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Tiêu đề Bioimaging of the unbalanced expression of microRNA9 and microRNA9* during the neuronal differentiation of P19 cells
Tác giả Mee Hyang Ko, Soonhag Kim, Do Won Hwang, Hae Young Ko, Young Ha Kim, Dong Soo Lee
Trường học Seoul National University College of Medicine
Chuyên ngành Neuroscience
Thể loại Research article
Năm xuất bản 2008
Thành phố Seoul
Định dạng
Số trang 12
Dung lượng 669,97 KB

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Nội dung

In this study, real-time PCR analysis and in vitro⁄ in vivo bioluminescent imaging demon-strated that the upstream region of a primary miR9-1 pri-miR9-1 can be used to monitor the highly

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and microRNA9* during the neuronal differentiation of

P19 cells

Mee Hyang Ko1,2,3, Soonhag Kim2,4,*, Do Won Hwang1,2,3, Hae Young Ko2,3, Young Ha Kim2,3and Dong Soo Lee2,4,*

1 Programs in Neuroscience, Seoul National University, Korea

2 Department of Nuclear Medicine, Seoul National University College of Medicine, Korea

3 Laboratory of Molecular Imaging and Therapy of Cancer Research Institute, Seoul National University College of Medicine, Korea

4 Medical Research Center, Seoul National University College of Medicine, Korea

MicroRNAs (miRs) are a class of small non-coding

RNA molecules, encoded as short inverted repeats in

the genomes of plants and animals miRs are believed

to modulate the post-transcriptional regulations of

their targets in diverse biological regulatory systems

including cellular development [1,2], cell differentiation [3], fat metabolism [4], cell proliferation and cell death [5] Hundreds of miRs have been isolated from mam-malian species and a dozen of these, including miR124a, miR9, miR128, miR131, miR178 and

Keywords

bioimaging; Luciferase; microRNA;

microRNA9 and microRNA9*; neurogenesis

Correspondence

S Kim, Department of Nuclear Medicine,

Medical Research Center, Seoul National

University College of Medicine, 28

Yongon-dong, Jongno-gu, Seoul 110 744, Korea

Fax: +82 2 3668 7090

Tel: +82 2 3668 7028

E-mail: kimsoonhag@empal.com

D S Lee, Department of Nuclear Medicine,

Medical Research Center, Seoul National

University College of Medicine, 28

Yongon-dong, Jongno-gu, Seoul 110 744, Korea

Fax: +82 2 3668 7090

Tel: +82 2 2072 2501

E-mail: dsl@plaza.snu.ac.kr

*These authors contributed equally to this

work

(Received 18 January 2008, revised 10

March 2008, accepted 17 March 2008)

doi:10.1111/j.1742-4658.2008.06408.x

Generally, the 3¢-end of the duplex microRNA (miR) precursor (pre-miR)

is known to be stable in vivo and serve as a mature form of miR However, both the 3¢-end (miR9) and 5¢-end (miR9*) of a brain-specific miR9 have been shown to function biologically in brain development In this study, real-time PCR analysis and in vitro⁄ in vivo bioluminescent imaging demon-strated that the upstream region of a primary miR9-1 (pri-miR9-1) can be used to monitor the highly expressed pattern of endogenous pri-miR9-1 during neurogenesis, and that the Luciferase reporter gene can image the unequal expression patterns of miR9 and miR9* seen during the neuronal differentiation of P19 cells This demonstrates that our bioimaging system can be used to study the participation of miRs in the regulation of neur-onal differentiation

Abbreviations

Dicer, RNase III endonuclease; FLuc, Firefly Luciferase; GLuc, Gaussia Luciferase; miR, microRNA; miR9*, microRNA9*, 5¢-end of pre-miR9; miR9, microRNA9, 3¢-end of miR9 precursor; piRNA, Piwi-interacting RNA; pre-miR, precursor microRNA; pre-miR9, miR9 precursor or precursor miR9; pri-miR9-1, primary miR9-1; ROI, region of interest analysis.

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miR125b, have been found to be associated with

polyr-ibosomes in primary neurons [6,7] These studies have

shown that both microRNA9 [miR9, 3¢-end of miR9

precursor (pre-miR9)] and microRNA9* (miR9*,

5¢-end of pre-miR9) originate from the hairpin-loop

structure of the same pre-miR9, and are highly

co-expressed and neuron-specific during brain

devel-opment

In general, intergenic or intragenic miRs are

tran-scribed into primary miRNA (pri-miR) by RNA

polymerase II and processed into a 70-nucleotide

hair-pin-structured pre-miR in the nucleus by Drosha

[8–10] Pre-miRs are transported to the cytoplasm by

exportin-5 (a member of the Ran transport receptor

family) and another factor Ran [11] Pre-miR hairpin

is further processed into a 19- to 23-nucleotide

single-stranded mature miR by RNase III endonuclease

(Dicer) [12] During Dicer cleavage, duplex pre-miRs

are uncoiled by helicase into two single strands,

mature miR (from the 3¢-end of duplex pre-miR) or

miR* (opposite strand, from the 5¢-end of duplex

pre-miR), although miR* is generally rapidly

degraded by an unknown enzyme nuclease [13]

