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Tiêu đề Nucleolin/C23 mediates the antiapoptotic effect of heat shock protein 70 during oxidative stress
Tác giả Bimei Jiang, Bin Zhang, Pengfei Liang, Juan Song, Hongbing Deng, Zizhi Tu, Gonghua Deng, Xianzhong Xiao
Trường học Xiangya School of Medicine, Central South University
Chuyên ngành Pathophysiology
Thể loại Journal article
Năm xuất bản 2009
Thành phố Changsha
Định dạng
Số trang 11
Dung lượng 563,96 KB

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Nội dung

Results Overexpression of Hsp70 protects cardiomyocytes from H2O2-induced apoptosis First, to overexpress Hsp70 we transiently transfected cardiomyocytes with a plasmid carrying human Hs

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shock protein 70 during oxidative stress

Bimei Jiang1, Bin Zhang1, Pengfei Liang2, Juan Song1, Hongbing Deng1, Zizhi Tu1, Gonghua Deng1 and Xianzhong Xiao1

1 Department of Pathophysiology, Xiangya School of Medicine, Central South University, Changsha, Hunan, China

2 Department of Burns and Plastic Surgery, Xiangya Hospital, Central South University, Changsha, Hunan, China

Introduction

Characterized by cellular and nuclear shrinkage,

cyto-plasmic blebbing, chromatin condensation and DNA

fragmentation [1,2], apoptosis can cause irreversible

loss of terminally differentiated cardiac myocytes and,

therefore, contributes significantly to the pathogenesis

of many cardiovascular diseases Apoptosis has been

identified in cardiac myocytes from patients suffering

from myocardial infarction, diabetic cardiomyopathy,

and end-stage congestive heart failure

Apoptosis is a highly regulated programme of cell

death and can be mediated by death receptors in the

plasma membrane, as well as in the mitochondria and

the endoplasmic reticulum [3] Studies on apoptotic

pathways in cardiomyocytes have revealed several

molecules as key regulators [4] Heat shock protein

70 (Hsp70) is a major stress-inducible heat shock pro-tein that has been shown to protect cells from apoptosis induced by heat shock, tumour necrosis factor, growth factor withdrawal, oxidative stress and radiation [5,6] Hsp70 is also a major self-preservation protein in the heart; its overexpression enhances myocardial tolerance to ischaemia⁄ reperfusion injury

in both transgenic animals [7] and cell cultures [8] Although substantial progress has been made in understanding the control and mechanisms of apopto-sis, how Hsp70 protects cardiomyocytes against apop-tosis induced by a variety of stresses remains to be investigated

Keywords

apoptosis; cardiomyocytes; heat shock

protein 70; hydrogen peroxide;

nucleolin ⁄ C23

Correspondence

Xianzhong Xiao, Department of

Pathophysiology, Xiangya School of

Medicine, Central South University,

Changsha, Hunan 410008, China

Fax: +86 731 82355019

Tel: +86 731 2355019

E-mail: xianzhongxiao@xysm.net

(Received 22 August 2009, revised 26

October 2009, accepted 23 November

2009)

doi:10.1111/j.1742-4658.2009.07510.x

Although heat shock protein 70 (Hsp70) has been shown to markedly inhi-bit H2O2-induced apoptosis in C2C12 cells, and nucleolin⁄ C23 has also been implicated in apoptosis, the relationship of these two molecules is still largely unknown The aim of the current study was to investigate the potential involvement of nucleolin⁄ C23 in the antiapoptotic mechanism of Hsp70 We found that primary cultures of neonatal rat cardiomyocytes underwent apoptosis upon H2O2 treatment, and in these cells nucleo-lin⁄ C23 protein was highly unstable and had a half-life of less than 4 h However, transfection with Hsp70 greatly stabilized nucleolin⁄ C23 and also protected the cells from H2O2-induced apoptosis When nucleolin⁄ C23 was knocked down with an antisense oligomer, H2O2-induced apoptosis became more severe, even in Hsp70-overexpressed cells, demonstrating an essential role of nucleolin⁄ C23 in the antiapoptotic effects of Hsp70 Similar results were obtained by both nuclear morphology observation and caspase-3 activity assay Therefore, these data provide evidence that nucleolin⁄ C23 is

an essential downstream effecter of Hsp70 in the protection of cardiomyo-cytes against oxidative stress-induced apoptosis

Abbreviations

DMEM, Dulbecco’s modified Eagle’s medium; FITC, fluorescein isothiocyanate; GAPDH, glyceraldehyde-3-phosphate dehydrogenase; Hsp70, heat shock protein 70; PBS, phosphate-buffered saline; PI, pyridine iodination; SEM, standard error of the mean.

