Western blot analysis

Myoblast cells were harvested at 4C in RIPA lysis buffer (1% Nonidet P40, 0.5% sodium deoxycholate, 0.1% SDS

in 50 mm NaCl, 20 mm Tris⁄ HCl, pH 7.6) containing a mix of protease inhibitors Lysates were cleared by centrifu-gation at 12 000 g (Heraeus Megafuge 1.0R) for 15 min at

4C before determination of protein concentration by bi-cinchoninic acid assay (Pierce, Celbio SRL, Milan, Italy) SDS⁄ PAGE was performed on 10% acrylamide gel West-ern blots were visualized by enhanced chemiluminescence (Chemicon Ltd., Chandlers Ford, UK) For the detection

of phosphorylated ERK1⁄ 2, a mouse monoclonal antibody was used (clone E-4; Santa Cruz Biotechnology, Santa Cruz, CA, USA) A polyclonal antibody against ERK1⁄ 2 was used for the detection of total ERK1⁄ 2 (Santa Cruz

(Ser473) and P70S6K (Thr389) were detected using rabbit polyclonal antibodies (Cell Signalling Ltd., Hitchin, UK) The detection of myogenin was performed using a mouse monoclonal antibody (clone F5-D; Santa Cruz Biotechno-logy) An antibody against a-tubulin (Sigma) was used to normalize the loading in the different western blots

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