Mature miRs are then incorporated into the

RNA-induced silencing complex and bound to the 3¢-UTR

of its target mRNA to induce either mRNA

degrada-tion or transladegrada-tional inhibidegrada-tion [2,14,15] Interestingly,

unlike most miRs, which have a single mature miR,

miR cloning and sequencing from the human and

miRNAMap database (http://mirnamap.mbc.nctu

edu.tw) showed that a few miRs, including miR302b,

miR302c, miR373 and miR9, have two types of

mature form, miR and miR* [16,17] This is similar

to the final functional forms of Piwi-interacting RNA

(piRNA), which are also small RNA molecules

although distinct in size from miR Even though

25- to 31-nucleotide long piRNAs are not generated

by Dicer, both sense and antisense strands of the

piRNA hairpin are involved in formation of the

piR-NA-interacting complex (piRC) and function in the

transcriptional gene silencing of retrotransposons and

genetic elements in germline cells [18]

Investigations into the gene expression of

endoge-nous miR in cells or tissues are useful for

understand-ing cellular metabolism, disease diagnosis and the

effects of therapies related to miR However, current

methods of monitoring endogenous miR levels, such as

northern blotting, RT-PCR, and microarrays are

time-consuming, laborious, and non-reproducible In a

pre-vious study, we successfully imaged miR23a biogenesis

in small animals to noninvasively monitor the

expres-sion patterns of endogenous miR23a in different cells

[19] This type of bioluminescence imaging technology

may be clinically relevant and could be applied to the real-time analysis of miR biogenesis in living animals Currently, the most widely used bioluminescent pro-teins in living animals are Gaussia Luciferase (GLuc) and Firefly Luciferase (FLuc) GLuc emits light at a

480 nm by oxidizing its substrate coelenterazine [20], FLuc emits at 562 nm when it oxidizes d-luciferine [21]

We cloned the upstream region of miR9 and studied the expression pattern of endogenous pri-miR9-1 to try to understand miR9 biogenesis during the neuronal differentiation of P19 cells using RT-PCR and biolu-minescent imaging The unbalanced biogenesis of mature miR9 and miR9* during neurogenesis was monitored by real-time PCR and in vitro and in vivo Luciferase reporter gene systems

Results

Detection of the endogenous level of the pri-miR9s

To study miR9 biogenesis during neurogenesis, we first investigated the primary transcript level of miR9

in P19 cells that had differentiated into neuronal cells following retinoic acid treatment Mouse and human genomes from the UCSC database showed three dif-ferent loci that can be processed into mature miR9 and⁄ or miR9* Three different primary transcripts

of miR9 in mouse are located at chromosome 3 (pri-miR9-1), chromosome 13 (pri-miR9-2), and chro-mosome 7 (pri-miR9-3; Fig 1A) The gene-expression levels of the primary transcripts of miR9 were moni-tored by sequence-specific RT-PCR analysis using total RNA from P19 cells induced to differentiate by retinoic acid PCR primers were designed by aligning the sequences of three different pri-miR9s to match their unique pri-miR9s, but not to amplify alternative sequences (Fig 1B) Gene-expression analysis of P19 cells treated with retinoic acid for 6 days showed a gradual increase in MAP2 transcript levels, a neuro-nal marker gene, which was expected to occur during neuronal differentiation (Fig 1C) The gene expres-sions of the three different pri-miR9s exhibited vari-ous transcript patterns during neuronal differentiation

of P19 cells Pri-miR9-1 showed a dramatic change in gene expression immediately after treatment with reti-noic acid, i.e a gradual increase in primary transcript level until the third day, followed by a sudden decrease By contrast, pri-miR9-3 was relatively highly expressed even before neuronal differentiation, increasing gradually during neurogenesis until the fourth day and then completely disappeared Unlike

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the other two pri-miR9s, pri-miR9-2 expression

was barely detectable in undifferentiated and P19 cells

differentiated by retinoic acid This suggests that the

transcript level of pri-miR9-1 is a good bioindicator

for the neuronal differentiation of P19 cells treated

with retinoic acid

Bioimaging of the highly expressed pri-miR9-1 during neurogenesis

To monitor the endogenous expression of pri-miR9s using the bioluminescent Luciferase reporter gene system during neuronal differentiation in P19 cells,

A

B

C

Fig 1 Detecting the gene-expression

pat-terns of the three different pri-miR9s during

neurogenesis (A) Chromosomal locations of

the three different pri-miR9s in mice from

the UCSC database (B) Primer positions

and sequences used to amplify pri-miR9-1,

9-2 and 9-3 Arrows indicate the position

and orientation of the primers Bold font

represents the sequence of mature miR9*

and italic fonts the sequence of mature

miR9 (C) RT-PCR analysis of pri-miR9s

dur-ing the neuronal differentiation of P19 cells

treated with retinoic acid (RA) pri-miR9-1

and -9-3 were gradually increased during

neuronal differentiation, whereas the

pri-miR9-2 transcript was barely detected.