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Nucleolin⁄ C23 is a 110 kDa multifunctional

phos-phoprotein It is abundantly expressed in both normal

and cancerous cells [9], and ubiquitously distributed in

the nucleolus, nucleus and cytoplasm of the cell, as

well as at the cell surface [10] Nucleolin⁄ C23 regulates

many aspects of DNA and RNA metabolism, such as

RNA polymerase I-mediated transcription, the folding,

maturation, ribosome assembly and nucleocytoplasmic

transport of newly synthesized pre-rRNAs [11]

Because of its widespread distribution and broad range

of involvement, as well as the cross-talking among

molecules of different cellular processes, dissection of

nucleolin⁄ C23’s specific functions is particularly

chal-lenging

Recently, nucleolin⁄ C23 has also been implicated in

apoptosis All-trans retinoic acid-induced apoptosis

leads to nucleolin downregulation and bcl-2 mRNA

instability; overexpression of nucleolin⁄ C23 in chronic

lymphocytic leukaemia cells stabilizes bcl-2 mRNA

[12,13] Our previous study showed that oxidative

stress induces nucleolin⁄ C23 cleavage and apoptosis

[14], and that nucleolin downregulation induces

apop-tosis in C2C12 cells [15] These data suggest the roles

of nucleolin⁄ C23 in oxidative stress-induced apoptosis,

but whether nucleolin⁄ C23 participates in

Hsp70-medi-ated protection against H2O2-induced apoptosis is not

clear In the present investigation, we further studied

the effects of nucleolin⁄ C23 ablation on

Hsp70-medi-ated protection from apoptosis and examined the

expression and stability of nucleolin⁄ C23 with Hsp70

overexpression in response to H2O2-induced apoptosis

using primary culture cardiomyocytes

Results

Overexpression of Hsp70 protects

cardiomyocytes from H2O2-induced apoptosis

First, to overexpress Hsp70 we transiently transfected

cardiomyocytes with a plasmid carrying human Hsp70

cDNA, and examined the protein levels by western

blot analysis with Hsp70 antiserum after 36 h The

effi-ciency of transfection mediated by the Lipofectamine

Plus reagent ranged between 30 and 50% (data not

shown) As can be seen in Fig 1A, Hsp70

overexpres-sion was confirmed in the cells transfected with Hsp70

cDNA, but not in the cells transfected with the vector

alone

To determine the effect of Hsp70 overexpression on

H2O2-induced apoptosis, the above transfected cells

were exposed to H2O2 (0.5 mmolÆL)1) for the indicated

time periods and the percentages of apoptotic cells

examined by morphological observation (Fig 1B)

A

B

C

Fig 1 Overexpression of Hsp70 renders cardiomyocytes resistant

to H2O2 Cardiomyocytes were transiently transfected with full-length Hsp70 plasmid pcDNA ⁄ Hsp70 (Hsp70 ⁄ C) or pcDNA vector (pcDNA ⁄ C) (A) Immunoblot analysis of Hsp70 expression At 36 h post-transfection, cells were analysed by immunoblotting with anti-bodies against Hsp70 or GAPDH (as an internal control of protein loading) The results shown are representative of three indepen-dent experiments (B) Quantification of apoptotic cells by nuclear staining Untransfected or transfected cells were exposed to 0.5 mmolÆL)1 H 2 O 2 for the indicated durations and stained with Hoechst 33258; apoptotic cells showing condensed chromatin fragments were scored and expressed as the percentage of the total cell number counted The results from three indepen-dent experiments are presented as mean ± SEM *P < 0.05 versus control group; #P < 0.05 versus pcDNA3.1 + H2O2 group (n = 3) (C) Caspase-3 activity assay Thirty-six hours after transient transfection, cells were treated with or without 0.5 mmolÆL)1H2O2.

At different time points, cells were harvested for protease activity

of caspase-3 using the caspase colorimetric assay kit Data were obtained from four independent experiments *P < 0.05 versus control group; #P < 0.05 versus pcDNA3.1 + H2O2group.

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After 24 h of H2O2 exposure, 44% of untransfected

control cells and 45% of cells transfected with the

empty vector (pcDNA3.1) exhibited similar features of

apoptotic cells, such as highly condensed nuclei and

decreased cell size However, only 22% of the cells

transfected with Hsp70 underwent apoptosis (Fig 1B)

We also investigated the effects of Hsp70 on caspase-3

activation induced by oxidative stress Using an in vitro

substrate-cleavage reaction, H2O2 treatment

signi-ficantly induced the activation of caspase-3 in the

untransfected control cells as well as cells transfected

with the vector alone in a time-dependent manner, but

Hsp70 overexpression significantly reduced caspase-3

activation in response to H2O2treatment (Fig 1C)