MAP2, a neuronal marker gene, showed

that retinoic acid treatment efficiently

induced neuronal differentiation of P19 cells.

B-Actin was used as an internal control.

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1343 bp of the upstream region of the pri-miR9-1 from

human genomic DNA was cloned and fused into a

pro-moterless reporter vector, pGL3_Basic, which contained

the ORF of the FLuc reporter gene (Fig 2A) FLuc

activity was measured to determine the promoter

activ-ity of pri-miR9-1 during retinoic acid-induced neuronal

differentiation The upstream region of the pri-miR9-1

was randomly split into five different segments by PCR,

)1387 to )44 bp (miR9-1PN1_Fluc), )846 to )44 bp

(miR9-1PN2_Fluc),)530 to )44 bp (miR9-1PN3_Fluc),

)236 to )44 bp (miR9-1PN4_Fluc), and )135 to )44 bp

(miR9-1PN5_Fluc; Fig 2B) These five different

con-structs were then transfected into P19 cells and their

pro-moter activities monitored using an in vitro Luciferase

assay over 2 days following treatment of P19 cells with

retinoic acid (Fig 2C) Most of the constructs from P19

cells treated or not with retinoic acid had equal or lower

promoter activities than did the pGL3_Basic vector used

as a negative control However, miR9-1PN3_Fluc

showed a relatively stronger FLuc signal and a higher

expression level after neuronal differentiation than the

other segments, which indicated an increased

endoge-nous level of pri-miR9-1 during neurogenesis This

indi-cates that negative promoter elements of pri-miR9-1

transcription may be involved in the upstream region

between -846 and -531 bp and that positive elements

may be involved between -530 and -237 bp These

find-ings indicate that the miR9-1PN3_Fluc construct could

be used for in vivo imaging of gene expression of

endoge-nous pri-miR9 during neurogenesis

To image in vivo the endogenous expression of the

pri-miR9 in small animals, 2.5· 106 of P19 cells

bear-ing the miR9-1PN3_Fluc construct were

subcutane-ously implanted into mice and region of interest

(ROI) analysis was performed on the basis of the

resultant bioluminescent signals obtained 2 days after

inducing neuronal differentiation with retinoic acid

(Fig 2D) All the Luciferase signals of the

CMV_Fluc, a positive control, from the right

shoul-der, showed constant and high FLuc expression at 0,

18, 24, and 48 h after retinoic acid treatment The

negative control, pGL3_Basic, in left shoulders, was

found to show weak or undetectable FLuc expression

throughout the investigation FLuc intensities of

miR9-1PN3_Fluc (right thighs; normalized versus

CMV_Fluc) showed a gradual increase in the presence

of retinoic acid compared with left thighs which were

not treated with retinoic acid ROI analysis showed

that miR9-1PN3_Fluc showed an almost fivefold

increase in FLuc activity 1 day after retinoic acid

treatment The findings of our in vitro and in vivo

Luciferase assays showed that miR9-1PN3_Fluc

biolu-minescence reflects elevated endogenous pri-miR9-1

levels during the neuronal differentiation of P19 cells treated with retinoic acid

Mature miR9 was relatively higher expressed than mature miR9* during neurogenesis Mature miR9 and miR9*, which may be processed from the same pre-miR9, are known to be highly expressed at the same time during neuronal develop-ment [17] To quantify their relative expression levels during neurogenesis, we conducted real-time PCR using small RNAs extracted from the neuronal differ-entiation of P19 cells at 0, 1, 2, 3, 4, 5 and 6 days after treatment with retinoic acid The amplicons produced using pairs of specific primers for mature miR9 and miR9* were quantified and normalized using U6 small RNA Endogenous mature miR9 and miR9* were barely detectable prior to the neuronal differentiation

of P19 cells (Fig 3A) However, these mature miRs showed a similar and gradually increased expression pattern during neuronal differentiation of P19 cells Interestingly, mature miR9 was consistently expressed

at a  40% higher level than mature miR9* during differentiation

To image the endogenously unequal expressions of mature miR9 and miR9* during neurogenesis, a GLuc reporter gene vector was first designed containing the following components in order: a CMV promoter, an ORF of GLuc, three copies of perfectly complemen-tary sequences of mature miR9 (designated as CMV⁄ Gluc ⁄ 3xPT_mir9) or miR9* (designated as CMV⁄ Gluc ⁄ 3xPT_mir9*) (Fig 3B) When mature miR9 or miR9* is present in cells, the GLuc activities

of CMV⁄ Gluc ⁄ 3xPT_mir9 andCMV ⁄ Gluc ⁄ 3xPT_mir9* are repressed by cognate mature miR9 and miR9*, respectively To demonstrate the specificity of the bio-luminescent reporter system to monitor both mature miR9 and miR9*, CMV⁄ Gluc ⁄ 3xPT_mir9 or CMV ⁄ Gluc⁄ 3xPT_mir9* with a negative control vector, CMV_Gluc, were transfected into HeLa cells which do not express mature miR (Fig 3C) The CMV_Gluc construct, which was not repressed by exogenous pre-miR was used to normalize the GLuc activities of the CMV⁄ Gluc ⁄ 3xPT_mir9 and CMV ⁄ Gluc ⁄ 3xPT_mir9*

in HeLa cells treated with various concentrations (0, 2.5, 5, 10, 20 nm) of exogenously derived pre-miR9 or pre-miR9* The GLuc expressions of both CMV⁄ Gluc⁄ 3xPT_mir9 and CMV ⁄ Gluc ⁄ 3xPT_mir9* showed

a dramatic decrease in response to exogenous pre-miR9 and pre-miR9*, respectively The CMV⁄ Gluc ⁄ 3xPT_mir23a vector, which has previously been reported to monitor mature miR23a [19], was transfected into HeLa cells and found not to change

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B

C

D

Fig 2 In vitro and in vivo GLuc expression

of pri-miR9-1 during neuronal differentiation.

(A) The chromosomal region of

has-pri-miR9-1 (B) Schematic diagram of the

upstream region of pri-miR9-1 fused to a

promoterless FLuc reporter vector The

pro-moter sizes of the construct are indicated

by numbers in parentheses )44 means

located 44 bp upstream of the first base pair

at the 5¢-end of pre-miR-9-1 defined as +1.

FLuc is the ORF of the Firefly Luciferase

reporter gene (C) In vitro bioluminescent

assay of pri-miR9-1 during neuronal

differen-tiation of P19 cells Five different upstream

regions of pri-miR9-1 were transfected into

P19 cells, miR9-1PN3_Fluc produced a

strong FLuc signal after neuronal

differentia-tion of P19 cells, pGL3_Basic vector was

used to normalize the FLuc activities

obtained from the five different constructs.

Transfections were performed in triplicate

and results are expressed as mean ± SD.

(D) Bioluminescence image of pri-miR9-1

expression in nude mice P19 cells

(2.5 · 10 6 ) were transiently transfected with

miR9-1PN3_Fluc and injected into nude

mice In right thighs, neuronal differentiation

was induced by retinoic acid, whereas left

thighs were not treated with retinoic acid.

The pGL3_Basic vector in the right

shoul-ders was used as a negative control and

CMV_Fluc in right shoulders as a positive

control, and were used to normalize FLuc

activities acquired on each day

Biolumines-cence intensities in right thighs, expressing

pri-miR9-1 were increased during neuronal

differentiation of P19 cells compared with

the left thigh (n = 3 mice ⁄ group) The lower

panel shows ROI analysis of the

biolumines-cence image Fold ratios of FLuc activities

were normalized versus FLuc intensity on

day 0 Experiments were performed in

tripli-cate and results are expressed as

mean ± SD.

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GLuc expression significantly after treatment with

exogenous pre-miR9 or pre-miR9* Both CMV⁄ Gluc ⁄

3xPT_mir9 and CMV⁄ Gluc ⁄ 3xPT_mir9* reporter

sys-tems demonstrated a great specificity of monitoring its

cognate mature miR9 and miR9*, respectively

In vitro bioluminescent Luciferase assays of the

unequally expressed mature miR9 and miR9* during

neurogenesis were conducted in P19 cells treated with retinoic acid for 4 days The CMV⁄ Gluc ⁄ 3xPT_mir9

or CMV⁄ Gluc ⁄ 3xPT_mir9* construct was transfected into P19 cells and GLuc activities, representing the endogenous levels of mature miR9 or miR9*, were

(Fig 3D) As observed for mature miR9 or miR9* during the neuronal differentiation of P19 cells by real-time PCR, GLuc expressions of CMV⁄ Gluc ⁄ 3xPT_ mir9 and CMV⁄ Gluc ⁄ 3xPT_mir9* were both significantly lower in neuronally differentiated than in undifferentiated P19 cells and were observed to gradu-ally decreased during the neuronal differentiation In addition, the GLuc signal of CMV⁄ Gluc ⁄ 3xPT_mir9 was relatively smaller than that of CMV⁄ Gluc ⁄ 3xPT_ mir9* throughout the investigation, which implies a