Increased nucleolin/C23 protein levels in

Hsp70-transfected cells in response to

H2O2-induced apoptosis

We next examined the expression of nucleolin⁄ C23

protein in these cells in response to H2O2 exposure

Upon treatment with H2O2 for up to 8 h, all cells

showed a time-dependent decrease in the 110 kDa

nucleolin⁄ C23 fragment accompanied by the

appear-ance and an increase in the 80 kDa fragment (Fig 2)

Although both the untransfected cells and the cells

transfected with the vector alone started to show the

80 kDa fragment at time points as early as 2–4 h after

H2O2 treatment, this smaller protein fragment

appeared in the Hsp70-overexpressed cells at the 8 h

time point (Fig 2A,B) Overall, the change in

nucleo-lin⁄ C23 protein levels was least significant in cells

transfected with Hsp70 cDNA (Fig 2B), suggesting a

protective effect of Hsp70 on the degradation of

nucleolin⁄ C23 protein

Prolonged half-life of nucleolin/C23 in Hsp70-transfected cells in response to H2O2 exposure

To compare the stability of nucleolin⁄ C23 protein in cells transfected with the vector alone and cells trans-fected with Hsp70 cDNA during H2O2 exposure, the cells were treated with H2O2 for 2 h Protein synthesis was then inhibited by cycloheximide (5 lgÆmL)1) Western blot analysis revealed a time-dependent rapid decline in nucleolin⁄ C23 110 kDa bands in H2O2 -trea-ted cells transfec-trea-ted with the vector alone; the half-life

of the protein was estimated to be less than 2 h (Fig 3, left panel) At the same time, the 80 kDa degraded product was detected in an increasing amount in H2O2-treated cells transfected with the vector alone shortly after cycloheximide treatment (2–8 h) By contrast, nucleolin⁄ C23 in cells transfected with Hsp70 cDNA was more stable in response to

H2O2 exposure, reaching its half-life at 8 h after cyclo-heximide treatment (Fig 3, right panel)

Overexpression of nucleolin/C23 protects cardiomyocytes from H2O2-induced apoptosis

To determine the effect of nucleolin⁄ C23 overexpres-sion on H2O2-induced apoptosis in cardiomyocytes, we first transiently transfected cells with plasmids carrying human nucleolin⁄ C23 cDNA or the empty vector Using western blot analysis we confirmed nucleo-lin⁄ C23 overexpression only in cells transfected with nucleolin⁄ C23 cDNA but not the empty vector (pcDNA⁄ C) (Fig 4A) Then, transfected cells were exposed to H2O2 (0.5 mmolÆL)1) and apoptosis was assayed by both Hoechst nuclear staining (Fig 4B)

Ctrl 0 h

Nucleolin/C23

Nucleolin/C23 GAPDH

GAPDH PcDNA/C cells with H2O2 exposure Hsp70/C cells with H2O2 exposure

H2O2

A

B

Fig 2 Changes in nucleolin ⁄ C23 protein levels in cells transfected with pcDNA vector (pcDNA ⁄ C) or Hsp70 cDNA (Hsp70 ⁄ C) during H 2 O 2 exposure Cardiomyocytes were untransfected (A) or transiently transfected with pcDNA vector (pcDNA ⁄ C)

or pcDNA ⁄ Hsp70 (Hsp70 ⁄ C) for 36 h (B), and were treated with 0.5 mmolÆL)1H2O2 for 0–8 h Cells were harvested and protein lysates were prepared for western blot anal-ysis with monoclonal antibodies against nucleolin ⁄ C23 or GAPDH The results shown are the representatives of three independent experiments.

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and caspase-3 activity assays (Fig 4C) By counting

apoptotic nuclei, at 24 h H2O2 exposure,  45% of

cells transfected with the vector alone were apoptotic

However, only 22% of cells transfected with

nucleo-lin⁄ C23 cDNA underwent apoptosis (Fig 4B)

Consis-tently, H2O2 treatment significantly induced caspase-3

activation in cells transfected with the vector alone in

a time-dependent manner, and nucleolin⁄ C23

overex-pression significantly reduced caspase-3 activation

(Fig 4C) However, simultaneous Hsp70

overexpres-sion afforded the cells no significant protection by

nucleolin⁄ C23 against oxidant stress (Fig 4D)

In addition, H2O2 induced apoptosis in

cardiomyo-cytes with a marked downregulation of Bcl-2 protein,

and nucleolin overexpression could inhibit the

down-regulation of Bcl-2 protein (Fig 5A) Furthermore, we

compared the stability of Bcl-2 mRNA in cells

transfect-ed with nucleolin cDNA (pcDNA3.1-C23) or vector

control (pcDNA3.1) in the presence or absence of H2O2

by incubating the cells with actinomycin D (5 lgÆmL)1)

for up to 3 h Bcl-2 mRNA in H2O2-treated vector

con-trol cells was found to be highly unstable In contrast,

Bcl-2 in H2O2-treated nucleolin-overexpressed cells was

significantly more stable (Fig 5B)