A

B

C

D

Fig 3 Gene expressions of mature miR9 and miR9* during neuro-nal differentiation (A) Using real-time PCR The gene expressions

of endogenous mature miR9 and miR9* during the neuronal differ-entiation of P19 cells treated with retinoic acid for 6 days were determined The expressions of mature miR9 and miR9* gradually increased during neurogenesis, but mature miR9 was found to be expressed 1.4-fold more than mature miR9* The line with a trian-gular head represents the fold ratio of miR9 to miR9* expression values (right y-axis) The left y-axis shows the real-time PCR intensi-ties of each mature miRNAs normalized versus U6 snRNA (C T = C T-before – C T-day, C T = C T-miRNA – C T-U6RNA ) Experiments were performed in triplicate and results are expressed as mean ± SD (B) Schematic diagram of the reporter genes used to monitor mature miR9 and miR9* The black and gray boxes indicated three copies of perfectly complementary sequences of mature miR9 and miR9*, respectively These three copies were located between the stop codon and the polyadenylation sequence of the GLuc gene These systems were designed to repress GLuc expression when mature miR9 and miR9* were present (C) Specification of the recombination constructs CMV ⁄ Gluc ⁄ 3xPT_mir9 and CMV ⁄ Gluc ⁄ 3xPT_mir9* regulated by miR9 and miR9*, respectively The GLuc activities of CMV ⁄ Gluc ⁄ 3xPT_mir9, CMV ⁄ Gluc ⁄ 3xPT_mir9*, or CMV ⁄ Gluc ⁄ 3xPT_mir23a constructs were normalized using CMV_Gluc vector and determined at five different concentrations (n M on the x-axis) of exogenous pre-miR9 or pre-miR9* in HeLa cells Experiments were performed in triplicate and results are shown as means ± SDs (D) In vitro Luciferase assay of endoge-nous mature miR9 and miR9* during the neuronal differentiation of P19 cells CMV ⁄ Gluc ⁄ 3xPT_mir9 or CMV ⁄ Gluc ⁄ 3xPT_mir9* were transfected and endogenous levels of mature miR9 and miR9* in P19 cells treated with retinoic acid were determined The y-axis represents the fold ratio of GLuc expression during neuronal differ-entiation versus GLuc expression from undifferentiated P19 cells; the white bar represents mature miR9 and the black bar mature miR9*, and the line with a triangular head indicates the ratio (numerical values shown on the top of bar) of mature miR9 to miR9* Experiments were performed in triplicate and results are expressed as mean ± SD.

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higher endogenous level of mature miR9 than of

mature miR9*

In vivo visualization of unbalanced expressions of

mature miR9 and miR9* during neurogenesis

To monitor in vivo the endogenously unequal

expres-sion of mature miR9 and miR9* during neuronal

dif-ferentiation in P19 cells, CMV⁄ Gluc ⁄ 3xPT_mir9,

CMV⁄ Gluc ⁄ 3xPT_mir9* or CMV_Gluc (a negative

control), were transfected into 2.5· 106 of P19 cells

and subcutaneously implanted into nude mice in the

presence or absence of retinoic acid (Fig 4A) In addi-tion to in vivo imaging of endogenous mature miR9 or miR9* during neurogenesis, CMV_Fluc vector, which expressed constant FLuc activity regardless of the pres-ence of mature miR9 or miR9* or retinoic acid, was cotransfected with CMV⁄ Gluc ⁄ 3xPT_mir9 or CMV ⁄ Gluc⁄ 3xPT_mir9* into P19 cells as an internal control FLuc activities of left thighs not treated with retinoic acid and of treated right thighs showed no significant change after CMV⁄ Gluc ⁄ 3xPT_mir9 or CMV ⁄ Gluc ⁄ 3xPT_mir9* transfection (Fig 4B,C, lower) GLuc signals, as determined by ROI analysis, from

A

B

C

Fig 4 In vivo Luciferase imaging of the

mature miR9 and miR9* during the neuronal

differentiation (A) The strategy used to

implant P19 cells into mice to image mature

miR9 and miR9* during neurogenesis.

CMV_Gluc tranfected into right shoulders

was used to normalize GLuc signals and

CMV_Fluc transfected into left and right

thighs was used as an internal control (B,C)

In vivo imaging of mature miR9 and miR9*

during the neuronal differentiation of P19

cells treated with retinoic acid FLuc signals

of CMV_Fluc in the lower panel showed

similar strong expressions in the presence

(right thigh) or absence (left thigh) of retinoic

acid ROI analysis results in the right panel

and bioluminescence imaging results in the

left upper panel show that the GLuc

activi-ties of CMV ⁄ Gluc ⁄ 3xPT_mir9 in right thighs

(B) and left shoulders (C) were more

repressed during the neuronal differentiation

of P19 cells than CMV ⁄ Gluc ⁄ 3xPT_mir9* in

left shoulders (B) and right thighs (C) ROI

fold ratios were normalized versus GLuc

intensity at 0 h Experiments were

per-formed in triplicate and results are

expressed as mean ± SD.

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CMV⁄ Gluc ⁄ 3xPT_mir9 with retinoic acid in right

thighs were dramatically reduced compared with

CMV⁄ Gluc ⁄ 3xPT_mir9 without retinoic acid in left

thighs, and had almost disappeared 2 days after

neuro-nal differentiation (Fig 4B,C, upper) Similarly,

CMV⁄ Gluc ⁄ 3xPT_mir9* in right thighs showed

signifi-cant GLuc repression during the neuronal

differentia-tion of P19 cells treated with retinoic acid compared

with left thighs not treated with retinoic acid Fold

ratios of ROI of CMV⁄ Gluc ⁄ 3xPT_mir9 and

CMV⁄ Gluc ⁄ 3xPT_mir9* on day 1 between pre- and

post differentiation were 6- and 14-fold, respectively

The bioluminescent signals and ROI analysis in

Fig 4B,C showed that CMV⁄ Gluc ⁄ 3xPT_mir9 had

higher repression of the GLuc intensity during

neuro-genesis than CMV⁄ Gluc ⁄ 3xPT_mir9*, indicating that

mature miR9 are relatively more expressed than

miR9* during neuronal differentiation of P19 cells

treated with retinoic acid

Discussion

Thousands of miRs proven by the cloning of hundreds

of miRs from various species have been identified by

bioinformatics analysis [22] and tens of miRs have

been reported to be related to specific tissue

develop-ment, cellular differentiation, proliferation, apoptosis,

and various diseases including cancers, cardiovascular

diseases, neurological diseases and metabolic disorders

[4,5] Even though the regulation and functions of

miRs are unclear, the basic molecular mechanisms of

miR biogenesis in cells have been shown to be

pro-cessed into the primary, precursor, and mature form of

miRs by RNA polymerase II, Drosha, exportin-5,

Dicer and RNA-induced silencing complex [1,11,12]

However, cellular gene-expression analysis of miRs has

been restricted to laborious and irreproducible

meth-ods like in situ hybridization and northern blotting

Moreover, these methods have been used to detect

only endogenous mature miRs in cells [17,23] Few

studies have examined miRs to determine initial gene

expression associated with miR biogenesis using the

upstream region of miRs, which is considered a

pro-moter Using the developed bioluminescent imaging

system to monitor 1 we found that

pri-miR9-1 is highly and specifically expressed in neurons during

the retinoic acid-induced differentiation of P19 cells

The upstream region of the pri-miR9-1 from )530 to

)44 bp was found to show substantial promoter

activ-ity during neurogeneis, whereas other constructs with

longer or shorter fragments were not found to be

effec-tive enough to monitor differences in endogenous

pri-miR9 expression during the neuronal

differentia-tion of P19 cells Recently, a number of important transcription factors, such as repressor element silenc-ing transcription factor, cAMP response element-bind-ing protwin, Nanog, and Octamer4 have been suggested to be involved in the transcriptional regula-tion of neuronal miRs [24–26] Unfortunately, the upstream region of the pri-miR9-1 does not have any homologue-binding sequence for the transcription factors that are required to maintain the neuronal differentiation of stem cells

Moreover, the molecular mechanisms of the bioge-neses of a number of miRs are equivocal miR23a, which was previously reported upon by our laboratory, showed unbalanced biogenesis in pri-miR23a and resultant mature 23a in HEK293 cells, but not in HeLa cells and P19 cells [19] Highly expressed pri-miR23a produced a relatively low endogenous level of mature miR23a in HEK293 cells, indicating a slow turnover from pri-miR23a to mature miR23a In this study, real-time PCR and in vitro and in vivo biolumi-nescent imaging demonstrated relatively higher expres-sion levels of mature miR9 than of miR9* during the neuronal differentiation of P19 cells treated with reti-noic acid, even though both mature miRs probably originated from the hairpin sequences of the same pre-miR For strand selection from the secondary structure

of pre-miRs to be a single-stranded mature miR, ther-modynamic profiling of duplex pre-miR hairpin showed that in general, the 5¢ terminal sequence of pre-miR hairpin has less internal stability than the 3¢ terminal sequences of the pre-miRs, which implies that the mature miRs prefer miRs to miR*s [13,27] How-ever, this hypothesis is not applicable to several miRs cloned from several species miR18, miR106, miR16 and miR105 have a 5¢-end of precursor form in the mature form and miR142, miR17, miR302, miR373