Potentiation of apoptosis in Hsp70-transfected

cells by nucleolin/C23 antisense oligomer

Next, we used the gene knockdown approach with an

antisense oligonucleotide to examine whether

nucleo-lin⁄ C23 is necessary in the antiapoptotic function of

Hsp70 Fluorescein isothiocyanate (FITC)-labelled

phosphorothioate oligodeoxynucleotides were

success-fully transfected into primary cultured cardiomyocytes

with Lipofectamine 2000 and achieved a transfection

efficacy of  80% (Fig 6A) Transfection of

nucleo-lin⁄ C23 antisense oligonucleotide selectively reduced

the levels of endogenous nucleolin⁄ C23 protein by

more than 75% after 36 h, whereas transfection of the scrambled control oligonucleotide did not alter nucleo-lin⁄ C23 protein levels (Fig 6B)

Then, Hsp70 overexpressing cells were transfected with nonspecific control or nucleolin⁄ C23 antisense oligomers and the percentages of apoptotic cells in response to H2O2 treatment were examined by three methods First, by nuclear staining the apoptotic rates were 9–25% in cells transfected with the control oligo-mers and much lower at 13 and 44% in cells

transfect-ed with the nucleolin⁄ C23 antisense oligomer (Fig 6C) Second, the activity of caspase-3 was analy-sed as a marker of apoptotic cells using an in vitro substrate-cleaving reaction As shown in Fig 6D,

H2O2-induced apoptosis was increased in cells trans-fected with nucleolin⁄ C23 antisense oligonucleotide compared with those transfected with the scrambled control oligonucleotide, even in the presence of Hsp70 overexpression Finally, apoptosis was further assayed

by flow cytometry with annexin V–FITC⁄ pyridine iodination (PI) double staining, which identified apop-totic cells as annexin V positive, but PI negative This method obtained results consistent with those from the other two methods, showing that when nucleolin⁄ C23 was knocked down with an antisense oligomer, H2O2 -induced apoptosis was enhanced, even with the Hsp70-overexpressed cells (Fig 7A,B)

Discussion

Both our previous study [16] and the present study have provided evidence that oxidative stress induces apoptosis of cardiomyocytes, which can be character-ized by nuclear condensation and cell shrinkage Inter-estingly, upon transfection with an Hsp70-containing plasmid, these same cells become much less sensitive to

H2O2 exposure This observation was confirmed by both cell morphology and caspase-3 activity analyses

pcDNA/C cells with

H2O2 exposure 2 h

0 h

Nucleolin/C23

GAPDH

Hsp70/C cells with

H2O2 exposure 2 h

Fig 3 Nucleolin ⁄ C23 protein is stabilized in Hsp70-transfected cells during H 2 O 2 exposure Cardiomyocytes were transiently transfected with pcDNA vector (pcDNA ⁄ C) or pcDNA ⁄ Hsp70 (Hsp70 ⁄ C) After treatment with 0.5 mmolÆL)1 H2O2 for 2 h, cycloheximide (CHX;

5 lgÆmL)1) was added At different time points (2–8 h), cells were harvested and protein lysates were prepared for western blot analysis with monoclonal antibodies against nucleolin⁄ C23 or GAPDH The results shown are the representatives of three independent experiments.

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Hsp70 has been shown to regulate apoptotic

sig-nalling, effecter molecule activation, certain

down-stream events of caspase activation, the release of

cathepsins, cytochrome c, apoptosis-inducing factor

and even the death-associated lysosome permeabiliza-tion [17–21] Particularly, Hsp70 inhibits the release

of cytochrome c and apoptosis-inducing factor from mitochondria and prevents apoptosis [22,23] Our previous study showed that Hsp70 overexpression inhibited H2O2-mediated release of Smac (the second mitochondria-derived activator of caspases), activa-tion of caspase-3 and caspase-9, and apoptosis in C2C12 myogenic cells [24] Stankiewicz et al [25] found that Hsp70 overexpression stabilizes Mcl-1 protein in heat-shocked cells Hsp70 has also been suggested to play an important role in precondition-ing, a phenomenon of protection of a heart from strong ischaemic insult by prior exposure to mild ischaemia or other mild stresses In the present study, we have shown that Hsp70 renders nucleolin⁄ C23 enhanced stability; however, a decrease in nucle-olin⁄ C23 stability restrains such a protective effect of Hsp70 against the H2O2-induced apoptosis These data suggest that Hsp70 may inhibit apoptosis at multiple points and through a wide range of mechanisms

Nucleolin is a major nucleolar phosphoprotein that belongs to a large family of RNA-binding proteins [26] It plays a role in the pre-rRNA transcription

Ctrl pcDNA3.1 pcDNA3.1-C23

Nucleolin/C23

GAPDH

60

40

50

30

20

10

0

3

4

2.5

3.5

3.5

3

2.5

2

1.5

1

0.5

0

0.5 mmol·L –1 H2O2

2

1.5

1

0.5

0

Ctrl

Ctrl

pcDN

A3.1

pcDN A3.1-C23 pcDN A3.1-Hsp70

pcDN A3.1-C23 + pcDN

A3.1-Hsp70

pcDNA3.1 + H2O2

Ctrl pcDNA3.1 + H2O2

*

*

#

#

#

#

#

*

pcDNA3.1-C23 + H2O2

pcDNA3.1-C23 + H2O2

A

B

C

D

Fig 4 Overexpression of nucleolin ⁄ C23 protects cardiomyocytes from H2O2-induced apoptosis Cardiomyocytes were transiently transfected with full-length nucleolin plasmid (pcDNA3.1-C23) or pcDNA3.1 vector (A) Immunoblot analysis of nucleolin ⁄ C23 expres-sion At 36 h post-transfection, cells were analysed by immunoblot-ting with antibodies against nucleolin ⁄ C23 or GAPDH (as an internal control of protein loading) The results shown are represen-tatives of three independent experiments (B) Quantification of apoptotic cells by nuclear staining Untransfected or transfected cells were exposed to 0.5 mmolÆL)1H2O2 for the indicated dura-tions and stained with Hoechst 33258; apoptotic cells showing con-densed chromatin fragments were scored and expressed as a percentage of the total cell number counted The results from three independent experiments are presented as means ± SEM.

*P < 0.05 versus control group; #P < 0.05 versus pcDNA3.1 +

H2O2group (n = 3) (C) Caspase-3 activity assay Thirty-six hours after transient transfection, cells were treated with or without 0.5 mmolÆL)1H2O2for 12 h and harvested for the determination of protease activity of caspase-3 using the caspase colorimetric assay kit Data were obtained from four independent experiments.

*P < 0.05 versus control group; #P < 0.05 versus pcDNA3.1 +

H2O2 group (D) Caspase-3 activity assay Thirty-six hours after transfection with pcDNA3.1-C23 or pcDNA3.1-Hsp70 or transient cotransfection with pcDNA3.1-C23 and pcDNA3.1-Hsp70, cells were treated with or without 0.5 mmolÆL)1H2O2for 12 h and har-vested for protease activity of caspase-3 Data were obtained from four independent experiments *P < 0.05 versus control group;

#P < 0.05 versus pcDNA3.1 + H2O2group.

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and ribosome assembly that is implicated in the early

stage of preribosomal ribonucleoprotein assembly and

processing [27] Nucleolin has also been suggested to

regulate cell proliferation and growth, cytokinesis,

rep-lication, embryogenesis and nucleogenesis [28] by

forming large molecular complexes with other factors,

such as casein kinase II, c-Myb, midkine, histone H1,

nucleophosmin, p53 and protein phosphatase 1 A

number of studies, including our own, indicate that

nucleolin⁄ C23 may be one of the key components in

the regulation of apoptosis [12–14,29–31] In the

pres-ent study, we found that overexpression of

nucleo-lin⁄ C23 protects cardiomyocytes from H2O2-induced

apoptosis, and that the mechanism is probably

associ-ated with the increase in Bcl-2 mRNA stability (Fig 5) In addition, we have also established a strong relationship between nucleolin⁄ C23 and the antiapop-totic effect of Hsp70 Nucleolin⁄ C23 in Hsp70-trans-fected cells is significantly stabilized during H2O2 exposure, and simultaneous Hsp70 overexpression affords no additional protection against oxidant stress (Fig 4D) Therefore, Hsp70-transfected cells with a higher level of nucleolin⁄ C23 protein become more resistant to oxidative stress and less susceptible to apoptotic death More importantly, the role of nucleo-lin⁄ C23 in this scenario is indispensable, as the sup-pression of nucleolin⁄ C23 expression by an antisense oligomer potentiates apoptosis, even in the Hsp70-transfected cells These results also indicate that the nucleolin⁄ C23 gene has a functional role in the growth control of cardiomyocytes, and its regulation may be closely associated with the susceptibility of the cell to the induction of apoptosis

Caspases are important molecular mediators of apoptosis in the cell [32] Assays for caspase-3 activ-ity have also confirmed that H2O2 exposure induces cardiomyocytes to undergo apoptosis and Hsp70 overexpression prevents H2O2-induced caspase activa-tion; when nucleolin⁄ C23 protein is suppressed by the antisense oligonucleotide, the protection of Hsp70 is lost