[7,16,17,24] Even though the molecular mechanism of miR biogenesis is still unclear, interestingly, northern blotting and microarray analysis using human brain tissues also demonstrated that miR9 is more highly expressed than miR9* [6,17] Our previously reported dual Luciferase system will provide clearer and simul-taneous imaging of this phenomenon during miR bio-genesis [19]

The endogenous expression of mature miR9 has been recently reported to contribute to the develop-mental shift from neuron generation to glial cell gener-ation, and to be related to the expression of granuphilin⁄ slp4 in insulin-producing cells [28] More-over, miR9 and other neuronal miRs including miR125b and miR128, are involved in the Alzheimer’ disease [29]

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Our noninvasive bioluminescent imaging systems

devised to monitor miR9 can also be usefully applied

to study and monitor the biogenesis of other miRs

related to neuronal development, differentiation, and

neuronal diseases In addition, the in vitro and in vivo

imaging systems will undoubtedly provide information

about the molecular patterns and mechanisms of miR

biogenesis in various heterogeneous cells

Experimental procedures

Recombinant constructions of reporter gene to

monitor primary and mature form of miR9

To detect the transcript level of pri-miR9, the upstream

region of pri-miR9-1 was isolated from the genomic DNA

of HeLa cells and cloned into a promoterless vector,

pGL3_Basic vector (Promega, Madison, WI) containing the

ORF of FLuc Five different fragments, which were fused

into the HindIII site of the reporter gene and designated

miR9-1PN1_Fluc, miR9-1PN2_Fluc, miR9-1PN3_Fluc,

miR9-1PN4_Fluc, and miR9-1PN5_Fluc, were amplified

using the primer pairs listed in Table 1, and then sequenced

to determine the orientation of the fragments in the

repor-ter vector These constructs were then transfected into P19

cells by liposome-mediated transfection using a Lipofectin

reagent kit (Invitrogen, Grand Island, NY, USA) and FLuc

activity was monitored during the neuronal differentiation

of P19 cells treated with retinoic acid (retinoic acid)

To study the mature forms miR9 and miR9*, mature

sequences of has-miR-9 and mature has-miR-9* were

obtained from the MirnaMap database

(http://mirna-map.mbc.nctu.edu.tw) and oligonucleotides containing

three copies of a perfectly complementary sequence of mature miR9 or miR9* were synthesized (Table 1) Each pair of sense and antisense oligos was annealed in annealing buffer (·1 TE buffer + 50 mm NaCl) for 10 min at 60 C and ligated into the XhoI and XbaI sites of CMV_Gluc vec-tor (Targeting Systems, San Diego, CA, USA) to create CMV⁄ Gluc ⁄ 3xPT_mir9 and CMV ⁄ Gluc ⁄ 3xPT_mir9*

Cell culture and neuronal induction of P19 cells P19 (a mouse embryonic carcinoma cell line) was purchased from the American Type Culture Collection (Manassa, VA, USA) P19 cells were grown in a-MEM (Gibco, Grand Island, NY, USA) supplemented with 2.5% fetal bovine serum (Cellgro, Herndon, VA, USA), 7.5% bovine calf serum (Gibco), and 1% antibiotics–antimycotic (Cellgro) [30] To induce neuronal differentiation, P19 cells were cul-tured under serum-free conditions in Dulbecco’s modified Eagle’s medium⁄ 12(1 : 1) media (Gibco) supplemented with insulin, transferring, and selenium (ITS; Gibco) and then treated with 5· 10)7m all-trans retinoic acid (Sigma, St Louis, MO, USA) for 3 days HeLa cells (an adenocarci-noma cell line) were cultured routinely in RPMI (Jeil Bio-techservices Inc, Daegu, Korea) containing 10% fetal bovine serum and 1% antibiotics–antimycotic

Transfection of CMV⁄ Gluc ⁄ 3xPT_mir9

& CMV⁄ Gluc ⁄ 3xPT_mir9* and precursor miR9 & miR9*

P19 cells were seeded at 0.6· 105 (undifferentiated), 0.8· 105

(1 day), 0.6· 105

(2 days), 0.4· 105

(3 days), and 0.2· 105

(4 days) in a six-well plate 24 h prior to

Table 1 Primers used to amplify pri-miR9-1 promoter and clone the perfect target sequence of mature miR9 and miR9*.