Taken together, our results demonstrate an impor-tant relationship among the regulation of nucleo-lin⁄ C23, the activation of caspase-3 and the induction

of apoptosis under the setting of oxidative stress and Hsp70 overexpression More importantly, for the first time, we provide strong evidence that nucleolin⁄ C23 is

a downstream mediator of Hsp70’s antiapoptosis effects and it functions at the level of protein stability

in cardiomyocytes It is our hope that such studies on the mechanisms of apoptosis in cardiomyocytes will provide a molecular basis for new therapeutic strate-gies targeting specific pathways to treat human heart disease

Materials and methods

Animals

Neonatal Wistar rats (1-3 days) were purchased from the Animal Resource Center of Center South University The following procedures were approved by the Institutional Animal Care and Use Committee of the Center South Uni-versity, and were carried out in accordance with the National Institutes of Health Guide for the Care and Use

of Laboratory Animals All efforts were made to minimize the number of animals used and their suffering

H2O2 pcDNA3.1

100

10

Time (h)

pcDNA3.1 pcDNA3.1-C23

Bcl-2

GAPDH

A

B

Fig 5 Effect of nucleolin ⁄ C23 on Bcl-2 protein expression and

mRNA stability in the presence or absence of H 2 O 2 (A) Western

blot analyses showing the effect of nucleolin ⁄ C23 on Bcl-2 protein

expression Total cellular proteins were isolated and separated by

12% SDS ⁄ PAGE and analysed by immunoblotting with anti-Bcl-2.

Immunoblot analyses with GAPDH antiserum were used as the

protein loading control (B) Real-time PCR showing the effect of

nucleolin ⁄ C23 on Bcl-2 mRNA stability Cells transfected with

pcDNA3.1-C23 or the empty vector were cultured in the absence

or presence of H2O2(0.5 m M ) for 2 h Actinomycin D (5 lgÆmL)1)

was then added to the media and the cells were further incubated

for various times (0–3 h) Total RNAs were prepared and subjected

to real-time PCR analyses The amount of Bcl-2 mRNA was

normal-ized by that of GAPDH All experiments were performed in

tripli-cate and shown here by one representative *P < 0.05 versus

pcDNA3.1-transfected control group.

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Cell culture and treatment

Primary cultures of neonatal rat cardiomyocytes were

culti-vated as previously described [33,34] Briefly, hearts from

neonatal Wistar rats (1–3 days after birth) were removed, minced and trypsinized at 37C with gentle stirring in D-Hanks buffer containing 0.1% trypsin (Gibco, Rockville,

MD, USA) The cells were then centrifuged and resus-pended in Dulbecco’s modified Eagle’s medium (DMEM, Gibco) containing 15% fetal bovine serum (Hyclone, Logan, UT, USA) After incubation at 37C for 120 min, the suspended cardiomyocytes were seeded at a density of

5· 105cellsÆmL)1 All cells were cultured in DMEM con-taining 15% fetal bovine serum for 24 h before the initia-tion of experiments 5-Bromo-2¢-deoxyuridine (Sigma, St Louis, MO, USA) (0.1 mmolÆL)1) was added to the culture for 36 h to inhibit the proliferation of nonmyocytes H2O2

was first diluted in phosphate-buffered saline (PBS, pH 7.4) and further diluted in culture medium to a final concentra-tion of 0.5 mmolÆL)1 for all treatments Cycloheximide (Sigma) was diluted in the medium to a final concentration

of 5 lgÆmL)1

Quantification of apoptotic cells

At the predetermined time points after H2O2exposure, cells were detached from tissue culture plates with tryp-sin⁄ EDTA or cell scrapers, and collected together with the nonadherent cells After centrifugation at 500 g for 5 min, the cells were fixed with 4% paraformaldehyde for 30 min

at room temperature and then washed once with PBS The fixed cells were then incubated with Hoechst 33258 (50 ngÆmL)1) for 30 min at room temperature, and washed

60

Hsp70/C + NCL/C23-AsODNs Hsp70/C + NCL/C23-ScrODNs

Time (h) of H2O2 exposure

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* 50

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Hsp70/C + NCL/C23-ScrODNs

Time (h) of H2O2 exposure

0

0.5

1

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2

3

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Hsp70/C cells

Nucleolin/C23

Hsp70

GAPDH

A

B

C

D

Fig 6 Potentiation of apoptosis in Hsp70-overexpressed cells by nucleolin ⁄ C23 antisense oligomer (A) Transfection efficiency of phosphorothioate oligodeoxynucleotides in primary cultures of car-diomyocytes FITC-labelled phosphorothioate oligodeoxynucleotides were transfected into cells with Lipofectamine 2000 and cells were stained with Hoechst 33258 Right, the image under blue fluores-cence channel showing all cells with nuclear Hoechst staining; left, image under green fluorescence channel showing only cells posi-tive for FITC-labelled oligomers (B) Knocking-down of nucleo-lin ⁄ C23 in cardiomyocytes The Hsp70-transfected cardiomyocytes (Hsp70 ⁄ C) were cotransfected with nucleolin ⁄ C23 scrambled (NCL ⁄ C23-ScrODNs) or antisense (NCL ⁄ C23-AsODNs) oligomers After 36 h, cells were harvested for western blot analysis with monoclonal antibody against nucleolin ⁄ C23 (NCL ⁄ C23) or GAPDH (C) Determination of the percentage of apoptotic cells by Hoechst staining Hsp70 ⁄ C cells were cotransfected with NCL ⁄ C23-Scr-ODNs or NCL ⁄ C23-AsODNs and then treated with H 2 O 2 for 6–36 h The results from three independent experiments are shown as mean ± SEM *P < 0.05 versus NCL ⁄ C23-ScrODNs group (D) Determination of percentage of apoptotic cells by cas-pase-3 activity assay Hsp70 ⁄ C cells were transfected and treated

as above, and assayed for caspase-3 activity Data were obtained from four independent experiments *P < 0.05 versus NCL ⁄ C23-ScrODNs group.

Trang 8

again with PBS Cells were mounted on to glass slides and

examined by fluorescence microscopy Apoptotic cells were

identified by the condensation and fragmentation of their

nuclei The percentage of apoptotic cells was calculated as

the number of apoptotic cells divided by the total number

of cells counted A minimum of 500 cells were counted for

each slide

Flow cytometry

Both adherent and floating cells were collected after treatment, washed with ice-cold PBS and stained with FITC-conju-gated annexin V (BD Biosciences, Franklin Lakes, NJ, USA) and PI for 20 min at room temperature in the dark The stained cells were then analysed by a flow cytometer

A

B

Fig 7 Flow cytometry analysis of apoptosis

with annexin V–FITC ⁄ PI double staining.

Hsp70-transfected cardiomyocytes

(Hsp70 ⁄ C) were cotransfected with the

nucleolin ⁄ C23 scrambled (NCL ⁄

C23-ScrO-DNs) or antisense (NCL⁄ C23-AsOC23-ScrO-DNs)

oligomers Twenty-four hours later, they

were treated with 0.5 mmolÆL)1H2O2for 6

or 12 h Cells were harvested and

pro-cessed for annexin V–FITC and PI costaining

and analysed by flow cytometry (A) Q3

cells were the control cells, Q4 cells were

cells at the early apoptosis stage, Q2 cells

were cells at the late apoptosis stage, and

Q1 cells were necrotic cells The percentage

of apoptotic cells was also calculated (B).

The results are representative of three

independent experiments Data are the

mean ± SEM of triplicate samples.

*Significant difference (P < 0.05) versus the

pcDNA3.1 control group; #significant

difference (P < 0.05) versus the control

group.

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(Beckman Coulter, Fullerton, CA, USA) FITC-conjugated

annexin V binds to phosphatidylserine molecules only

pres-ent at the surface of apoptotic cells where they were

trans-located from the internal side of the plasma membrane

during apoptosis Cells were simultaneously stained with PI

to discriminate membrane-permeable necrotic cells from

FITC-labelled apoptotic cells Apoptotic cells were

identi-fied as those positive for annexin V–FITC staining but

negative for PI staining, and the percentage of apoptotic

cells in the total number of cells was calculated

Western blot analyses

Cells were washed with PBS and collected by

centrifuga-tion Cell pellets were resuspended with 5 volumes of cold

lysis buffer [50 mmolÆL)1 Tris⁄ HCl (pH 7.5), 250

mmo-lÆL)1 NaCl, 5 mmolÆL)1 EDTA, 50 mmolÆL)1 NaF, 0.5%

Nonidet P-40] containing a protease inhibitor mixture

(Roche Applied Science, Burgess Hill, UK) The cell lysate

was incubated on ice for 30 min and centrifuged at

10 000 g for 10 min at 4C The protein concentration of

the supernatant was determined using the Bradford assay

(Bio-Rad, Hercules, CA, USA) Equal amounts of protein

(5–10 lg) were loaded on to and separated by SDS⁄ PAGE

and transferred to a nitrocellulose membrane The blot

was blocked with 2% albumin in 20 mmolÆL)1 Tris⁄ HCl,

pH 8.0, 150 mmolÆL)1 NaCl, 0.1% Tween 20 (TBST)

overnight at 4C and then incubated with the rabbit

anti-C23 (Sigma) or anti-(glyceraldehyde-3-phosphate

dehydro-genase) (GAPDH; Santa Cruz Biotechnology, Santa Cruz,

CA, USA) for 2 h After washing with TBST buffer three

times for 15 min each, the blot was incubated with

horse-radish peroxidase-conjugated goat anti-mouse IgG (diluted

1 : 2000 in TBST buffer) at room temperature for 1 h,

and finally washed three times with TBST for 15 min

each Immunoreactivity was visualized using the enhanced

chemiluminescence reaction (Amersham, Piscataway, NJ,

USA)