Perfect target seq.

of miR9 sense

TCGAGAATCTAGT TCA TAC AGC TAG ATA ACC AAA GA TAGTA TCA TAC AGC TAG ATA ACC AAA GA TAGTA TCA TAC AGC TAG ATA ACC AAA GAT

Construction of CMV ⁄ Gluc ⁄ 3xPT_mir9

Perfect target seq.

of miR9 anti-sense

CTAGA TCT TTG GTT ATC TAG CTG TAT GA TACTA TCT TTG GTT ATC TAG CTG TAT GA TACTA TCT TTG GTT ATC TAG CTG TAT GA ACTAGATTC

Construction of CMV ⁄ Gluc ⁄ 3xPT_mir9

Perfect target seq.

of miR9* sense

TCGAGAATC TAG TAC TTT CGG TTA TCT AGC TTT A TAGTA ACT TTC GGT TAT CTA GCT TTA TAGTA ACT TTC GGT TAT CTA GCT TTAT

Construction of CMV ⁄ Gluc ⁄ 3xPT_mir9*

Perfect target seq.

of miR9* anti-sense

CTA GAT AAA GCT AGA TAA TTG AAA GT TACTA TAA AGC TAG ATA ACC GAA AGT TACTA TAA ACG TAC ATA ACC GAA AGT ACTAGATTC

Construction of CMV ⁄ Gluc ⁄ 3xPT_mir9*

Trang 10

tranfection Transient transfections were performed using

1 lg of DNA using lipofectamine (Invitrogen) HeLa (a

miR9 non-producing cell line) was seeded at 1· 105

cells to determine the expressions of miR9 and miR9*

Luciferase assays for FLuc and GLuc activities

P19 and HeLa cells were washed with NaCl⁄ Piand treated

with lysis buffer (200 lLÆwell)1) for Luciferase assays

Lysed cells were transferred to a 96-well white microplate

and Luciferase activities were measured using luminometer

(TR717; Applied Biosystems, Foster City, CA, USA) and

an exposed time of 1s All data are presented as

means ± SD calculated from triplicate wells

RT-PCR analysis in undifferentiated and

differentiated P19 cells

Total RNA was isolated from cultured cells using

Tri-zol reagent (Invitrogen) Reverse transcription to synthesize

first-strand cDNA was carried out using random-hexamer

primer and SuperScript II reverse transcriptase (Invitrogen),

according to the manufacturer’s instructions, and used as a

template for PCR amplification PCR amplifications of

MAP2 and b-actin cDNA were performed using i-Taq

DNA polymerase (Table 2) (iNtRON; Korea) PCR

prod-ucts were loaded on agarose gels containing ethidium

bromide, and bands were revealed under UV For

pri-miR9-1, pri-miR9-2 and pri-miR9-3, first-strand cDNA

synthesis was carried out using random-hexamer primer

and promoter primers (Table 2)

Quantitative RT-PCR of mature miR9 and miR9*

Small RNA was isolated from cultured cells using mirVana

miRNA isolation kits (Ambion, Austin, TX, USA), and

qRT-PCR was performed using mirVanaTMqRT-PCR miR

detection kits (Ambion) using a has-miR-9 or a has-miR-9*

primer set (Ambion) according to the manufacturer’s

instructions To normalize experimental samples for RNA

content, the U6 snRNA primer set (Ambion) was used as a control

In vivo visualization of primary miR9 expression

or mature miR9 and miR9* expressions in undifferentiated and differentiated P19 cells The miR9-1PN3_Fluc construct was transfected into P19 cells, which were divided into retinoic acid-treated and non-retinoic acid treated groups for in vivo imaging At 48 h after transfection, 1· 106 P19 cells were harvested with

100 lL NaCl⁄ Pi, and resuspended with retinoic acid for the neuronal differentiation group P19 cells were then subcuta-neously injected into each thigh of 6-week-old male Balb⁄ c nude mice, 3 mg of d-luciferin was administered intraperi-toneally [31] This study was approved by the IACUC (Institutional Animal Care and Use Committee) of Clinical Research Institute, Seoul National University Hospital (AAALAC accredited faculty) Bioluminescence images were acquired using an IVIS100 (In vivo Imaging System; Xenogen, Alameda, CA, USA) with the integration time of

5 min For in vivo GLuc imaging, nude mice were imaged using the IVIS100 system after direct administering 50 lg

of coelenterazine

Acknowledgements

This study was supported by Nano Bio Regenomics Project of Korean Science and Engineering Founda-tion and by InnovaFounda-tion Cluster for Advanced Medical Imaging Technology This study was made easier using KREONET, Korean Research Network, a nationwide giga-bps network system

References

1 Reinhart BJ, Slack FJ, Basson M, Pasquinelli AE, Bettinger JC, Rougvie AE, Horvitz HR & Ruvkun G (2000) The 21-nucleotide let-7 RNA regulates

Table 2 Primers used in real-time polymerase chain reaction (RT-PCR).

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