Caspase activity assay

The activity of caspase-3 was measured by in vitro

sub-strate-cleavage reactions using a commercial kit according

to the manufacturer’s protocol (R&D Systems,

Minneapo-lis, MN, USA) Briefly, cells cultured in 60 mm dishes were

treated with 0.5 mmolÆL)1H2O2for the indicated time

peri-ods The cells (5· 106

) were lysed with 250 lL chilled cell lysis buffer on ice for 10 min After centrifugation

(10 000 g, 1 min, 4C), the protein concentration in the

supernatant was determined using the BioRad protein

assay Supernatants containing equal amounts of protein

(corresponding to  5 · 105

cells) were used for caspase-3 colorimetric assays After protein samples were incubated

with substrates at 37C for 1.5 h, the absorbance at

405 nm was measured using a microtitre plate reader

(Molecular Devices, Sunnyvale, CA, USA) Fold increases

in caspase-3 activity over that before treatment were deter-mined

Lipofectamine-mediated gene transfection

Transfection of cells was carried out following the manu-facturer’s instructions (Lipofectamine 2000, Invitrogen, Carlsbad, CA, USA) Briefly,  5 · 105

cells in 5 mL appropriate complete growth medium per flask were grown

at 37C in a CO2incubator until the cells reached 70–80% confluence (24 h) After rinsing with serum-free and antibi-otic-free medium, the cells were transfected with pcDNA3.1-Hsp70 (HspA1A was a gift from I Benjamin, University of Utah Health Sciences Center) (experimental group) or pcDNA3.1 (vector control), at 8 lg DNA per

20 lL Lipofectamine, followed by incubation at 37C in a

CO2incubator for 6 h The medium was then replaced with DMEM culture medium containing 20% fetal bovine serum

Nucleolin/C23 antisense oligodeoxynucleotide

The phosphorothioate oligodeoxynucleotides used in this study were manufactured by Bioasia Biotech (Shanghai, China) The sequence of nucleolin⁄ C23 antisense oli-godeoxynucleotide (NUL⁄ C23-AsODNs), corresponding to the rat nucleolin⁄ C23 translation initiation site, was 5¢-TG CGAGTTTCACCATGATGGC-3¢ A scrambled nucleolin ⁄ C23 oligodeoxynucleotide (NUL⁄ C23-ScrODNs; 5¢-CTGA TGTCACGTCCATGTGAG-3¢) was used as the control The oligodeoxynucleotides were diluted in 10 mmolÆL)1 Tris (pH 7.4) and 1 mmolÆL)1EDTA and kept at)20 C

RT-PCR

Total RNAs were prepared with the Rneasy kit (Qiagen, Cambridge, MA, USA) according to the manufacturer’s instructions and 2 lg samples were reverse transcribed using oligo(dT) primers The levels of gene expression were quanti-fied by real-time PCR, using a QuantiTect SYBR Green PCR Kit (Qiagen) and the 7500 Fast Real-Time PCR system (Applied Biosystems, Foster City, CA, USA) under the following conditions: 40 sequential cycles, each including

95C for 10 s and 60 C for 10 s Sequences of primers spe-cific to each target cDNA were: nucleolin, forward, 5-CA ATCAGGCTGGAGTTGCAAG-3; and reverse, 5-TGGC CCAGTCCAAGGTAACTT-3 (amplicon size: 282 bp);

and reverse, 5-TCCACCACCCTGTTGCTGTA-3 (size:

440 bp) The specificity of PCR products was verified by melt-ing curve analysis and electrophoresis on agarose gels The comparative threshold cycle method and an internal control (GAPDH) were used to normalize target gene expression

Trang 10

Statistical analyses

Data are presented as mean ± standard error of the mean

(SEM) of the values obtained from the indicated number of

independent experiments Differences between two groups

were analysed by unpaired Student’s t-test Differences

between three or more groups were analysed by one-way

ANOVA followed by Student–Newman–Keuls posthoc test

P< 0.05 was considered statistically significant

Acknowledgements

This study was supported by grants from the National

Basic Research Program of China (2007CB512007),

the National Natural Science Foundation of China

(30700290) and Special Funds for PhD Training from

The Ministry of Education of China (20060533009)

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